skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Observation and Modeling of the Thermal Runaway of High-Capacity Pouch Cells Due to an Internal Short Induced by an Indenter

Journal Article · · Journal of Energy Storage

Owing to the complexity of coupling mechanical and electrical solvers for finite element analysis (FEA) of mechanical abuse of a battery, the simulation should be performed by incorporating a local short circuit model activated based on the status of battery elements. However, the approach should also consider various other conditions of the battery simulated, such as the initial state of charge (SOC), for precise simulations of the internal short. This study proposes an approach developed with a mechanical model and single-particle battery model, along with a reaction kinetics model for thermal abuse using LS-DYNA. Several key parameters were selected, such as the activation criteria, kinetic abuse and element integration points during the internal short circuit induced by the indenter. The impact of these key parameters in the FEA on thermal runaway response for various initial SOCs from 25 to 100 % were analyzed. The FEA results obtained were compared against experimental results with various parameters such as activation criterion of internal short, kinetic abuse based on accelerating rate calorimetry (ARC) data. Finally, the root causes of the discrepancy between the FEA and experimental results are discussed regarding integration point what solver can make difference during calculation.

Research Organization:
National Renewable Energy Laboratory (NREL), Golden, CO (United States)
Sponsoring Organization:
USDOE Office of Energy Efficiency and Renewable Energy (EERE)
DOE Contract Number:
AC36-08GO28308
OSTI ID:
1996397
Report Number(s):
NREL/JA-5700-87265; MainId:88040; UUID:557a4f67-e595-40a8-85f6-362e13d2b981; MainAdminID:70274
Journal Information:
Journal of Energy Storage, Vol. 72, Issue Part C
Country of Publication:
United States
Language:
English

References (47)

A review on the key issues for lithium-ion battery management in electric vehicles journal March 2013
Calibration and finite element simulation of pouch lithium-ion batteries for mechanical integrity journal March 2012
Modeling and short circuit detection of 18650 Li-ion cells under mechanical abuse conditions journal December 2012
Homogenized mechanical properties for the jellyroll of cylindrical Lithium-ion cells journal November 2013
Characterizing and modeling mechanical properties and onset of short circuit for three types of lithium-ion pouch cells journal February 2014
Prediction of shear crack formation of lithium-ion batteries under rod indentation: Comparison of seven failure criteria journal August 2019
Mechanical Deformation of Lithium-Ion Pouch Cells under in-plane Loads—Part II: Computational Modeling journal January 2020
Simulation and Optimization of the Dual Lithium Ion Insertion Cell journal January 1994
Development of First Principles Capacity Fade Model for Li-Ion Cells journal January 2004
Determination of the hydrogen diffusion coefficient in metal hydrides by impedance spectroscopy journal September 1998
Review of models for predicting the cycling performance of lithium ion batteries journal June 2006
Single-Particle Model for a Lithium-Ion Cell: Thermal Behavior journal January 2011
Review of simplified Pseudo-two-Dimensional models of lithium-ion batteries journal September 2016
Thermal Modeling of the Lithium/Polymer Battery journal January 1995
Thermal structures - Four decades of progress journal May 1992
Simultaneously Coupled Mechanical-Electrochemical-Thermal Simulation of Lithium-Ion Cells journal July 2016
A Simulation Framework for Battery Cell Impact Safety Modeling Using LS-DYNA journal January 2017
Two-way nonlinear mechanical-electrochemical-thermal coupled analysis method to predict thermal runaway of lithium-ion battery cells caused by quasi-static indentation journal November 2020
Transport Processes in a Li-ion Cell during an Internal Short-Circuit journal June 2020
Time Sequence Map for Interpreting the Thermal Runaway Mechanism of Lithium-Ion Batteries With LiNixCoyMnzO2 Cathode journal November 2018
Thermal Model of Cylindrical and Prismatic Lithium-Ion Cells journal January 2001
Modelling electro-thermal response of lithium-ion batteries from normal to abuse conditions journal November 2017
A Comprehensive Numerical and Experimental Study for the Passive Thermal Management in Battery Modules and Packs journal November 2022
A Multiphysics Computational Framework for Cylindrical Battery Behavior upon Mechanical Loading Based on LS-DYNA journal January 2019
Optimization of Lithium-Ion Battery Pouch Cell for Maximization of Energy Density while Preventing Internal Short Circuit Caused by Separator Failure under Crush Load journal March 2021
Integrated computation model of lithium-ion battery subject to nail penetration journal December 2016
Multiphysics computational framework for cylindrical lithium-ion batteries under mechanical abusive loading journal December 2017
High-efficiency multiphysics coupling framework for cylindrical lithium-ion battery under mechanical abuse journal March 2021
Identifiability of Generalized Randles Circuit Models journal November 2017
Modeling extreme deformations in lithium ion batteries journal May 2020
A multiphysics understanding of internal short circuit mechanisms in lithium-ion batteries upon mechanical stress abuse journal March 2022
Modelling Li-Ion Cell Thermal Runaway Triggered by an Internal Short Circuit Device Using an Efficiency Factor and Arrhenius Formulations journal January 2017
Analysis on the Fault Features for Internal Short Circuit Detection Using an Electrochemical-Thermal Coupled Model journal January 2018
Probing the Thermal Safety of Li Metal Batteries journal August 2020
Multi-field interpretation of internal short circuit and thermal runaway behavior for lithium-ion batteries under mechanical abuse journal January 2023
Comprehensive Battery Safety Risk Evaluation: Aged Cells versus Fresh Cells Upon Mechanical Abusive Loadings journal May 2023
Effect of State-of-Charge and Air Exposure on Tensile Mechanical Properties of Lithium-Ion Battery Electrodes journal January 2020
Thermal Model for Lithium Ion Battery Pack with Mixed Parallel and Series Configuration journal January 2011
Mechanical testing and macro-mechanical finite element simulation of the deformation, fracture, and short circuit initiation of cylindrical Lithium ion battery cells journal September 2012
Cubic Spline Regression for the Open-Circuit Potential Curves of a Lithium-Ion Battery journal January 2005
Extension of physics-based single particle model for higher charge–discharge rates journal February 2013
Thermal Modeling of the Lithium/Polymer Battery journal January 1995
Accelerating Rate Calorimetry Study on the Thermal Stability of Lithium Intercalated Graphite in Electrolyte. II. Modeling the Results and Predicting Differential Scanning Calorimeter Curves journal June 1999
Thermal runaway features of large format prismatic lithium ion battery using extended volume accelerating rate calorimetry journal June 2014
Effects of the environmental temperature and heat dissipation condition on the thermal runaway of lithium ion batteries during the charge-discharge process journal September 2017
Internal short circuit and failure mechanisms of lithium-ion pouch cells under mechanical indentation abuse conditions:An experimental study journal April 2020
State-of-Charge Dependence of Mechanical Response of Lithium-Ion Batteries: A Result of Internal Stress journal January 2018