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Title: Minimizing thickness variation in monolithic U-10Mo fuel foil and Zr interlayer during hot rolling: A microstructure-based finite element method analysis

Journal Article · · Materials Today Communications

Low-enriched uranium alloyed with 10 wt. % molybdenum (U-10Mo) has been identified as a promising alternative to highly enriched uranium fuel for the United States’ high performance research reactors. The monolithic U-10Mo fuel plate consists of a metallic U-10Mo fuel foil with a 25 µm Zr interlayer and a relatively thick cladding of aluminum alloy 6061. The Zr interlayer is typically applied during the hot co-rolling process, and this process dictates the uniformity of the Zr interlayer. Thickness variation observed in the U-10Mo and Zr interlayer has been attributed to several sources: the initial grain size of the U-10Mo castings, can materials, rolling temperature, inhomogeneous molybdenum content, and porosity in the cast U-10Mo. This thickness variation limits the ability to meet the dimensional specification; thus, a better understanding of the factors causing the nonuniform thickness is needed. In this work, we used a novel, microstructure-based finite element method to model the hot rolling process to address these concerns. Grain microstructures in U-10Mo were tessellated and explicitly considered in the finite element model. Each grain was assigned a random material property to mimic the grain strength variations induced by different grain orientations. Simulations were performed using six steel can thicknesses, four grain sizes, and with or without a Zr interlayer to investigate the influences of those variables on the thickness nonuniformity. The simulation results showed that a thinner steel can and finer U-10Mo grain size reduce thickness variations in both the U-10Mo fuel foil and Zr interlayer. The direct findings from the simulations and analysis can be used to optimize the hot rolling schedule, reduce fabrication defects, and meet the dimensional specifications. The proposed microstructure-based finite element model can be also coupled with experimental microstructure characterization data, images, and models to simulate multi-pass hot rolling.

Research Organization:
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
AC05-79RL01830; AC05-76RL01830
OSTI ID:
1874813
Alternate ID(s):
OSTI ID: 1883368
Report Number(s):
PNNL-SA-168343
Journal Information:
Materials Today Communications, Vol. 32; ISSN 2352-4928
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English

References (36)

Growth kinetics and microstructural evolution during hot isostatic pressing of U-10wt.% Mo monolithic fuel plate in AA6061 cladding with Zr diffusion barrier journal April 2014
Microstructural based models for bcc and fcc metals with temperature and strain rate dependency journal February 2005
High-density, low-enriched uranium fuel for nuclear research reactors journal September 2003
Fracture criterion for predicting edge-cracking in Hot rolling of twin-roll casted AZ31 Mg alloy journal May 2020
Microstructural development from interdiffusion and reaction between U Mo and AA6061 alloys annealed at 600° and 550 °C journal August 2016
Thermal compatibility studies of unirradiated UMo alloys dispersed in aluminum journal November 1997
Finite-element model to predict roll-separation force and defects during rolling of U-10Mo alloys journal October 2017
Three-dimensional microstructural evolution in ideal grain growth—general statistics journal April 2000
Modeling and simulation of mass flow during hot rolling low carbon steel I-beam journal April 2021
Kinetics of cellular transformation and competing precipitation mechanisms during sub-eutectoid annealing of U10Mo alloys journal November 2017
Effects of heat treatment on U–Mo fuel foils with a zirconium diffusion barrier journal May 2015
Interdiffusion and reaction between U and Zr journal April 2018
Mechanical properties examined by nanoindentation for selected phases relevant to the development of monolithic uranium-molybdenum metallic fuels journal April 2017
Multi-pass hot-rolling simulation using a meshless method journal January 2018
Phase Transformations and Microstructural Development in the U-10 Wt Pct Mo Alloy with Varying Zr Contents After Heat Treatments Relevant to the Monolithic Fuel Plate Fabrication Process journal October 2018
Interdiffusion Between Zr Diffusion Barrier and U-Mo Alloy journal September 2012
Assessment of residual stresses on U10Mo alloy based monolithic mini-plates during Hot Isostatic Pressing journal December 2011
Interdiffusion and reactions between U–Mo and Zr at 650 °C as a function of time journal January 2015
A crystal plasticity model for body-centered cubic molybdenum: Experiments and simulations journal December 2018
Low-temperature irradiation behavior of uranium–molybdenum alloy dispersion fuel journal August 2002
Simulations of post-recrystallization grain growth in monolithic U–10Mo fuel processing journal December 2019
Microstructural analysis of as-processed U–10wt.%Mo monolithic fuel plate in AA6061 matrix with Zr diffusion barrier journal July 2010
Finite element modelling of surface defect evolution during hot rolling of Silicon steel journal June 2019
Microstructure-Based Multiscale Analysis of Hot Rolling of Duplex Stainless Steel Using Various Simulation Software journal March 2017
Development of very-high-density low-enriched-uranium fuels journal December 1997
Thermomechanical process optimization of U-10 wt% Mo – Part 1: high-temperature compressive properties and microstructure journal October 2015
Grain boundary engineering to control the discontinuous precipitation in multicomponent U10Mo alloy journal June 2018
The effect of thermomechanical processing on second phase particle redistribution in U-10 wt%Mo journal March 2018
Thermomechanical process optimization of U-10wt% Mo – Part 2: The effect of homogenization on the mechanical properties and microstructure journal October 2015
BCC single crystal plasticity modeling and its experimental identification journal October 2008
Large-scale 3D random polycrystals for the finite element method: Generation, meshing and remeshing journal April 2011
Microstructural anomalies in hot-isostatic pressed U–10 wt.% Mo fuel plates with Zr diffusion barrier journal May 2015
Microstructure-based multiscale modeling of large strain plastic deformation by coupling a full-field crystal plasticity-spectral solver with an implicit finite element solver journal February 2020
Phase transformation kinetics in rolled U-10 wt. % Mo foil: Effect of post-rolling heat treatment and prior γ-UMo grain size journal December 2017
Mechanical Properties of DU-xMo Alloys with x = 7 to 12 Weight Percent journal March 2009
Modeling the homogenization kinetics of as-cast U-10wt% Mo alloys journal April 2016