Luminescent MOFs (LMOFs): recent advancement towards a greener WLED technology

Karmakar, Avishek; Li, Jing

doi:10.1039/d2cc03330e

Title: Luminescent MOFs (LMOFs): recent advancement towards a greener WLED technology

Journal Article · Tue Aug 16 00:00:00 EDT 2022 · ChemComm

DOI:https://doi.org/10.1039/d2cc03330e· OSTI ID:2305676

Karmakar, Avishek ^[1];

^[1]

Rutgers University, Piscataway, NJ (United States)

The replacement of traditional incandescent, halogen and fluorescent lamps by white light emitting diodes (WLEDs) is expected to reduce the global electricity consumption by one-third by 2030, according to the US Department of Energy. The current WLED technology uses rare-earth element (REE) based phosphor materials, which, not only is cost-intensive but also constitutes an environmental concern. Hence, researchers are in a quest for a new-generation of opto-electronic materials that can replace the conventional phosphors in WLEDs and thus aim towards a cleaner and more energy efficient lighting technology for the future. Luminescent metal–organic frameworks (LMOFs) have recently emerged as a new sub-class of MOFs which have demonstrated enormous potential for applications in sensing, imaging, optoelectronics and in solid-state lighting (SSL) technology. LMOFs could be game changers as lighting phosphors due to advantages such as high luminescence quantum yield, tunable excitation and emission which can be achieved by rational design and optimization of metal centers, linkers, and the guest molecules, facile fabrication into devices, and structural robustness. These clear advantageous features of LMOFs make them score over other contemporary materials, and enable them to be futuristic phosphor materials for WLED technology. Here, in this feature article, we will provide an overview of the most recent developments of LMOF-based phosphor materials for SSL with a special focus on WLED technology. The emphasis will be centered around REE-free LMOFs, as the aim is to direct the attention of the readers towards a more viable and greener lighting technology.

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Research Organization:: Wake Forest University, Winston-Salem, NC (United States); Wake Forest Univ., Winston-Salem, NC (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: SC0019902

OSTI ID:: 2305676

Alternate ID(s):: OSTI ID: 1886727; OSTI ID: 1978855; OSTI ID: 2305678

Journal Information:: ChemComm, Vol. 58, Issue 77; ISSN 1359-7345

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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Encapsulation of Dyes in Luminescent Metal-Organic Frameworks for White Light Emitting Diodes Sun, Zhihong; Khurshid, Aaqib; Sohail, Muhammad Nanomaterials, Vol. 11, Issue 10 https://doi.org/10.3390/nano11102761	journal	October 2021
The rules and roles of metal–organic framework in combination with molecular dyes Ryu, Unjin; Lee, Hyeon Shin; Park, Kyo Sung Polyhedron, Vol. 154 https://doi.org/10.1016/j.poly.2018.07.043	journal	November 2018
White‐Light Emission from Dual‐Way Photon Energy Conversion in a Dye‐Encapsulated Metal–Organic Framework Wang, Zheng; Zhu, Cheng‐Yi; Mo, Jun‐Ting Angewandte Chemie International Edition, Vol. 58, Issue 29 https://doi.org/10.1002/anie.201905186	journal	July 2019
Confinement of Luminescent Guests in Metal–Organic Frameworks: Understanding Pathways from Synthesis and Multimodal Characterization to Potential Applications of LG@MOF Systems Gutiérrez, Mario; Zhang, Yang; Tan, Jin-Chong Chemical Reviews, Vol. 122, Issue 11 https://doi.org/10.1021/acs.chemrev.1c00980	journal	April 2022
Dye Encapsulated Metal-Organic Framework for Warm-White LED with High Color-Rendering Index Cui, Yuanjing; Song, Tao; Yu, Jiancan Advanced Functional Materials, Vol. 25, Issue 30 https://doi.org/10.1002/adfm.201501756	journal	July 2015
Warm-White-Light-Emitting Diode Based on a Dye-Loaded Metal–Organic Framework for Fast White-Light Communication Wang, Zhiye; Wang, Zi; Lin, Bangjiang ACS Applied Materials & Interfaces, Vol. 9, Issue 40 https://doi.org/10.1021/acsami.7b11277	journal	September 2017
Introduction of Red-Green-Blue Fluorescent Dyes into a Metal-Organic Framework for Tunable White Light Emission Wen, Yuehong; Sheng, Tianlu; Zhu, Xiaoquan Advanced Materials, Vol. 29, Issue 37 https://doi.org/10.1002/adma.201700778	journal	August 2017
Nanovesicular MOF with Omniphilic Porosity: Bimodal Functionality for White-Light Emission and Photocatalysis by Dye Encapsulation Samanta, Debabrata; Verma, Parul; Roy, Syamantak ACS Applied Materials & Interfaces, Vol. 10, Issue 27 https://doi.org/10.1021/acsami.8b06363	journal	June 2018
Three Models To Encapsulate Multicomponent Dyes into Nanocrystal Pores: A New Strategy for Generating High-Quality White Light Liu, Xiao-Yuan; Xing, Kai; Li, Yang Journal of the American Chemical Society, Vol. 141, Issue 37 https://doi.org/10.1021/jacs.9b07236	journal	August 2019
Core–Shell Structured Cyclodextrin Metal–Organic Frameworks with Hierarchical Dye Encapsulation for Tunable Light Emission Chen, Yifu; Yu, Bo; Cui, Yingdan Chemistry of Materials, Vol. 31, Issue 4 https://doi.org/10.1021/acs.chemmater.8b04126	journal	February 2019
Polyurethane-coated luminescent dye@MOF composites for highly-stable white LEDs Tang, Ying; Cao, Wenqian; Yao, Lijia Journal of Materials Chemistry C, Vol. 8, Issue 35 https://doi.org/10.1039/D0TC02887H	journal	January 2020
Encapsulating carbon quantum dot and organic dye in multi-shell nanostructured MOFs for use in white light-emitting diode Lu, Yantong; Wang, Shuo; Yu, Kuangli Microporous and Mesoporous Materials, Vol. 319 https://doi.org/10.1016/j.micromeso.2021.111062	journal	May 2021
Efficient and tunable white-light emission of metal–organic frameworks by iridium-complex encapsulation Sun, Chun-Yi; Wang, Xin-Long; Zhang, Xiao Nature Communications, Vol. 4, Issue 1 https://doi.org/10.1038/ncomms3717	journal	November 2013
A luminescent metal–organic framework with mixed-linker strategy for white-light-emitting by iridium-complex encapsulation Zhang, Shu-Ran; Xu, Guang-Juan; Xie, Wei Inorganic Chemistry Communications, Vol. 123 https://doi.org/10.1016/j.inoche.2020.108359	journal	January 2021
A stable Alq3@MOF composite for white-light emission Xie, Wei; He, Wen-Wen; Du, Dong-Ying Chemical Communications, Vol. 52, Issue 16 https://doi.org/10.1039/C5CC08703A	journal	January 2016
Fluorescent carbon dots and their sensing applications Sun, Xiangcheng; Lei, Yu TrAC Trends in Analytical Chemistry, Vol. 89 https://doi.org/10.1016/j.trac.2017.02.001	journal	April 2017
Carbon Dots: A New Type of Carbon-Based Nanomaterial with Wide Applications Liu, Junjun; Li, Rui; Yang, Bai ACS Central Science, Vol. 6, Issue 12 https://doi.org/10.1021/acscentsci.0c01306	journal	December 2020
Rare earth-free composites of carbon dots/metal–organic frameworks as white light emitting phosphors Wang, Aiwu; Hou, Yun-Long; Kang, Fengwen Journal of Materials Chemistry C, Vol. 7, Issue 8 https://doi.org/10.1039/C8TC04171G	journal	January 2019
Improving stability against desolvation and mercury removal performance of Zr(iv)–carboxylate frameworks by using bulky sulfur functions He, Yonghe; Hou, Yun-Long; Wong, Yan-Lung Journal of Materials Chemistry A, Vol. 6, Issue 4 https://doi.org/10.1039/C7TA06118H	journal	January 2018
Solid Confinement of Quantum Dots in ZIF-8 for Efficient and Stable Color-Conversion White LEDs Ying, Wen; Mao, Yiyin; Wang, Xiaobing ChemSusChem, Vol. 10, Issue 7 https://doi.org/10.1002/cssc.201700223	journal	March 2017
Linker Engineering toward Full-Color Emission of UiO-68 Type Metal–Organic Frameworks Wu, Shenjie; Ren, Daming; Zhou, Kang Journal of the American Chemical Society, Vol. 143, Issue 28 https://doi.org/10.1021/jacs.1c04810	journal	July 2021
Tuning and Directing Energy Transfer in the Whole Visible Spectrum through Linker Installation in Metal–Organic Frameworks Ren, Daming; Xia, Hai‐Lun; Zhou, Kang Angewandte Chemie International Edition, Vol. 60, Issue 47 https://doi.org/10.1002/anie.202110531	journal	October 2021
Full-Color Emission in Multicomponent Metal–Organic Frameworks via Linker Installation Han, Guodong; Wu, Shenjie; Zhou, Kang Inorganic Chemistry, Vol. 61, Issue 8 https://doi.org/10.1021/acs.inorgchem.1c02977	journal	December 2021
Solid State Multicolor Emission in Substitutional Solid Solutions of Metal–Organic Frameworks Newsome, Wesley J.; Ayad, Suliman; Cordova, Jesus Journal of the American Chemical Society, Vol. 141, Issue 28 https://doi.org/10.1021/jacs.9b05191	journal	June 2019
Metal-organic frameworks for white light emission: From synthesis to device fabrication Chiu, Nan-Chieh; Smith, Kyle T.; Stylianou, Kyriakos C. Coordination Chemistry Reviews, Vol. 459 https://doi.org/10.1016/j.ccr.2022.214441	journal	May 2022
Dual‐Guest Functionalized Zeolitic Imidazolate Framework‐8 for 3D Printing White Light‐Emitting Composites Chaudhari, Abhijeet K.; Tan, Jin‐Chong Advanced Optical Materials, Vol. 8, Issue 8 https://doi.org/10.1002/adom.201901912	journal	February 2020
Electroluminescent Guest@MOF Nanoparticles for Thin Film Optoelectronics and Solid‐State Lighting Gutiérrez, Mario; Martín, Cristina; Van der Auweraer, Mark Advanced Optical Materials, Vol. 8, Issue 16 https://doi.org/10.1002/adom.202000670	journal	June 2020
A Systematic Approach to Achieving High Performance Hybrid Lighting Phosphors with Excellent Thermal- and Photostability Fang, Yang; Liu, Wei; Teat, Simon J. Advanced Functional Materials, Vol. 27, Issue 3 https://doi.org/10.1002/adfm.201603444	journal	December 2016

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