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Title: Multistep Coulomb excitation of Ni 64 : Shape coexistence and nature of low-spin excitations

Journal Article · · Physical Review. C
 [1]; ORCiD logo [1]; ORCiD logo [1];  [2]; ORCiD logo [3];  [4];  [5]; ORCiD logo [6];  [5];  [7];  [6]; ORCiD logo [6];  [6];  [6];  [6];  [8]; ORCiD logo [8];  [9]; ORCiD logo [9]; ORCiD logo [10] more »; ORCiD logo [11] « less
  1. Univ. of North Carolina, Chapel Hill, NC (United States); Duke Univ., Durham, NC (United States)
  2. Brookhaven National Lab. (BNL), Upton, NY (United States)
  3. Univ. of Tsukuba, Ibaraki (Japan); Univ. of Tokyo (Japan)
  4. Univ. of Tokyo (Japan); RIKEN Nishina Center, Saitama (Japan); KU Leuven (Belgium)
  5. Michigan State Univ., East Lansing, MI (United States)
  6. Argonne National Lab. (ANL), Argonne, IL (United States)
  7. Michigan State Univ., East Lansing, MI (United States); TRIUMF, Vancouver, BC (Canada)
  8. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  9. Univ. of Massachusetts, Lowell, MA (United States)
  10. Univ. of Maryland, College Park, MD (United States); Georgia Tech Research Inst., Atlanta, GA (United States)
  11. Univ. of Maryland, College Park, MD (United States)

The structure of 64Ni, the heaviest stable Ni isotope, has been investigated via high-statistics, multistep safe Coulomb excitation to search for shape coexistence, a phenomenon recently observed in neutron-rich 66Ni and 70Ni as well as in doubly magic, N = 40, 68Ni. The study was motivated by recent, state-of-the-art Monte Carlo shell-model calculations (MCSM), where a Hamiltonian with effective interactions incorporating the monopole tensor force predicts the existence of shape coexistence, also in the lower-mass 62,64Ni isotopes. A set of transition and static E2 matrix elements for both yrast and near-yrast structures was extracted from the differential Coulomb excitation cross sections. From comparisons between the new results and MCSM as well as other shell-model calculations, a clearer picture of the structure of 64Ni emerges. Specifically, the low-spin states are shown to be dominated by proton and neutron excitations mainly within the fp shell, with minimal contribution from the g9/2 shape-driving neutron orbital. The agreement between experimental data and MCSM results indicates a small oblate deformation for the $$0$$$^{+}_{2}$$ level and a spherical shape for the $$0$$$^{+}_{3}$$ state. In addition, the small upper limit determined for the B(E2) probability of a transition associated with the decay of the recently observed 3463-keV, $$0$$$^{+}_{4}$$ state agrees with its proposed assignment to a prolate shape, herewith providing first evidence for triple shape coexistence in a stable Ni isotope.

Research Organization:
Michigan State Univ., East Lansing, MI (United States); Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States); University of North Carolina, Chapel Hill, NC (United States); Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Nuclear Physics (NP); National Science Foundation (NSF); USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division; Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan
Grant/Contract Number:
SC0020451; PHY-1565546; FG02-97ER41041; FG02-94ER4084; AC02-05CH11231; AC02-06CH11357; FG02-97ER41033; FG02-08ER41556; FG02-94ER40848; AC52-07NA27344
OSTI ID:
1892378
Alternate ID(s):
OSTI ID: 1893589; OSTI ID: 1895050; OSTI ID: 1908106
Report Number(s):
LLNL-JRNL-835854; TRN: US2310181
Journal Information:
Physical Review. C, Vol. 106, Issue 4; ISSN 2469-9985
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (48)

Search for shape-coexisting 0 + states in Ni 66 from lifetime measurements journal June 2017
Erratum: Analogous intruder behavior near Ni, Sn, and Pb isotopes [Phys. Rev. C 92 , 024319 (2015)] journal December 2016
Role of the ν g 9 / 2 orbital in the development of collectivity in the A 60 region: The case of Co 61 journal April 2015
Nuclear Data Sheets for A=64 journal December 2021
Analogous intruder behavior near Ni, Sn, and Pb isotopes journal August 2015
Spectroscopic study of the 64 , 66 , 68 Ni isotopes populated in 64 Ni +  238 U collisions journal December 2012
Level structure of the neutron-rich Cr 56 , 58 , 60 isotopes: Single-particle and collective aspects journal December 2006
Extension of the N = 40 Island of Inversion towards N = 50 : Spectroscopy of Cr 66 , Fe 70 , 72 journal November 2015
Single-particle and collective excitations in 63 Ni journal November 2013
Yrast structure of Fe 64 journal December 2006
In-beam γ -ray spectroscopy of Cr 62 , 64 journal January 2021
Shape Coexistence at Zero Spin in Ni 64 Driven by the Monopole Tensor Interaction journal September 2020
Single-particle and collective excitations in Ni 62 journal September 2016
The role of shell evolution in shape coexistence journal January 2016
Proton spectroscopy of Ni 48 , Fe 46 , and Cr 44 journal July 2014
In-beam γ-ray spectroscopy and inclusive two-proton knockout cross section measurements at N 40 journal May 2008
Monte Carlo shell model for atomic nuclei journal January 2001
Low-lying excitations in Ni 72 journal March 2016
Evolution of Nuclear Shells due to the Tensor Force journal November 2005
Variational procedure for nuclear shell-model calculations and energy-variance extrapolation journal May 2012
Yrast structures in the neutron-rich isotopes Fe 59 , 60 and the role of the g 9 / 2 orbital journal November 2007
High-precision B ( E 2 ) measurements of semi-magic Ni 58 , 60 , 62 , 64 by Coulomb excitation journal September 2014
Shape coexistence along N = 40 journal December 2011
In-beam γ -ray spectroscopy of Fe68 from charge exchange on Co68 projectiles journal August 2021
Structure of Fe 60 , 62 and the onset of ν g 9 / 2 occupancy journal October 2010
Shape coexistence in Ni 68 journal February 2014
Single-particle and dipole excitations in Co62 journal April 2022
Novel shape evolution in exotic Ni isotopes and configuration-dependent shell structure journal March 2014
Shape isomerism at N = 40 : Discovery of a proton intruder state in Co 67 journal October 2008
CHICO2, a two-dimensional pixelated parallel-plate avalanche counter
  • Wu, C. Y.; Cline, D.; Hayes, A.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 814 https://doi.org/10.1016/j.nima.2016.01.034
journal April 2016
Magic features of 68Ni journal June 1982
Changes in <mml:math altimg="si1.gif" overflow="scroll" xmlns:xocs="http://www.elsevier.com/xml/xocs/dtd" xmlns:xs="http://www.w3.org/2001/XMLSchema" xmlns:xsi="http://www.w3.org/2001/XMLSchema-instance" xmlns="http://www.elsevier.com/xml/ja/dtd" xmlns:ja="http://www.elsevier.com/xml/ja/dtd" xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:tb="http://www.elsevier.com/xml/common/table/dtd" xmlns:sb="http://www.elsevier.com/xml/common/struct-bib/dtd" xmlns:ce="http://www.elsevier.com/xml/common/dtd" xmlns:xlink="http://www.w3.org/1999/xlink" xmlns:cals="http://www.elsevier.com/xml/common/cals/dtd"><mml:mi>ν</mml:mi><mml:msub><mml:mi mathvariant="normal">g</mml:mi><mml:mrow><mml:mn>9</mml:mn><mml:mo stretchy="false">/</mml:mo><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:math> shape polarisation across the odd neutron-rich Cr isotopes journal August 2005
New T = 1 effective interactions for the f 5 2 p 3 2 p 1 2 g 9 2 model space: Implications for valence-mirror symmetry and seniority isomers journal October 2004
Nature of yrast excitations near N = 40 : Level structure of 67 Ni journal March 2012
Evidence for a new nuclear ‘magic number’ from the level structure of 54Ca journal October 2013
Collectivity at N = 40 in neutron-rich Cr 64 journal May 2010
Shell-model description of neutron-rich pf-shell nuclei with a new effective interaction GXPF 1 journal April 2005
The performance of the Gamma-Ray Energy Tracking In-beam Nuclear Array GRETINA
  • Paschalis, S.; Lee, I. Y.; Macchiavelli, A. O.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 709 https://doi.org/10.1016/j.nima.2013.01.009
journal May 2013
β -decay measurements for N > 40 Mn nuclei and inference of collectivity for neutron-rich Fe isotopes journal May 2011
Measurements of g factors and lifetimes of low lying states in 58 64 Ni and their shell model implications journal May 2001
78Ni revealed as a doubly magic stronghold against nuclear deformation journal May 2019
Multifaceted Quadruplet of Low-Lying Spin-Zero States in Ni 66 : Emergence of Shape Isomerism in Light Nuclei journal April 2017
Structure of 52,54Ti and shell closures in neutron-rich nuclei above 48Ca journal October 2002
New evidence for a subshell gap at N=32 journal June 2001
N = 40 Neutron Subshell Closure in the Ni 68 Nucleus journal February 1995
Decay properties of 68,69,70 Mn: Probing collectivity up to N = 44 in Fe isotopic chain journal December 2015
Shape coexistence in neutron-rich nuclei near N = 40 journal April 2013
Shape coexistence from lifetime and branching-ratio measurements in 68,70 Ni journal December 2016