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Title: Low-temperature rupture behavior of Zircaloy clad pressurized water reactor spent fuel rods under dry storage conditions

Technical Report ·
OSTI ID:5244914

Creep rupture studies on five well-characterized Zircaloy clad pressurized water reactor spent fuel rods, which were pressurized to a hoop stress of approximately 145 MPa, were conducted for up to 2101 h at 323/sup 0/C. The conditions were chosen for limited annealing of in-reactor irradiation-hardening. No cladding breaches occurred, although significant hydride agglomeration and reorientation took place in rods that cooled under stress. Observations are interpreted in terms of a conservatively modified Larson-Miller curve to provide a lower bound on permissible maximum dry-storage temperatures, assuming creep rupture as the life-limiting mechanism. If hydride reorientation can be ruled out during dry storage, 305/sup 0/C is a conservative lower bound, based on the creep rupture mechanism, for the maximum storage temperature of rods with irradiation hardened cladding to ensure a 100-year cladding lifetime in an inert atmosphere. An oxidizing atmosphere reduces the lower bound on the maximum permissible storage temperature by approx. 5/sup 0/C. While high-temperature tests based on creep rupture as the limiting mechanism indicate that storage at temperatures between 400/sup 0/C and 440/sup 0/C may be feasible for rods which are annealed, tests to study rod performance in the 305/sup 0/ to 400/sup 0/C temperature range have not been conducted. 37 references, 10 figures, 7 tables.

Research Organization:
Hanford Engineering Development Lab., Richland, WA (USA); Battelle Columbus Labs., OH (USA)
DOE Contract Number:
AC06-76FF02170
OSTI ID:
5244914
Report Number(s):
HEDL-7400; ON: DE84007170
Country of Publication:
United States
Language:
English