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Title: Short-Range Nematic Fluctuations in Sr1-xNaxFe2As2 Superconductors

Journal Article · · Physical Review Letters
ORCiD logo [1];  [2];  [3];  [4];  [5];  [1]; ORCiD logo [6]; ORCiD logo [7];  [7];  [8];  [8];  [8];  [1]
  1. Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  2. Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Zhejiang Univ., Hangzhou (China)
  3. Univ. of California, Berkeley, CA (United States)
  4. Univ. of California, San Diego, CA (United States)
  5. Rice Univ., Houston, TX (United States)
  6. Japan Synchrotron Radiation Research Inst., Sayo (Japan)
  7. Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source (APS)
  8. Karlsruhe Inst. of Technology (KIT) (Germany). Inst. for Quantum Materials and Technologies

Interactions between nematic fluctuations, magnetic order and superconductivity are central to the physics of iron-based superconductors. Here we report on in-plane transverse acoustic phonons in hole-doped Sr1-xNaxFe2As2 measured via inelastic x-ray scattering, and extract both the nematic susceptibility and the nematic correlation length. By a self-contained method of analysis, for the underdoped (x = 0.36) sample, which harbors a magnetically ordered tetragonal phase, we find it hosts a short nematic correlation length ξ ~ 10Å and a large nematic susceptibility Χnem. The optimal-doped (x = 0.55) sample exhibits weaker phonon softening effects, indicative of both reduced xi and Χnem. Overall, our results suggest short-range nematic fluctuations may favor superconductivity, placing emphasis on the nematic correlation length for understanding the iron-based superconductors.

Research Organization:
Argonne National Lab. (ANL), Argonne, IL (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
Alfred P. Sloan Foundation; Welch Foundation; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division
Grant/Contract Number:
AC02-06CH11357; AC02-05CH11231
OSTI ID:
1787865
Alternate ID(s):
OSTI ID: 1877039
Journal Information:
Physical Review Letters, Vol. 126, Issue 10; ISSN 0031-9007
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (59)

Electronic nematic susceptibility of iron-based superconductors journal January 2016
Nematicity as a Probe of Superconducting Pairing in Iron-Based Superconductors journal September 2013
Elastic coupling and spin-driven nematicity in iron-based superconductors journal February 2016
Soft elastic constants from phonon spectroscopy in hole-doped Ba 1 x ( K , Na ) x Fe 2 As 2 and Sr 1 x Na x Fe 2 As 2 journal October 2020
Isostructural Spin-Density-Wave and Superconducting Gap Anisotropies in Iron-Arsenide Superconductors journal June 2020
Double-Q spin-density wave in iron arsenide superconductors journal January 2016
Manifestations of nematic degrees of freedom in the magnetic, elastic, and superconducting properties of the iron pnictides journal July 2012
Nematic Correlation Length in Iron-Based Superconductors Probed by Inelastic X-Ray Scattering journal April 2020
Magnetically driven suppression of nematic order in an iron-based superconductor journal May 2014
Widespread orthorhombic fluctuations in the ( Sr , Na ) Fe 2 As 2 family of superconductors journal November 2018
Using disorder to detect locally ordered electron nematics via hysteresis journal July 2011
Critical spin fluctuations and the origin of nematic order in Ba(Fe1−xCox)2As2 journal January 2016
Detailed magnetic and structural analysis mapping a robust magnetic C 4 dome in Sr 1 x Na x Fe 2 As 2 journal April 2016
Coexistence of Competing Antiferromagnetic and Superconducting Phases in the Underdoped Ba ( Fe 0.953 Co 0.047 ) 2 As 2 Compound Using X-ray and Neutron Scattering Techniques journal August 2009
An X-ray scattering beamline for studying dynamics journal March 2000
Soft phonons reveal the nematic correlation length in Ba ( Fe 0.94 Co 0.06 ) 2 As 2 journal July 2018
Strong correlations, strong coupling, and s -wave superconductivity in hole-doped BaFe 2 As 2 single crystals journal November 2016
Divergent Nematic Susceptibility in an Iron Arsenide Superconductor journal August 2012
Superconductivity with broken time-reversal symmetry inside a superconducting s-wave state journal May 2020
Local Orthorhombicity in the Magnetic C 4 Phase of the Hole-Doped Iron-Arsenide Superconductor Sr 1 x Na x Fe 2 As 2 journal October 2017
Raman scattering study of the tetragonal magnetic phase in Sr 1 x Na x Fe 2 As 2 : Structural symmetry and electronic gap journal November 2017
Large nematic susceptibility in the double- Q C 4 magnetic phase of Ba 1 x Na x Fe 2 As 2 journal June 2018
Disorder-promoted C 4 -symmetric magnetic order in iron-based superconductors journal April 2016
Anomalous Suppression of the Orthorhombic Lattice Distortion in Superconducting Ba ( Fe 1 x Co x ) 2 As 2 Single Crystals journal February 2010
Antiferromagnetic critical fluctuations in BaFe 2 As 2 journal October 2010
Effects of Nematic Fluctuations on the Elastic Properties of Iron Arsenide Superconductors journal October 2010
Local nematic susceptibility in stressed BaFe 2 As 2 from NMR electric field gradient measurements journal December 2017
Nematic Fermi Fluids in Condensed Matter Physics journal August 2010
Dynamic competition between spin-density wave order and superconductivity in underdoped Ba1−xKxFe2As2 journal April 2014
Ubiquitous signatures of nematic quantum criticality in optimally doped Fe-based superconductors journal May 2016
Character of the structural and magnetic phase transitions in the parent and electron-doped BaFe 2 As 2 compounds journal April 2011
Close correlation between magnetic properties and the soft phonon mode of the structural transition in BaFe 2 As 2 and SrFe 2 As 2 journal April 2015
Spin reorientation driven by the interplay between spin-orbit coupling and Hund's rule coupling in iron pnictides journal December 2015
Determination of anisotropic H c 2 up to 60 T in Ba 0.55 K 0.45 Fe 2 As 2 single crystals journal December 2008
Structural Quantum Criticality and Superconductivity in Iron-Based Superconductor Ba(Fe 1- x Co x ) 2 As 2 journal February 2012
Antiferromagnetic order and spin dynamics in iron-based superconductors journal August 2015
Superconductivity and electronic fluctuations in Ba 1 x K x Fe 2 As 2 studied by Raman scattering journal February 2017
Superconductivity-induced re-entrance of the orthorhombic distortion in Ba1−xKxFe2As2 journal July 2015
Enhancement of Superconductivity near a Nematic Quantum Critical Point journal March 2015
Competing magnetic double- Q phases and superconductivity-induced reentrance of C 2 magnetic stripe order in iron pnictides journal October 2015
Observation of the magnetic C 4 phase in Ca 1 x Na x Fe 2 As 2 and its universality in the hole-doped 122 superconductors journal February 2017
Nearly isotropic superconductivity in (Ba,K)Fe2As2 journal January 2009
Charge nematicity and electronic Raman scattering in iron-based superconductors journal January 2016
Six-reflection meV-monochromator for synchrotron radiation journal May 2011
Spin reorientation in Ba 0.65 Na 0.35 Fe 2 As 2 studied by single-crystal neutron diffraction journal February 2015
Spectral Evidence for Emergent Order in Ba 1 x Na x Fe 2 As 2 journal September 2018
Dynamic Spin-Lattice Coupling and Nematic Fluctuations in NaFeAs journal June 2018
Competing Electronic Phases near the Onset of Superconductivity in Hole-doped SrFe 2 As 2 journal October 2019
First- and second-order magnetic and structural transitions in BaFe 2 ( 1 x ) Co 2 x As 2 journal September 2011
Complex phase diagram of Ba 1 x Na x Fe 2 As 2 : A multitude of phases striving for the electronic entropy journal January 2016
Acoustic phonon instabilities and structural phase transitions journal June 1976
Electronic nematicity above the structural and superconducting transition in BaFe2(As1−xP x )2 journal June 2012
What drives nematic order in iron-based superconductors? journal January 2014
Phonon softening near the structural transition in BaFe 2 As 2 observed by inelastic x-ray scattering journal December 2011
In-Plane Resistivity Anisotropy in an Underdoped Iron Arsenide Superconductor journal August 2010
High-energy-resolution inelastic X-ray scattering spectrometer at beamline 30-ID of the Advanced Photon Source journal April 2020
Mean field theory, the Ginzburg criterion, and marginal dimensionality of phase transitions journal June 1977
Noise predictions for STM in systems with local electron nematic order journal June 2010
Local orthorhombic lattice distortions in the paramagnetic tetragonal phase of superconducting NaFe1−xNixAs journal August 2018