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Title: Spectrum-averaged cross-section measurement of /sup 103/Rh(n,n)/sup 103m/Rh in the /sup 252/Cf fission neutron spectrum

Journal Article · · Nucl. Sci. Eng.; (United States)
OSTI ID:6059031

Because of the similarity in energy dependence of the /sup 103/Rh(n,n') differential cross section to the kerma muscle response function for neutrons, rhodium may be useful as a neutron kerma monitor. In support of its use as a neutron monitor, the spectrum-averaged cross section sigma-bar has been measured for a /sup 252/Cf fission neutron spectrum. Pairs of thin rhodium samples were irradiated on opposite sides of a thinly encapsulated /sup 252/Cf neutron source. The neutron emission rate of the /sup 252/Cf source was determined by the manganous sulfate (MnSO/sub 4/) bath technique. In this method, the californium source emission rate is determined by comparison to the known emission rate of NBS-I, a standard radium-beryllium neutron source. The neutron fluence incident on the rhodium samples is determined from the californium source strength, average sample-to-source distance, and the duration of the irradiation. Corrections are made for neutron scattering saturation of activity, and attenuation of the X rays by the sample during counting. The X rays were detected with an intrinsic germanium detector designed specifically for low-energy X-ray detection. The activity was not determined by absolute counting so that the final results depend on the value of P/sub KAPPAx/, to total KAPPA X-ray emission probability. The results of five separate irradiations yield a value of sigma-bar . P/sub KAPPAx/ = 62.3 +- 1.9 mb. Using the most recently published value of P/sub KAPPAx/ gives a value of sigma-bar = 739 +- 22 mb. A discussion of systematic uncertainties is given.

Research Organization:
National Bureau of Standards, Gaithersburg, MD (US)
OSTI ID:
6059031
Journal Information:
Nucl. Sci. Eng.; (United States), Vol. 100:1
Country of Publication:
United States
Language:
English