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Title: Measurements and calculations of radionuclides created by [sup 181]Ta([gamma],xn yp) reactions for bremsstrahlung photons produced by 150-MeV electrons

Journal Article · · Nuclear Science and Engineering; (United States)
OSTI ID:6521489
;  [1]
  1. Oak Ridge National Lab., TN (United States)

Twenty-three radionuclides, including isomers, from [sup 168m]Lu to [sup 180]Ta, having half-lives between 7 min and 1.4 yr, produced by photon interactions with a sample of elemental tantalum, were observed in decay gamma-ray data obtained using high-resolution detection systems. Yields of production range over six orders of magnitude. The measured yield data for masses [>=] 171 were compared with calculated values. Good agreement was obtained for masses [>=] 174, but for lighter masses, the calculations tend to overestimate the experimental yields by up to a factor of 5. An empirical 'rule-or-two- is proposed, governing reduction in measured mass yield for each additional emitted nucleon following ([gamma], 3n) reactions. These results should have practical use not only for present electron accelerator operation but also for shielding calculations needed for future accelerator designs and applications.

OSTI ID:
6521489
Journal Information:
Nuclear Science and Engineering; (United States), Vol. 114:2; ISSN 0029-5639
Country of Publication:
United States
Language:
English