A room temperature rechargeable Li2O-based lithium-air battery enabled by a solid electrolyte

Kondori, Alireza; Esmaeilirad, Mohammadreza; Harzandi, Ahmad Mosen; Amine, Rachid; Saray, Mahmoud Tamadoni; Yu, Lei; Liu, Tongchao; Wen, Jianguo; Shan, Nannan; Wang, Hsien-Hau; Ngo, Anh T.; Redfern, Paul C.; Johnson, Christopher S.; Amine, Khalil; Shahbazian-Yassar, Reza; Curtiss, Larry A.; Asadi, Mohammad

doi:10.1126/science.abq1347

Title: A room temperature rechargeable Li₂O-based lithium-air battery enabled by a solid electrolyte

Journal Article · Fri Feb 03 00:00:00 EST 2023 · Science

DOI:https://doi.org/10.1126/science.abq1347· OSTI ID:1960522

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^[1]; Harzandi, Ahmad Mosen ^[1]; Amine, Rachid ^[2]; Saray, Mahmoud Tamadoni ^[3]; Yu, Lei ^[4]; Liu, Tongchao ^[5];

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^[2]; Ngo, Anh T. ^[6];

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Illinois Institute of Technology, Chicago, IL (United States)
Argonne National Laboratory (ANL), Argonne, IL (United States). Materials Science Division
University of Illinois, Chicago, IL (United States)
Argonne National Laboratory (ANL), Argonne, IL (United States). Center for Nanoscale Materials (CNM)
Argonne National Laboratory (ANL), Argonne, IL (United States). Chemical Sciences and Engineering Division
Argonne National Laboratory (ANL), Argonne, IL (United States). Materials Science Division; University of Illinois, Chicago, IL (United States)

Lithium-air batteries have scope to compete with gasoline in terms of energy density. However, in most systems, the reaction pathways either involve one- or two-electron transfer, leading to lithium peroxide (Li₂O₂) or lithium superoxide (LiO₂), respectively. Kondori et al. investigated a lithium-air battery that uses a ceramic-polyethylene oxide–based composite solid electrolyte and found that it can undergo a four-electron redox reaction through lithium oxide (Li₂O) formation and decomposition (see the Perspective by Dong and Lu). The composite electrolyte embedded with Li₁₀GeP₂S₁₂ nanoparticles shows high ionic conductivity and stability and high cycle stability through a four-electron transfer process.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Office of Sustainable Transportation. Vehicle Technologies Office (VTO); USDOE Office of Science (SC), Basic Energy Sciences (BES); Illinois Institute of Technology; National Science Foundation (NSF); Keck Foundation; State of Illinois

Grant/Contract Number:: AC02-06CH11357; 262029 221E 2300; DMR-1809439; ECCS-1542205; DMR-1720139

OSTI ID:: 1960522

Journal Information:: Science, Vol. 379, Issue 6631; ISSN 0036-8075

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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