Impact of dry intrusion events on the composition and mixing state of particles during the winter Aerosol and Cloud Experiment in the Eastern North Atlantic (ACE-ENA)

Tomlin, Jay M.; Jankowski, Kevin A.; Veghte, Daniel P.; China, Swarup; Wang, Peiwen; Fraund, Matthew; Weis, Johannes; Zheng, Guangjie; Wang, Yang; Rivera-Adorno, Felipe; Raveh-Rubin, Shira; Knopf, Daniel A.; Wang, Jian; Gilles, Mary K.; Moffet, Ryan C.; Laskin, Alexander

doi:10.5194/acp-21-18123-2021

Title: Impact of dry intrusion events on the composition and mixing state of particles during the winter Aerosol and Cloud Experiment in the Eastern North Atlantic (ACE-ENA)

Journal Article · Tue Dec 14 00:00:00 EST 2021 · Atmospheric Chemistry and Physics (Online)

DOI:https://doi.org/10.5194/acp-21-18123-2021· OSTI ID:1835634

; Jankowski, Kevin A.; Veghte, Daniel P.;

; Wang, Peiwen;

; Weis, Johannes;

;

; Rivera-Adorno, Felipe;

;

; Gilles, Mary K.;

;

Long-range transport of continental emissions has a far-reaching influence over remote regions, resulting in substantial change in the size, morphology, and composition of the local aerosol population and cloud condensation nuclei (CCN) budget. Here, we investigate the physicochemical properties of atmospheric particles collected on board a research aircraft flown over the Azores during the winter 2018 Aerosol and Cloud Experiment in the Eastern North Atlantic (ACE-ENA) campaign. Particles were collected within the marine boundary layer (MBL) and free troposphere (FT) after long-range atmospheric transport episodes facilitated by dry intrusion (DI) events. Chemical and physical properties of individual particles were investigated using complementary capabilities of computer-controlled scanning electron microscopy and X-ray spectromicroscopy to probe particle external and internal mixing state characteristics. Furthermore, real-time measurements of aerosol size distribution, cloud condensation nuclei (CCN) concentration, and back-trajectory calculations were utilized to help bring into context the findings from offline spectromicroscopy analysis. While carbonaceous particles were found to be the dominant particle type in the region, changes in the percent contribution of organics across the particle population (i.e., external mixing) shifted from 68 % to 43 % in the MBL and from 92 % to 46 % in FT samples during DI events. This change in carbonaceous contribution is counterbalanced by the increase in inorganics from 32 % to 57 % in the MBL and 8 % to 55 % in FT. The quantification of the organic volume fraction (OVF) of individual particles derived from X-ray spectromicroscopy, which relates to the multi-component internal composition of individual particles, showed a factor of 2.06 ± 0.16 and 1.11 ± 0.04 increase in the MBL and FT, respectively, among DI samples. We show that supplying particle OVF into the κ-Köhler equation can be used as a good approximation of field-measured in situ CCN concentrations. We also report changes in the κ values in the MBL from _{κ_{MBL, non-DI}}=0.48 to _{κ_{MBL, DI}}=0.41, while changes in the FT result in κFT, non-DI=0.36 to κFT, DI=0.33, which is consistent with enhancements in OVF followed by the DI episodes. Our observations suggest that entrainment of particles from long-range continental sources alters the mixing state population and CCN properties of aerosol in the region. Here, the work presented here provides field observation data that can inform atmospheric models that simulate sources and particle composition in the eastern North Atlantic.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Atmospheric Radiation Measurement (ARM) Data Center; Washington Univ., St. Louis, MO (United States); Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Purdue Univ., West Lafayette, IN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Biological and Environmental Research (BER); Israel Science Foundation (ISF)

Grant/Contract Number:: SC0018948; SC0020259; SC0016370; SC0021034; 1347/18; AC05-76RL01830

OSTI ID:: 1835634

Alternate ID(s):: OSTI ID: 1835566; OSTI ID: 1837829; OSTI ID: 1841576; OSTI ID: 1908097

Report Number(s):: PNNL-SA-164890

Journal Information:: Atmospheric Chemistry and Physics (Online), Journal Name: Atmospheric Chemistry and Physics (Online) Vol. 21 Journal Issue: 24; ISSN 1680-7324

Publisher:: Copernicus GmbHCopyright Statement

Country of Publication:: Germany

Language:: English

References (145)

Mixing states of Amazon basin aerosol particles transported over long distances using transmission electron microscopy Adachi, Kouji; Oshima, Naga; Gong, Zhaoheng Atmospheric Chemistry and Physics, Vol. 20, Issue 20 https://doi.org/10.5194/acp-20-11923-2020	journal	January 2020
Biomass burning smoke aerosol properties measured during Fire Laboratory at Missoula Experiments (FLAME) Levin, E. J. T.; McMeeking, G. R.; Carrico, C. M. Journal of Geophysical Research, Vol. 115, Issue D18 https://doi.org/10.1029/2009JD013601	journal	January 2010
Review: Cloud invigoration by aerosols—Coupling between microphysics and dynamics Altaratz, O.; Koren, I.; Remer, L. A. Atmospheric Research, Vol. 140-141 https://doi.org/10.1016/j.atmosres.2014.01.009	journal	April 2014
Chemical composition of aerosol particles from direct emissions of vegetation fires in the Amazon Basin: water-soluble species and trace elements Yamasoe, Márcia A.; Artaxo, Paulo; Miguel, Antonio H. Atmospheric Environment, Vol. 34, Issue 10 https://doi.org/10.1016/S1352-2310(99)00329-5	journal	January 2000
Biogenically driven organic contribution to marine aerosol O'Dowd, Colin D.; Facchini, Maria Cristina; Cavalli, Fabrizia Nature, Vol. 431, Issue 7009 https://doi.org/10.1038/nature02959	journal	October 2004
Aerosol Pollution Impact on Precipitation: A Scientific Review Levin, Zev; Cotton, William R. https://doi.org/10.1007/978-1-4020-8690-8	book	January 2009
Strong radiative heating due to the mixing state of black carbon in atmospheric aerosols Jacobson, Mark Z. Nature, Vol. 409, Issue 6821 https://doi.org/10.1038/35055518	journal	February 2001
Collocated observations of cloud condensation nuclei, particle size distributions, and chemical composition Schmale, Julia; Henning, Silvia; Henzing, Bas Scientific Data, Vol. 4, Issue 1 https://doi.org/10.1038/sdata.2017.3	journal	March 2017
Single-Particle SEM-EDX Analysis of Iron-Containing Coarse Particulate Matter in an Urban Environment: Sources and Distribution of Iron within Cleveland, Ohio Ault, Andrew P.; Peters, Thomas M.; Sawvel, Eric J. Environmental Science & Technology, Vol. 46, Issue 8 https://doi.org/10.1021/es204006k	journal	April 2012
An interfacial mechanism for cloud droplet formation on organic aerosols Ruehl, C. R.; Davies, J. F.; Wilson, K. R. Science, Vol. 351, Issue 6280 https://doi.org/10.1126/science.aad4889	journal	March 2016
Automated Chemical Analysis of Internally Mixed Aerosol Particles Using X-ray Spectromicroscopy at the Carbon K-Edge ^† Moffet, Ryan C.; Henn, Tobias; Laskin, Alexander Analytical Chemistry, Vol. 82, Issue 19 https://doi.org/10.1021/ac1012909	journal	October 2010
Emissions Inventory of PM _2.5 Trace Elements across the United States Reff, Adam; Bhave, Prakash V.; Simon, Heather Environmental Science & Technology, Vol. 43, Issue 15 https://doi.org/10.1021/es802930x	journal	August 2009
Aircraft measurements of aerosol and trace gas chemistry in the eastern North Atlantic Zawadowicz, Maria A.; Suski, Kaitlyn; Liu, Jiumeng Atmospheric Chemistry and Physics, Vol. 21, Issue 10 https://doi.org/10.5194/acp-21-7983-2021	journal	May 2021
Black Carbon Aerosol Concentration in Five Cities and Its Scaling with City Population Paredes-Miranda, G.; Arnott, W. P.; Moosmüller, H. Bulletin of the American Meteorological Society, Vol. 94, Issue 1 https://doi.org/10.1175/BAMS-D-11-00225.1	journal	January 2013
Effects of near-source coagulation of biomass burning aerosols on global predictions of aerosol size distributions and implications for aerosol radiative effects Ramnarine, Emily; Kodros, John K.; Hodshire, Anna L. Atmospheric Chemistry and Physics, Vol. 19, Issue 9 https://doi.org/10.5194/acp-19-6561-2019	journal	January 2019
Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) Wang, Jian; Wood, Rob; Jensen, Michael P. Bulletin of the American Meteorological Society, Vol. 103, Issue 2 https://doi.org/10.1175/BAMS-D-19-0220.1	journal	February 2022
Vertical profiles of trace gas and aerosol properties over the eastern North Atlantic: variations with season and synoptic condition Wang, Yang; Zheng, Guangjie; Jensen, Michael P. Atmospheric Chemistry and Physics, Vol. 21, Issue 14 https://doi.org/10.5194/acp-21-11079-2021	journal	January 2021
A review of particle formation events and growth in the atmosphere in the various environments and discussion of mechanistic implications Holmes, N. S. Atmospheric Environment, Vol. 41, Issue 10 https://doi.org/10.1016/j.atmosenv.2006.10.058	journal	March 2007
Wet deposition of black carbon: A synthesis Barrett, T. E.; Ponette-González, A. G.; Rindy, J. E. Atmospheric Environment, Vol. 213 https://doi.org/10.1016/j.atmosenv.2019.06.033	journal	September 2019
Long-range transported North American wildfire aerosols observed in marine boundary layer of eastern North Atlantic Zheng, Guangjie; Sedlacek, Arthur J.; Aiken, Allison C. Environment International, Vol. 139 https://doi.org/10.1016/j.envint.2020.105680	journal	June 2020
Impacts of long-range transport of aerosols on marine-boundary-layer clouds in the eastern North Atlantic Wang, Yuan; Zheng, Xiaojian; Dong, Xiquan Atmospheric Chemistry and Physics, Vol. 20, Issue 23 https://doi.org/10.5194/acp-20-14741-2020	journal	January 2020
Entrainment of free tropospheric aerosols as a regulating mechanism for cloud condensation nuclei in the remote marine boundary layer Raes, Frank Journal of Geophysical Research, Vol. 100, Issue D2 https://doi.org/10.1029/94JD02832	journal	January 1995
A lagrangian-based analysis of extratropical cyclones. II: A detailed case-study Wernli, Heini Quarterly Journal of the Royal Meteorological Society, Vol. 123, Issue 542 https://doi.org/10.1002/qj.49712354211	journal	July 1997
Development and implementation of a new biomass burning emissions injection height scheme (BBEIH v1.0) for the GEOS-Chem model (v9-01-01) Zhu, Liye; Val Martin, Maria; Gatti, Luciana V. Geoscientific Model Development, Vol. 11, Issue 10 https://doi.org/10.5194/gmd-11-4103-2018	journal	January 2018
The Ejection of Drops from the Sea and Their Enrichment with Bacteria and Other Materials: A Review Blanchard, Duncan C. Estuaries, Vol. 12, Issue 3 https://doi.org/10.2307/1351816	journal	September 1989
The LAGRANTO Lagrangian analysis tool – version 2.0 Sprenger, M.; Wernli, H. Geoscientific Model Development, Vol. 8, Issue 8 https://doi.org/10.5194/gmd-8-2569-2015	journal	January 2015
Airborne minerals and related aerosol particles: Effects on climate and the environment Buseck, P. R.; Posfai, M. Proceedings of the National Academy of Sciences, Vol. 96, Issue 7 https://doi.org/10.1073/pnas.96.7.3372	journal	March 1999
Evolution of Asian aerosols during transpacific transport in INTEX-B Dunlea, E. J.; DeCarlo, P. F.; Aiken, A. C. Atmospheric Chemistry and Physics, Vol. 9, Issue 19 https://doi.org/10.5194/acp-9-7257-2009	journal	January 2009
Are climate model simulations of clouds improving? An evaluation using the ISCCP simulator: EVALUATING CLOUDS IN CLIMATE MODELS Klein, Stephen A.; Zhang, Yuying; Zelinka, Mark D. Journal of Geophysical Research: Atmospheres, Vol. 118, Issue 3 https://doi.org/10.1002/jgrd.50141	journal	February 2013
Influence of an organic coating on the reactivity of aqueous aerosols probed by the heterogeneous hydrolysis of N ₂ O ₅ : ORGANIC COATINGS AND AEROSOL REACTIVITY Folkers, M.; Mentel, Th. F.; Wahner, A. Geophysical Research Letters, Vol. 30, Issue 12 https://doi.org/10.1029/2003GL017168	journal	June 2003
An analysis of the mechanisms of North American pollutant transport to the central North Atlantic lower free troposphere: LOWER FREE TROPOSPHERE EXPORT MECHANISMS Owen, R. C.; Cooper, O. R.; Stohl, A. Journal of Geophysical Research: Atmospheres, Vol. 111, Issue D23 https://doi.org/10.1029/2006JD007062	journal	August 2006
Major secondary aerosol formation in southern African open biomass burning plumes Vakkari, Ville; Beukes, Johan P.; Dal Maso, Miikka Nature Geoscience, Vol. 11, Issue 8 https://doi.org/10.1038/s41561-018-0170-0	journal	June 2018
Aircraft measurements of vertical profiles of aerosol mixing states Pratt, Kerri A.; Prather, Kimberly A. Journal of Geophysical Research, Vol. 115, Issue D11 https://doi.org/10.1029/2009JD013150	journal	January 2010
The deposition ice nucleation and immersion freezing potential of amorphous secondary organic aerosol: Pathways for ice and mixed-phase cloud formation: ICE NUCLEATION BY AMORPHOUS SOA Wang, Bingbing; Lambe, Andrew T.; Massoli, Paola Journal of Geophysical Research: Atmospheres, Vol. 117, Issue D16 https://doi.org/10.1029/2012JD018063	journal	August 2012
Marine boundary layer aerosol in the eastern North Atlantic: seasonal variations and key controlling processes Zheng, Guangjie; Wang, Yang; Aiken, Allison C. Atmospheric Chemistry and Physics, Vol. 18, Issue 23 https://doi.org/10.5194/acp-18-17615-2018	journal	January 2018
Effect of precipitation on the albedo susceptibility of clouds in the marine boundary layer Pincus, Robert; Baker, Marcia B. Nature, Vol. 372, Issue 6503 https://doi.org/10.1038/372250a0	journal	November 1994
Reactivity of Liquid and Semisolid Secondary Organic Carbon with Chloride and Nitrate in Atmospheric Aerosols Wang, Bingbing; O’Brien, Rachel E.; Kelly, Stephen T. The Journal of Physical Chemistry A, Vol. 119, Issue 19 https://doi.org/10.1021/jp510336q	journal	November 2014
Spectro-microscopic measurements of carbonaceous aerosol aging in Central California Moffet, R. C.; Rödel, T. C.; Kelly, S. T. Atmospheric Chemistry and Physics, Vol. 13, Issue 20 https://doi.org/10.5194/acp-13-10445-2013	journal	January 2013
Sea salt aerosols as a reactive surface for inorganic and organic acidic gases in the Arctic troposphere Chi, J. W.; Li, W. J.; Zhang, D. Z. Atmospheric Chemistry and Physics, Vol. 15, Issue 19 https://doi.org/10.5194/acp-15-11341-2015	journal	January 2015
The potential role of methanesulfonic acid (MSA) in aerosol formation and growth and the associated radiative forcings Hodshire, Anna L.; Campuzano-Jost, Pedro; Kodros, John K. Atmospheric Chemistry and Physics, Vol. 19, Issue 5 https://doi.org/10.5194/acp-19-3137-2019	journal	January 2019
Quantitative capabilities of STXM to measure spatially resolved organic volume fractions of mixed organic ∕ inorganic particles Fraund, Matthew; Park, Tim; Yao, Lin Atmospheric Measurement Techniques, Vol. 12, Issue 3 https://doi.org/10.5194/amt-12-1619-2019	journal	January 2019
The semi-direct aerosol effect: Impact of absorbing aerosols on marine stratocumulus Johnson, B. T.; Shine, K. P.; Forster, P. M. Quarterly Journal of the Royal Meteorological Society, Vol. 130, Issue 599 https://doi.org/10.1256/qj.03.61	journal	April 2004
Field-Deployable, High-Resolution, Time-of-Flight Aerosol Mass Spectrometer DeCarlo, Peter F.; Kimmel, Joel R.; Trimborn, Achim Analytical Chemistry, Vol. 78, Issue 24 https://doi.org/10.1021/ac061249n	journal	December 2006
Contributions of transported Prudhoe Bay oil field emissions to the aerosol population in Utqiaġvik, Alaska Gunsch, Matthew J.; Kirpes, Rachel M.; Kolesar, Katheryn R. Atmospheric Chemistry and Physics, Vol. 17, Issue 17 https://doi.org/10.5194/acp-17-10879-2017	journal	January 2017
Effect of Particle Morphology on Cloud Condensation Nuclei Activity Altaf, Muhammad Bilal; Dutcher, Dabrina D.; Raymond, Timothy M. ACS Earth and Space Chemistry, Vol. 2, Issue 6 https://doi.org/10.1021/acsearthspacechem.7b00146	journal	April 2018
Stratocumulus Clouds Wood, Robert Monthly Weather Review, Vol. 140, Issue 8 https://doi.org/10.1175/MWR-D-11-00121.1	journal	August 2012
New particle formation in the remote marine boundary layer Zheng, Guangjie; Wang, Yang; Wood, Robert Nature Communications, Vol. 12, Issue 1 https://doi.org/10.1038/s41467-020-20773-1	journal	January 2021
Nitrogenated and aliphatic organic vapors as possible drivers for marine secondary organic aerosol growth: MARINE SECONDARY ORGANIC AEROSOL GROWTH Dall'Osto, Manuel; Ceburnis, Darius; Monahan, Ciaran Journal of Geophysical Research: Atmospheres, Vol. 117, Issue D12 https://doi.org/10.1029/2012JD017522	journal	June 2012
Role of OH-Initiated Oxidation of Isoprene in Aging of Combustion Soot Khalizov, Alexei F.; Lin, Yun; Qiu, Chong Environmental Science & Technology, Vol. 47, Issue 5 https://doi.org/10.1021/es3045339	journal	February 2013
Solid supported multicomponent lipid membranes studied by x-ray spectromicroscopy Nováková, Eva; Mitrea, Genoveva; Peth, Christian Biointerphases, Vol. 3, Issue 2 https://doi.org/10.1116/1.2976445	journal	June 2008
The T1-T2 study: evolution of aerosol properties downwind of Mexico City Doran, J. C.; Barnard, J. C.; Arnott, W. P. Atmospheric Chemistry and Physics, Vol. 7, Issue 6 https://doi.org/10.5194/acp-7-1585-2007	journal	January 2007
Analysis of individual environmental particles using modern methods of electron microscopy and X-ray microanalysis Laskin, A.; Cowin, J. P.; Iedema, M. J. Journal of Electron Spectroscopy and Related Phenomena, Vol. 150, Issue 2-3 https://doi.org/10.1016/j.elspec.2005.06.008	journal	February 2006
The Impact of Aerosol Particle Mixing State on the Hygroscopicity of Sea Spray Aerosol Schill, Steven R.; Collins, Douglas B.; Lee, Christopher ACS Central Science, Vol. 1, Issue 3 https://doi.org/10.1021/acscentsci.5b00174	journal	June 2015
Climatology and dynamics of the link between dry intrusions and cold fronts during winter. Part I: global climatology Catto, Jennifer L.; Raveh-Rubin, Shira Climate Dynamics, Vol. 53, Issue 3-4 https://doi.org/10.1007/s00382-019-04745-w	journal	May 2019
Bringing the ocean into the laboratory to probe the chemical complexity of sea spray aerosol Prather, K. A.; Bertram, T. H.; Grassian, V. H. Proceedings of the National Academy of Sciences, Vol. 110, Issue 19 https://doi.org/10.1073/pnas.1300262110	journal	April 2013
Quantifying the Impact of Biomass Burning Emissions on Major Inorganic Aerosols and Their Precursors in the U.S.: Burning Impact on Inorganic Aerosols Souri, Amir H.; Choi, Yunsoo; Jeon, Wonbae Journal of Geophysical Research: Atmospheres, Vol. 122, Issue 21 https://doi.org/10.1002/2017JD026788	journal	November 2017
Dimethyl sulfide in the marine atmosphere Andreae, M. O.; Ferek, R. J.; Bermond, F. Journal of Geophysical Research, Vol. 90, Issue D7 https://doi.org/10.1029/JD090iD07p12891	journal	January 1985
Substantial Seasonal Contribution of Observed Biogenic Sulfate Particles to Cloud Condensation Nuclei Sanchez, Kevin J.; Chen, Chia-Li; Russell, Lynn M. Scientific Reports, Vol. 8, Issue 1 https://doi.org/10.1038/s41598-018-21590-9	journal	February 2018
A chemical kinetic model for reactive transformations of aerosol particles: REACTIVE TRANSFORMATION OF AEROSOL PARTICLES Worsnop, D. R.; Morris, J. W.; Shi, Q. Geophysical Research Letters, Vol. 29, Issue 20 https://doi.org/10.1029/2002GL015542	journal	October 2002
Investigating Primary Marine Aerosol Properties: CCN Activity of Sea Salt and Mixed Inorganic–Organic Particles King, Stephanie M.; Butcher, Andrew C.; Rosenoern, Thomas Environmental Science & Technology, Vol. 46, Issue 19 https://doi.org/10.1021/es300574u	journal	August 2012
Chemical transfer of dissolved organic matter from surface seawater to sea spray water-soluble organic aerosol in the marine atmosphere Miyazaki, Yuzo; Yamashita, Youhei; Kawana, Kaori Scientific Reports, Vol. 8, Issue 1 https://doi.org/10.1038/s41598-018-32864-7	journal	October 2018
Climatology and dynamics of the link between dry intrusions and cold fronts during winter, Part II: Front-centred perspective Raveh-Rubin, Shira; Catto, Jennifer L. Climate Dynamics, Vol. 53, Issue 3-4 https://doi.org/10.1007/s00382-019-04793-2	journal	May 2019
Aerosol time-of-flight mass spectrometry data analysis: A benchmark of clustering algorithms Rebotier, Thomas P.; Prather, Kimberly A. Analytica Chimica Acta, Vol. 585, Issue 1 https://doi.org/10.1016/j.aca.2006.12.009	journal	February 2007
Single Particle Characterization of Ultrafine and Accumulation Mode Particles from Heavy Duty Diesel Vehicles Using Aerosol Time-of-Flight Mass Spectrometry Toner, Stephen M.; Sodeman, David A.; Prather, Kimberly A. Environmental Science & Technology, Vol. 40, Issue 12 https://doi.org/10.1021/es051455x	journal	June 2006
Iron speciation and mixing in single aerosol particles from the Asian continental outflow: AEROSOL IRON SPECIATION IN ASIAN OUTFLOW Moffet, Ryan C.; Furutani, Hiroshi; Rödel, Tobias C. Journal of Geophysical Research: Atmospheres, Vol. 117, Issue D7 https://doi.org/10.1029/2011JD016746	journal	April 2012
Marine boundary layer clouds at the heart of tropical cloud feedback uncertainties in climate models Bony, Sandrine Geophysical Research Letters, Vol. 32, Issue 20 https://doi.org/10.1029/2005GL023851	journal	January 2005
Organic Aerosol Growth Mechanisms and Their Climate-Forcing Implications Maria, S. F. Science, Vol. 306, Issue 5703 https://doi.org/10.1126/science.1103491	journal	December 2004
Dry Intrusions: Lagrangian Climatology and Dynamical Impact on the Planetary Boundary Layer Raveh-Rubin, Shira Journal of Climate, Vol. 30, Issue 17 https://doi.org/10.1175/JCLI-D-16-0782.1	journal	September 2017
Stable sulphate clusters as a source of new atmospheric particles Kulmala, Markku; Pirjola, Liisa; Mäkelä, Jyrki M. Nature, Vol. 404, Issue 6773 https://doi.org/10.1038/35003550	journal	March 2000
The Tropospheric Chemistry of Sea Salt: A Molecular-Level View of the Chemistry of NaCl and NaBr Finlayson-Pitts, B. J. Chemical Reviews, Vol. 103, Issue 12 https://doi.org/10.1021/cr020653t	journal	December 2003
Motor exhaust emissions as a primary source for dicarboxylic acids in Los Angeles ambient air Kawamura, Kimitaka.; Kaplan, Isaac R. Environmental Science & Technology, Vol. 21, Issue 1 https://doi.org/10.1021/es00155a014	journal	January 1987
Chemical Imaging of Fine Mode Atmospheric Particles Collected from a Research Aircraft over Agricultural Fields Tomlin, Jay M.; Jankowski, Kevin A.; Rivera-Adorno, Felipe A. ACS Earth and Space Chemistry, Vol. 4, Issue 11 https://doi.org/10.1021/acsearthspacechem.0c00172	journal	November 2020
Interferometer-controlled scanning transmission X-ray microscopes at the Advanced Light Source Kilcoyne, A. L. D.; Tyliszczak, T.; Steele, W. F. Journal of Synchrotron Radiation, Vol. 10, Issue 2 https://doi.org/10.1107/S0909049502017739	journal	February 2003
Primary submicron marine aerosol dominated by insoluble organic colloids and aggregates Facchini, Maria Cristina; Rinaldi, Matteo; Decesari, Stefano Geophysical Research Letters, Vol. 35, Issue 17 https://doi.org/10.1029/2008GL034210	journal	January 2008
The versatility of algae and their lipid metabolism Harwood, John L.; Guschina, Irina A. Biochimie, Vol. 91, Issue 6 https://doi.org/10.1016/j.biochi.2008.11.004	journal	June 2009
Significant enhancements of nitrogen oxides, black carbon, and ozone in the North Atlantic lower free troposphere resulting from North American boreal wildfires: WILDFIRE IMPACTS ON BC, NO Val Martín, M.; Honrath, R. E.; Owen, R. C. Journal of Geophysical Research: Atmospheres, Vol. 111, Issue D23 https://doi.org/10.1029/2006JD007530	journal	December 2006
Elemental Mixing State of Aerosol Particles Collected in Central Amazonia during GoAmazon2014/15 Fraund, Matthew; Pham, Don; Bonanno, Daniel Atmosphere, Vol. 8, Issue 12 https://doi.org/10.3390/atmos8090173	journal	September 2017
Clouds, Aerosols, and Precipitation in the Marine Boundary Layer: An Arm Mobile Facility Deployment Wood, Robert; Wyant, Matthew; Bretherton, Christopher S. Bulletin of the American Meteorological Society, Vol. 96, Issue 3 https://doi.org/10.1175/BAMS-D-13-00180.1	journal	March 2015
Small Ice Particles in Tropospheric Clouds: Fact or Artifact? Airborne Icing Instrumentation Evaluation Experiment Korolev, A. V.; Emery, E. F.; Strapp, J. W. Bulletin of the American Meteorological Society, Vol. 92, Issue 8 https://doi.org/10.1175/2010BAMS3141.1	journal	August 2011
Occurrence of pristine aerosol environments on a polluted planet Hamilton, Douglas S.; Lee, Lindsay A.; Pringle, Kirsty J. Proceedings of the National Academy of Sciences, Vol. 111, Issue 52 https://doi.org/10.1073/pnas.1415440111	journal	December 2014
Chemical Imaging of Atmospheric Particles Laskin, Alexander; Moffet, Ryan C.; Gilles, Mary K. Accounts of Chemical Research, Vol. 52, Issue 12 https://doi.org/10.1021/acs.accounts.9b00396	journal	November 2019
Tropospheric chemistry of internally mixed sea salt and organic particles: Surprising reactivity of NaCl with weak organic acids: MIXED SEA SALT/ORGANICS PARTICLES Laskin, Alexander; Moffet, Ryan C.; Gilles, Mary K. Journal of Geophysical Research: Atmospheres, Vol. 117, Issue D15 https://doi.org/10.1029/2012JD017743	journal	August 2012
The impact of humidity above stratiform clouds on indirect aerosol climate forcing Ackerman, Andrew S.; Kirkpatrick, Michael P.; Stevens, David E. Nature, Vol. 432, Issue 7020 https://doi.org/10.1038/nature03174	journal	December 2004
The dry intrusion perspective of extra-tropical cyclone development Browning, K. A. Meteorological Applications, Vol. 4, Issue 4 https://doi.org/10.1017/S1350482797000613	journal	December 1997
Chemical bonding and structure of black carbon reference materials and individual carbonaceous atmospheric aerosols Hopkins, Rebecca J.; Tivanski, Alexei V.; Marten, Bryan D. Journal of Aerosol Science, Vol. 38, Issue 6 https://doi.org/10.1016/j.jaerosci.2007.03.009	journal	June 2007
Heterogeneous chemistry of individual mineral dust particles with nitric acid: A combined CCSEM/EDX, ESEM, and ICP-MS study Laskin, A. Journal of Geophysical Research, Vol. 110, Issue D10 https://doi.org/10.1029/2004JD005206	journal	January 2005
Scanning Transmission X-Ray, Laser Scanning, and Transmission Electron Microscopy Mapping of the Exopolymeric Matrix of Microbial Biofilms Lawrence, J. R.; Swerhone, G. D. W.; Leppard, G. G. Applied and Environmental Microbiology, Vol. 69, Issue 9 https://doi.org/10.1128/AEM.69.9.5543-5554.2003	journal	September 2003
Real-time Environmental Applications and Display sYstem: READY Rolph, Glenn; Stein, Ariel; Stunder, Barbara Environmental Modelling & Software, Vol. 95 https://doi.org/10.1016/j.envsoft.2017.06.025	journal	September 2017
Aircraft-based aerosol size and composition measurements during ACE-Asia using an Aerodyne aerosol mass spectrometer Bahreini, Roya Journal of Geophysical Research, Vol. 108, Issue D23 https://doi.org/10.1029/2002JD003226	journal	January 2003
Chemical composition of single aerosol particles at Idaho Hill: Negative ion measurements Murphy, D. M.; Thomson, D. S. Journal of Geophysical Research: Atmospheres, Vol. 102, Issue D5 https://doi.org/10.1029/96JD00859	journal	March 1997
Free tropospheric aerosols at the Mt. Bachelor Observatory: more oxidized and higher sulfate content compared to boundary layer aerosols Zhou, Shan; Collier, Sonya; Jaffe, Daniel A. Atmospheric Chemistry and Physics, Vol. 19, Issue 3 https://doi.org/10.5194/acp-19-1571-2019	journal	January 2019
Ice cloud formation potential by free tropospheric particles from long-range transport over the Northern Atlantic Ocean: ICE CLOUD FORMATION BY AGED PARTICLES China, Swarup; Alpert, Peter A.; Zhang, Bo Journal of Geophysical Research: Atmospheres, Vol. 122, Issue 5 https://doi.org/10.1002/2016JD025817	journal	March 2017
Aerosol Growth and the Condensation Coefficient for Water: A Review Mozurkewich, Michael Aerosol Science and Technology, Vol. 5, Issue 2 https://doi.org/10.1080/02786828608959089	journal	January 1986
A study of the ability of pure secondary organic aerosol to act as cloud condensation nuclei Cruz, Celia N.; Pandis, Spyros N. Atmospheric Environment, Vol. 31, Issue 15 https://doi.org/10.1016/S1352-2310(97)00054-X	journal	August 1997
Time-Resolved Aerosol Collector for CCSEM/EDX Single-Particle Analysis Laskin, Alexander; Iedema, Martin J.; Cowin, James P. Aerosol Science and Technology, Vol. 37, Issue 3 https://doi.org/10.1080/02786820300945	journal	March 2003
Surface tension prevails over solute effect in organic-influenced cloud droplet activation Ovadnevaite, Jurgita; Zuend, Andreas; Laaksonen, Ari Nature, Vol. 546, Issue 7660 https://doi.org/10.1038/nature22806	journal	June 2017
Characterization of Residential Woodsmoke PM2.5 in the Adirondacks of New York Allen, George; Rector, Lisa Aerosol and Air Quality Research, Vol. 20, Issue 11 https://doi.org/10.4209/aaqr.2020.01.0005	journal	January 2020
Using different assumptions of aerosol mixing state and chemical composition to predict CCN concentrations based on field measurements in urban Beijing Ren, Jingye; Zhang, Fang; Wang, Yuying Atmospheric Chemistry and Physics, Vol. 18, Issue 9 https://doi.org/10.5194/acp-18-6907-2018	journal	January 2018
Morphology and mixing state of aged soot particles at a remote marine free troposphere site: Implications for optical properties: Morphology and mixing state of aged soot China, Swarup; Scarnato, Barbara; Owen, Robert C. Geophysical Research Letters, Vol. 42, Issue 4 https://doi.org/10.1002/2014GL062404	journal	February 2015
Primary versus secondary contributions to particle number concentrations in the European boundary layer Reddington, C. L.; Carslaw, K. S.; Spracklen, D. V. Atmospheric Chemistry and Physics, Vol. 11, Issue 23 https://doi.org/10.5194/acp-11-12007-2011	journal	January 2011
The ERA-Interim reanalysis: configuration and performance of the data assimilation system Dee, D. P.; Uppala, S. M.; Simmons, A. J. Quarterly Journal of the Royal Meteorological Society, Vol. 137, Issue 656 https://doi.org/10.1002/qj.828	journal	April 2011
A conceptual framework for mixing structures in individual aerosol particles: Individual Aerosol Mixing Structure Li, Weijun; Sun, Jiaxing; Xu, Liang Journal of Geophysical Research: Atmospheres, Vol. 121, Issue 22 https://doi.org/10.1002/2016JD025252	journal	November 2016
NOAA’s HYSPLIT Atmospheric Transport and Dispersion Modeling System Stein, A. F.; Draxler, R. R.; Rolph, G. D. Bulletin of the American Meteorological Society, Vol. 96, Issue 12 https://doi.org/10.1175/BAMS-D-14-00110.1	journal	December 2015
The diverse chemical mixing state of aerosol particles in the southeastern United States Bondy, Amy L.; Bonanno, Daniel; Moffet, Ryan C. Atmospheric Chemistry and Physics, Vol. 18, Issue 16 https://doi.org/10.5194/acp-18-12595-2018	journal	January 2018
The Impact of Slantwise Descending Dry Intrusions on the Marine Boundary Layer and Air‐Sea Interface Over the ARM Eastern North Atlantic Site Ilotoviz, E.; Ghate, V. P.; Raveh‐Rubin, S. Journal of Geophysical Research: Atmospheres, Vol. 126, Issue 4 https://doi.org/10.1029/2020JD033879	journal	February 2021
New fast integrated mobility spectrometer for real-time measurement of aerosol size distribution—I: Concept and theory Kulkarni, Pramod; Wang, Jian Journal of Aerosol Science, Vol. 37, Issue 10 https://doi.org/10.1016/j.jaerosci.2006.01.005	journal	October 2006
Microbial Control of Sea Spray Aerosol Composition: A Tale of Two Blooms Wang, Xiaofei; Sultana, Camille M.; Trueblood, Jonathan ACS Central Science, Vol. 1, Issue 3 https://doi.org/10.1021/acscentsci.5b00148	journal	May 2015
Nitrogen Cycling in the Ocean: New Perspectives on Processes and Paradigms Zehr, J. P.; Ward, B. B. Applied and Environmental Microbiology, Vol. 68, Issue 3 https://doi.org/10.1128/AEM.68.3.1015-1024.2002	journal	March 2002
Characterization of particle cloud droplet activity and composition in the free troposphere and the boundary layer during INTEX-B Roberts, G. C.; Day, D. A.; Russell, L. M. Atmospheric Chemistry and Physics, Vol. 10, Issue 14 https://doi.org/10.5194/acp-10-6627-2010	journal	January 2010
Emissions from prescribed burning of agricultural fields in the Pacific Northwest Holder, A. L.; Gullett, B. K.; Urbanski, S. P. Atmospheric Environment, Vol. 166 https://doi.org/10.1016/j.atmosenv.2017.06.043	journal	October 2017
Changes to the Chemical Composition of Soot from Heterogeneous Oxidation Reactions Browne, Eleanor C.; Franklin, Jonathan P.; Canagaratna, Manjula R. The Journal of Physical Chemistry A, Vol. 119, Issue 7 https://doi.org/10.1021/jp511507d	journal	February 2015
Large contribution of organics to condensational growth and formation of cloud condensation nuclei (CCN) in the remote marine boundary layer Zheng, Guangjie; Kuang, Chongai; Uin, Janek Atmospheric Chemistry and Physics, Vol. 20, Issue 21 https://doi.org/10.5194/acp-20-12515-2020	journal	January 2020
Organic matter distributions in the Eastern North Atlantic–Azores Front region Doval, M. D.; Álvarez-Salgado, X. A.; Pérez, F. F. Journal of Marine Systems, Vol. 30, Issue 1-2 https://doi.org/10.1016/S0924-7963(01)00036-7	journal	August 2001
Influence of oceanic dimethyl sulfide emissions on cloud condensation nuclei concentrations and seasonality over the remote Southern Hemisphere oceans: A global model study Korhonen, Hannele; Carslaw, Kenneth S.; Spracklen, Dominick V. Journal of Geophysical Research, Vol. 113, Issue D15 https://doi.org/10.1029/2007JD009718	journal	January 2008
Revising the hygroscopicity of inorganic sea salt particles Zieger, P.; Väisänen, O.; Corbin, J. C. Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/ncomms15883	journal	July 2017
A single parameter representation of hygroscopic growth and cloud condensation nucleus activity Petters, M. D.; Kreidenweis, S. M. Atmospheric Chemistry and Physics, Vol. 7, Issue 8 https://doi.org/10.5194/acp-7-1961-2007	journal	January 2007
A technology-based global inventory of black and organic carbon emissions from combustion Bond, Tami C. Journal of Geophysical Research, Vol. 109, Issue D14 https://doi.org/10.1029/2003JD003697	journal	January 2004
Morphology and mixing of black carbon particles collected in central California during the CARES field study Moffet, Ryan C.; O'Brien, Rachel E.; Alpert, Peter A. Atmospheric Chemistry and Physics, Vol. 16, Issue 22 https://doi.org/10.5194/acp-16-14515-2016	journal	January 2016
Fire and biofuel contributions to annual mean aerosol mass concentrations in the United States Park, Rokjin J.; Jacob, Daniel J.; Logan, Jennifer A. Atmospheric Environment, Vol. 41, Issue 35 https://doi.org/10.1016/j.atmosenv.2007.05.061	journal	November 2007
A new multicomponent heterogeneous ice nucleation model and its application to Snomax bacterial particles and a Snomax–illite mineral particle mixture Beydoun, Hassan; Polen, Michael; Sullivan, Ryan C. Atmospheric Chemistry and Physics, Vol. 17, Issue 22 https://doi.org/10.5194/acp-17-13545-2017	journal	January 2017
Black carbon lofts wildfire smoke high into the stratosphere to form a persistent plume Yu, Pengfei; Toon, Owen B.; Bardeen, Charles G. Science, Vol. 365, Issue 6453 https://doi.org/10.1126/science.aax1748	journal	August 2019
Biological Impacts on Carbon Speciation and Morphology of Sea Spray Aerosol Pham, Don Q.; O’Brien, Rachel; Fraund, Matthew ACS Earth and Space Chemistry, Vol. 1, Issue 9 https://doi.org/10.1021/acsearthspacechem.7b00069	journal	October 2017
Microscopic characterization of carbonaceous aerosol particle aging in the outflow from Mexico City Moffet, R. C.; Henn, T. R.; Tivanski, A. V. Atmospheric Chemistry and Physics, Vol. 10, Issue 3 https://doi.org/10.5194/acp-10-961-2010	journal	January 2010
Aerosol-driven droplet concentrations dominate coverage and water of oceanic low-level clouds Rosenfeld, Daniel; Zhu, Yannian; Wang, Minghuai Science, Vol. 363, Issue 6427 https://doi.org/10.1126/science.aav0566	journal	January 2019
Agricultural fires in the southeastern U.S. during SEAC ⁴ RS: Emissions of trace gases and particles and evolution of ozone, reactive nitrogen, and organic aerosol : Agricultural Fires in the SE US Liu, Xiaoxi; Zhang, Y.; Huey, L. G. Journal of Geophysical Research: Atmospheres, Vol. 121, Issue 12 https://doi.org/10.1002/2016JD025040	journal	June 2016
Soot Carbon and Excess Fine Potassium: Long-Range Transport of Combustion-Derived Aerosols Andreae, M. O. Science, Vol. 220, Issue 4602 https://doi.org/10.1126/science.220.4602.1148	journal	June 1983
Rapid measurement of sub-micrometer aerosol size distribution using a fast integrated mobility spectrometer Wang, Yang; Pinterich, Tamara; Wang, Jian Journal of Aerosol Science, Vol. 121 https://doi.org/10.1016/j.jaerosci.2018.03.006	journal	July 2018
Characterization of the Single Particle Mixing State of Individual Ship Plume Events Measured at the Port of Los Angeles Ault, Andrew P.; Gaston, Cassandra J.; Wang, Ying Environmental Science & Technology, Vol. 44, Issue 6 https://doi.org/10.1021/es902985h	journal	March 2010
A new method to quantify mineral dust and other aerosol species from aircraft platforms using single-particle mass spectrometry Froyd, Karl D.; Murphy, Daniel M.; Brock, Charles A. Atmospheric Measurement Techniques, Vol. 12, Issue 11 https://doi.org/10.5194/amt-12-6209-2019	journal	January 2019
Microlayer source of oxygenated volatile organic compounds in the summertime marine Arctic boundary layer Mungall, Emma L.; Abbatt, Jonathan P. D.; Wentzell, Jeremy J. B. Proceedings of the National Academy of Sciences, Vol. 114, Issue 24 https://doi.org/10.1073/pnas.1620571114	journal	May 2017
Aging of Atmospheric Brown Carbon Aerosol Hems, Rachel F.; Schnitzler, Elijah G.; Liu-Kang, Carolyn ACS Earth and Space Chemistry, Vol. 5, Issue 4 https://doi.org/10.1021/acsearthspacechem.0c00346	journal	April 2021
The free troposphere as a potential source of arctic boundary layer aerosol particles: Free Troposphere and Boundary Layer Arctic Aerosol Igel, Adele L.; Ekman, Annica M. L.; Leck, Caroline Geophysical Research Letters, Vol. 44, Issue 13 https://doi.org/10.1002/2017GL073808	journal	July 2017
Toward aerosol/cloud condensation nuclei (CCN) closure during CRYSTAL-FACE VanReken, Timothy M. Journal of Geophysical Research, Vol. 108, Issue D20 https://doi.org/10.1029/2003JD003582	journal	January 2003
Analysis of Atmospheric Aerosols Prather, Kimberly A.; Hatch, Courtney D.; Grassian, Vicki H. Annual Review of Analytical Chemistry, Vol. 1, Issue 1 https://doi.org/10.1146/annurev.anchem.1.031207.113030	journal	July 2008
Long-term cloud condensation nuclei number concentration, particle number size distribution and chemical composition measurements at regionally representative observatories Schmale, Julia; Henning, Silvia; Decesari, Stefano Atmospheric Chemistry and Physics, Vol. 18, Issue 4 https://doi.org/10.5194/acp-18-2853-2018	journal	January 2018
Individual aerosol particles from biomass burning in southern Africa: 2, Compositions and aging of inorganic particles: COMPOSITIONS AND AGING OF INORGANIC PARTICLES Li, Jia; Pósfai, Mihály; Hobbs, Peter V. Journal of Geophysical Research: Atmospheres, Vol. 108, Issue D13 https://doi.org/10.1029/2002JD002310	journal	March 2003
Transport of the 2017 Canadian wildfire plume to the tropics via the Asian monsoon circulation Kloss, Corinna; Berthet, Gwenaël; Sellitto, Pasquale Atmospheric Chemistry and Physics, Vol. 19, Issue 21 https://doi.org/10.5194/acp-19-13547-2019	journal	January 2019
Molecular characterization of free tropospheric aerosol collected at the Pico Mountain Observatory: a case study with a long-range transported biomass burning plume Dzepina, K.; Mazzoleni, C.; Fialho, P. Atmospheric Chemistry and Physics, Vol. 15, Issue 9 https://doi.org/10.5194/acp-15-5047-2015	journal	January 2015
Photochemical reactions on aerosols at West Antarctica: A molecular case-study of nitrate formation among sea salt aerosols Gonçalves, Sérgio J.; Weis, Johannes; China, Swarup Science of The Total Environment, Vol. 758 https://doi.org/10.1016/j.scitotenv.2020.143586	journal	March 2021
The time evolution of aerosol composition over the Mexico City plateau Kleinman, L. I.; Springston, S. R.; Daum, P. H. Atmospheric Chemistry and Physics, Vol. 8, Issue 6 https://doi.org/10.5194/acp-8-1559-2008	journal	January 2008
Aerosol Mixing State: Measurements, Modeling, and Impacts Riemer, N.; Ault, A. P.; West, M. Reviews of Geophysics, Vol. 57, Issue 2 https://doi.org/10.1029/2018RG000615	journal	May 2019
The importance of aerosol mixing state and size-resolved composition on CCN concentration and the variation of the importance with atmospheric aging of aerosols Wang, J.; Cubison, M. J.; Aiken, A. C. Atmospheric Chemistry and Physics, Vol. 10, Issue 15 https://doi.org/10.5194/acp-10-7267-2010	journal	January 2010
Effects of aging on organic aerosol from open biomass burning smoke in aircraft and laboratory studies Cubison, M. J.; Ortega, A. M.; Hayes, P. L. Atmospheric Chemistry and Physics, Vol. 11, Issue 23 https://doi.org/10.5194/acp-11-12049-2011	journal	January 2011
Size-Dependent Changes in Sea Spray Aerosol Composition and Properties with Different Seawater Conditions Ault, Andrew P.; Moffet, Ryan C.; Baltrusaitis, Jonas Environmental Science & Technology, Vol. 47, Issue 11 https://doi.org/10.1021/es400416g	journal	May 2013
Effects of aerosol organics on cloud condensation nucleus (CCN) concentration and first indirect aerosol effect Wang, J.; Lee, Y. -N.; Daum, P. H. Atmospheric Chemistry and Physics, Vol. 8, Issue 21 https://doi.org/10.5194/acp-8-6325-2008	journal	January 2008

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