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Title: The reduction of reactor effluent water radionuclides by the addition of sodium silicate to process water; 105D half plant addition

Thesis/Dissertation ·
OSTI ID:6585680

Research and development on the reduction of radionuclides discharged to the Columbia River in reactor effluent is described. Sodium silicate was added to the process water supplying 1/2 of the D Reactor at an average concentration of 15 ppm, which gradually reduced the radionuclide concentration entering the Columbia River. After the 8th month an equilibrium condition was reached, and the levels of /sup 76/As, /sup 51/Cr, /sup 239/Np, /sup 32/P, /sup 124/Sb, and /sup 64/Cu were lowered by factors of about 9.0, 7.0, 6.0, 3.0, 3.0 to 5.0 and 1.5 respectively. Concentration of /sup 65/Zn remained unchanged. The only significant increases were due to /sup 24/Na, and trace amounts of /sup 140/La and other rare earth elements. Cobalt-60 and /sup 46/Sc behaved erratically. The studies suggest that if sodium silicate were used on a full scale (5 reactor basis), river concentration of radionuclides could be proportionally reduced.

Research Organization:
Pacific Northwest Lab., Richland, WA (USA)
OSTI ID:
6585680
Resource Relation:
Other Information: Thesis (Ph.D.)
Country of Publication:
United States
Language:
English