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Title: Performance Assessment for Closure of the Calcined Solids Storage Facility at the INL Site - 19289

Conference ·
OSTI ID:23003044
 [1]; ;  [2];  [3]
  1. K-Spar Inc, Idaho Falls, Idaho (United States)
  2. Fluor Idaho, LLC Idaho Falls, Idaho (United States)
  3. North Wind Portage, Colorado Springs, Colorado (United States)

The Calcined Solids Storage Facility is composed of six discrete stainless steel 'bin sets' at the Idaho Nuclear Technology and Engineering Center at the INL Site. Approximately 4,440 m{sup 3} of the dry, granular calcine waste is stored in the facility. Closure of the facility will entail removal of the calcine waste followed by grouting. A 5-cm thick residual amount of calcine was assumed to remain at the bottom of the bins. Important radionuclides in the residual layer for the groundwater pathway were identified as the fission and activation products Tc-99, Se-79, I-129, Cs-135, H-3, and actinides Pu-239, and Pu-240. The stainless-steel bins prevent near-term release of grouted residual calcine waste to the environment. Future releases were conservatively based on the corrosion rate of the weld seams on the stainless-steel bins, which site-specific studies measured mean tunnel corrosion rates of 0.0132 mm/yr with a coefficient of variation of 0.333. Based on tunnel corrosion rates, mean bin hydrologic containment times were estimated to be between 238 years and 1,191 years, depending on the thickness of the bin. Any breach in the weld seam was assumed to result in water flow and radionuclide leaching through the bin. The structural integrity of the bin was assumed to be controlled by the general stainless-steel corrosion rate, which was much slower (3.5 x 10{sup -5} mm/yr), resulting in structural integrity times between 24,000 years to over 100,000 years. A mixing-cell model was used to compute water flow and transport through the hydrologically failed bins and the vadose zone. Credit was taken for the geochemical properties of the grout used to fill the bins at closure, which significantly slows the releases from the bins for key radionuclides like Tc-99. A semi-analytical model for three-dimensional dissolved-phase transport in an aquifer of constant unidirectional flow, infinite length and width, and finite thickness was used to compute concentrations in the aquifer across the model domain for a time varying source. Cumulative impacts from all bin sets were calculated by summation across the bin set sources that were superimposed on a uniform Cartesian grid. Effective doses were calculated for direct groundwater ingestion from wells located 100-m downgradient from each of the bin sets and ingestion of meat, milk, and vegetables irrigated with water derived from the well. Intruder doses were based on a well drilled through the grouted waste and cuttings spread around a home site after a 500-year institutional control period. Peak doses during the 1,000-year compliance period were less than 5% of the 250 μSv/yr (25 mrem/yr) performance objective and intruder doses were generally less 5% of the of the 5000 μSv/yr (500 mrem) and 1000 μSv/yr (100 mrem) performance objective for acute and chronic intruder exposure, respectively. Groundwater concentrations were all less than the maximum contaminant limits. In all cases, doses were highest for the oldest bin set because, compared to the other bin sets, it had the highest radionuclide concentrations in the calcine waste. The performance assessment results indicate that performance objectives can be met leaving considerably more than 5-cm of residual calcine waste in the bin sets. (authors)

Research Organization:
WM Symposia, Inc., PO Box 27646, 85285-7646 Tempe, AZ (United States)
OSTI ID:
23003044
Report Number(s):
INIS-US-21-WM-19289; TRN: US21V1160043377
Resource Relation:
Conference: WM2019: 45. Annual Waste Management Conference, Phoenix, AZ (United States), 3-7 Mar 2019; Other Information: Country of input: France; 17 refs.; available online at: https://www.xcdsystem.com/wmsym/2019/index.html
Country of Publication:
United States
Language:
English