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Title: Atomic-Scale Modulation of Synthetic Magnetic Order in Oxide Superlattices

Journal Article · · Small Methods

Abstract Atomic‐scale precision control of magnetic interactions facilitates a synthetic spin order useful for spintronics, including advanced memory and quantum logic devices. Conventional modulation of synthetic spin order has been limited to metallic heterostructures that exploit Ruderman–Kittel–Kasuya–Yosida interaction through a nonmagnetic metallic spacer; however, they face issues arising from Joule heating and/or electric breakdown. The practical realization and observation of a synthetic spin order across a nonmagnetic insulating spacer will lead to the development of spin‐related devices with a completely different concept. Herein, the atomic‐scale modulation of the synthetic spiral spin order in oxide superlattices composed of ferromagnetic metal and nonmagnetic insulator layers is reported. The atomically controlled superlattice exhibits an oscillatory magnetic behavior, representing the existence of a spiral spin structure. Depth‐sensitive polarized neutron reflectometry evidences modulated spiral spin structures as a function of the nonmagnetic insulator layer thickness. Atomic‐scale customization of the spin state can move the field one step further to actual spintronic applications.

Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC05-00OR22725
OSTI ID:
1907222
Alternate ID(s):
OSTI ID: 1995880
Journal Information:
Small Methods, Vol. 0, Issue 0; ISSN 2366-9608
Publisher:
WileyCopyright Statement
Country of Publication:
United States
Language:
English

References (28)

Spin-orientation dependence in neutron reflection from a single magnetic film journal April 1995
Switchable giant nonreciprocal frequency shift of propagating spin waves in synthetic antiferromagnets journal April 2020
Terahertz spin-transfer torque oscillator based on a synthetic antiferromagnet journal March 2020
Post-synthesis control of Berry phase driven magnetotransport in SrRuO3 films journal February 2021
Giant room-temperature magnetoresistance in single-crystal Fe/MgO/Fe magnetic tunnel junctions journal October 2004
Unconventional interlayer exchange coupling via chiral phonons in synthetic magnetic oxide heterostructures journal January 2022
Spin polarized neutron reflectivity of magnetic films and superlattices journal April 1994
Spin–phonon coupling in epitaxial SrRuO3 heterostructures journal January 2020
GenX : an extensible X-ray reflectivity refinement program utilizing differential evolution journal November 2007
Giant magnetoresistance in spin-valve multilayers journal September 1994
Polarized Neutron Reflectometry for the Analysis of Nanomagnetic Systems journal July 2008
Polarized neutron reflectivity studies of magnetic semiconductor superlattices journal July 2003
Transverse and Lateral Structure of the Spin-Flop Phase in F e / C r Antiferromagnetic Superlattices journal September 2002
Highlights from the magnetism reflectometer at the SNS journal September 2009
Magnetic structure in Fe/Sm-Co exchange spring bilayers with intermixed interfaces journal May 2011
Long-range p–d exchange interaction in a ferromagnet–semiconductor hybrid structure journal October 2015
Spin Hall effects journal October 2015
Skyrmions in magnetic multilayers journal August 2017
One Million Percent Tunnel Magnetoresistance in a Magnetic van der Waals Heterostructure journal July 2018
Room-Temperature Spin Hall Effect in Graphene/MoS 2 van der Waals Heterostructures journal January 2019
Atomistic Engineering of Phonons in Functional Oxide Heterostructures journal January 2022
Synthetic antiferromagnetic spintronics journal March 2018
Symmetry-Driven Spin-Wave Gap Modulation in Nanolayered SrRuO3/SrTiO3 Heterostructures: Implications for Spintronic Applications journal February 2021
Tailoring topological Hall effect in SrRuO3/SrTiO3 superlattices journal September 2021
Phase Instability amid Dimensional Crossover in Artificial Oxide Crystal journal January 2020
Propagation Control of Octahedral Tilt in SrRuO 3 via Artificial Heterostructuring journal June 2020
Exploiting Symmetry Mismatch to Control Magnetism in a Ferroelastic Heterostructure journal May 2019
Systematic variation of the strength and oscillation period of indirect magnetic exchange coupling through the 3 d , 4 d , and 5 d transition metals journal December 1991

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