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Title: Resolution Function Theory in Piezoresponse Force Microscopy: Domain Wall Profile, Spatial Resolution, and Tip Calibration

Journal Article · · Physical Review B

Piezoresponse force microscopy (PFM) has emerged as a primary tool for imaging, domain engineering, and switching spectroscopy on ferroelectric materials. Quantitative interpretation of PFM data, including measurements of the intrinsic width of the domain walls, determination of geometric parameters of the domain below the tip in local hysteresis loop measurements, as well as interpretation of local switching and coercive biases in terms of material properties and switching mechanisms, requires reliable knowledge on electrostatic and strain field structures produced by the tip. Using linear imaging theory, we develop a theoretical approach for the interpretation of these measurements and the determination of tip parameters from a suitable calibration standard. The resolution and object transfer functions in PFM are derived, and the effect of material parameters on resolution is determined. Closed-form solutions for domain-wall profiles in vertical and lateral PFM and signals from cylindrical and nested cylindrical domains in transversally isotropic piezoelectric are derived for point-charge and sphere-plane geometries of the tip.

Research Organization:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC)
DOE Contract Number:
DE-AC05-00OR22725
OSTI ID:
965286
Journal Information:
Physical Review B, Vol. 75, Issue 17; ISSN 1098-0121
Country of Publication:
United States
Language:
English