Multiple magnetic orders in LaFeAs1-xPxO uncover universality of iron-pnictide superconductors

Stadel, Ryan; Khalyavin, Dmitry D.; Manuel, Pascal; Yokoyama, Koji; Lapidus, Saul; Christensen, Morten H.; Fernandes, Rafael M.; Phelan, Daniel; Chung, Duck Young; Osborn, Raymond; Rosenkranz, Stephan; Chmaissem, Omar

doi:10.1038/s42005-022-00911-5

Title: Multiple magnetic orders in LaFeAs_1-xP_xO uncover universality of iron-pnictide superconductors

Journal Article · Tue Jun 14 00:00:00 EDT 2022 · Communications Physics

DOI:https://doi.org/10.1038/s42005-022-00911-5· OSTI ID:1906390

^[1]; Khalyavin, Dmitry D. ^[2];

^[3];

^[3]; Lapidus, Saul ^[4]; Christensen, Morten H. ^[5];

^[5]; Phelan, Daniel ^[6];

^[6];

^[7]

University of Maryland, College Park, MD (United States); Argonne National Laboratory (ANL), Lemont, IL (United States); Northern Illinois University, DeKalb, IL (United States)
Science and Technology Facilities Council (STFC), Oxford (United Kingdom). Rutherford Appleton Laboratory, ISIS Neutron Source
Science and Technology Facilities Council (STFC), Oxford (United Kingdom). Rutherford Appleton Laboratory, ISIS Neutron Sourc
Argonne National Laboratory (ANL), Lemont, IL (United States). Advanced Photon Source (APS)
University of Minnesota, Minneapolis, MN (United States)
Argonne National Laboratory (ANL), Lemont, IL (United States)
Argonne National Laboratory (ANL), Lemont, IL (United States); Northern Illinois University, DeKalb, IL (United States)

The iron-pnictide superconductors have generated tremendous excitement as the competition between magnetism and superconductivity has allowed unique in-roads towards elucidating a microscopic theory of unconventional high-temperature superconductivity. In addition to the stripe spin density wave ($$C^a_{2M}$$) phase observed in the parent compounds of all iron-pnictide superconductors, two novel magnetic orders have recently been discovered in different parent structures: an out-of-plane collinear double-Q ($$C^c_{4M}$$) structure in the hole-doped (Ca, Sr, Ba)_1-x(Na)_xFe₂As₂ and Ba_1-xK_xFe₂As₂ families, and a spin vortex crystal “hedgehog” ($$C^{ab}_{4M}$$) structure in the CaKFe₄As₄ family. Using neutron diffraction, we demonstrate that LaFeAs_1-xP_xO contains all three magnetic orders within a single-phase diagram as a function of substitution, all of which compete strongly with superconductivity. Our experimental observations combined with theoretical modeling demonstrate how the reduction in electronic correlations by chemical substitution results in larger Fermi surfaces and the sequential stabilization of multiple magnetic anisotropies. Our work presents a unified narrative for the competing magnetic and superconducting phases observed in various iron-pnictide systems with different crystal structures and chemistry.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States); Univ. of Minnesota, Minneapolis, MN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357; SC0020045

OSTI ID:: 1906390

Alternate ID(s):: OSTI ID: 1961324

Journal Information:: Communications Physics, Vol. 5, Issue 1; ISSN 2399-3650

Publisher:: Springer NatureCopyright Statement

Country of Publication:: United States

Language:: English

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Title: Multiple magnetic orders in LaFeAs_1-xP_xO uncover universality of iron-pnictide superconductors