Phase-only shaped laser pulses in optimal control theory: Application to indirect photofragmentation dynamics in the weak-field limit
Journal Article
·
· Journal of Chemical Physics
- Department of Chemistry, Building 207, Technical University of Denmark, DK-2800, Kongens Lyngby (Denmark)
We implement phase-only shaped laser pulses within quantum optimal control theory for laser-molecule interaction. This approach is applied to the indirect photofragmentation dynamics of NaI in the weak-field limit. It is shown that optimized phase-modulated pulses with a fixed frequency distribution can substantially modify transient dissociation probabilities as well as the momentum distribution associated with the relative motion of Na and I.
- OSTI ID:
- 22047162
- Journal Information:
- Journal of Chemical Physics, Vol. 136, Issue 4; Other Information: (c) 2012 American Institute of Physics; Country of input: International Atomic Energy Agency (IAEA); ISSN 0021-9606
- Country of Publication:
- United States
- Language:
- English
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