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Title: Chemical cycles and health risks of some crustal nuclides

Thesis/Dissertation ·
OSTI ID:5179840

This dissertation describes and utilizes an approach for assessing long term health risks due to dispersion of naturally occurring radionuclide series and chemical toxins by normal and altered landscape chemical cycles. In particular, the health risks resulting from geochemical mobilizations of arsenic, lead, uranium and radium are considered. Based on a review of toxic waste hazard-measures and risk assessment studies, a general expression is developed for quantifying health risks imposed by the introduction of toxic materials to components of the total environment. This general measure deals with long term interactions within and between the internal human environment and the external biogeochemical environment. Health hazards are expressed as dose factors which convert environmental concentrations into a corresponding dose field (organ doses in rad for radionuclides; daily intake for toxic elements). The dose field is translated into population health risk expressed as lifetime cancer risk for carcinogens and average blood levels for other toxins. The landscape cell (or prism) is presented as a tool for visualizing and mapping toxic material cycles near the crustal surface. The overall process is incorporated in the GEOTOX code which is a geochemical systems model for describing the dynamics of crustal toxins within a landscape and the resulting health risks. GEOTOX is used to investigate the response of regional landscapes to increased soil and rock inventories of /sup 238/U, /sup 226/Ra, arsenic and lead. It is found that each decay series of element imposes a hazard by its behavior in the total environment that can not be quantified by a similar measure of toxicity.

Research Organization:
California Univ., Los Angeles (USA)
OSTI ID:
5179840
Resource Relation:
Other Information: Thesis (Ph. D.)
Country of Publication:
United States
Language:
English

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