High performance high-power textured Mn/Cu-doped PIN-PMN-PT ceramics

Leng, Haoyang; Yan, Yongke; Wang, Bo; Yang, Tiannan; Liu, Hairui; Li, Xiaotian; Sriramdas, Rammohan; Wang, Ke; Fanton, Mark; Meyer, Richard J.; Chen, Long-Qing; Priya, Shashank

doi:10.1016/j.actamat.2022.118015

Title: High performance high-power textured Mn/Cu-doped PIN-PMN-PT ceramics

Journal Article · Sun May 08 00:00:00 EDT 2022 · Acta Materialia

DOI:https://doi.org/10.1016/j.actamat.2022.118015· OSTI ID:1880781

Leng, Haoyang ^[1]; Yan, Yongke ^[1]; Wang, Bo ^[1];

^[1]; Liu, Hairui ^[1]; Li, Xiaotian ^[1]; Sriramdas, Rammohan ^[1]; Wang, Ke ^[1]; Fanton, Mark ^[2]; Meyer, Richard J. ^[2]; Chen, Long-Qing ^[1]; Priya, Shashank ^[1]

Pennsylvania State Univ., University Park, PA (United States)
Pennsylvania State Univ., State College, PA (United States)

Piezoelectric ceramics with combinatory soft and hard characteristics are highly desired for high-power applications. However, it remains grand challenge to achieve simultaneous presence of hard (e.g. high coercive field, E_c; high mechanical quality factor, Q_m) and soft (e.g. high piezoelectric constant, d; high electromechanical coupling factor, k) piezoelectric properties in piezoelectric ceramics since the mechanism controlling the hard behavior (pinned domain walls) will significantly reduce the soft behavior. Here, we address this grand challenge and demonstrate <001> textured MnO₂ and CuO co-doped Pb(In_1/2Nb_1/2)O_3- Pb(Mg_1/3Nb_2/3)O_3-PbTiO₃ (PIN-PMN-PT) ceramics exhibiting ultrahigh combined soft and hard piezoelectric properties (d₃₃ = 713 pC N^–1, k₃₁ = 0.52, Q_m≈950, E_c = 9.6 kV cm^–1, tan δ = 0.45%). The outstanding electromechanical properties are explained by considering composition/phase selection, crystallographic anisotropy and defect engineering. Phase-field model in conjunction with high resolution electron microscopy and diffraction techniques is utilized to delineate the contributions arising from intrinsic piezoelectric response, domain dynamics, and local structural heterogeneity. Furthermore, these results will have significant impact in the development of high-power transducers and actuators.

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Research Organization:: Pennsylvania State Univ., University Park, PA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF); US Army Research Office (ARO)

Grant/Contract Number:: SC0020145

OSTI ID:: 1880781

Alternate ID(s):: OSTI ID: 1868748

Journal Information:: Acta Materialia, Vol. 234; ISSN 1359-6454

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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