Development and Evaluation of Chemistry‐Aerosol‐Climate Model CAM5‐Chem‐MAM7‐MOSAIC: Global Atmospheric Distribution and Radiative Effects of Nitrate Aerosol

Zaveri, Rahul A.; Easter, Richard C.; Singh, Balwinder; Wang, Hailong; Lu, Zheng; Tilmes, Simone; Emmons, Louisa K.; Vitt, Francis; Zhang, Rudong; Liu, Xiaohong; Ghan, Steven J.; Rasch, Philip J.

doi:10.1029/2020MS002346

Title: Development and Evaluation of Chemistry‐Aerosol‐Climate Model CAM5‐Chem‐MAM7‐MOSAIC: Global Atmospheric Distribution and Radiative Effects of Nitrate Aerosol

Journal Article · Fri Apr 16 00:00:00 EDT 2021 · Journal of Advances in Modeling Earth Systems

DOI:https://doi.org/10.1029/2020MS002346· OSTI ID:1780219

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Atmospheric Sciences and Global Change Division Pacific Northwest National Laboratory Richland WA USA
Department of Atmospheric Sciences Texas A&,M University College Station TX USA
Atmospheric Chemistry Observations and Modeling Laboratory National Center for Atmospheric Research Boulder CO USA

Abstract An advanced aerosol treatment, with a focus on semivolatile nitrate formation, is introduced into the Community Atmosphere Model version 5 with interactive chemistry (CAM5‐chem) by coupling the Model for Simulating Aerosol Interactions and Chemistry (MOSAIC) with the 7‐mode Modal Aerosol Module (MAM7). An important feature of MOSAIC is dynamic partitioning of all condensable gases to the different fine and coarse mode aerosols, as governed by mode‐resolved thermodynamics and heterogeneous chemical reactions. Applied in the free‐running mode from 1995 to 2005 with prescribed historical climatological conditions, the model simulates global distributions of sulfate, nitrate, and ammonium in good agreement with observations and previous studies. Inclusion of nitrate resulted in ∼10% higher global average accumulation mode number concentrations, indicating enhanced growth of Aitken mode aerosols from nitrate formation. While the simulated accumulation mode nitrate burdens are high over the anthropogenic source regions, the sea‐salt and dust modes respectively constitute about 74% and 17% of the annual global average nitrate burden. Regional clear‐sky shortwave radiative cooling of up to −5 W m ⁻² due to nitrate is seen, with a much smaller global average cooling of −0.05 W m ⁻² . Significant enhancements in regional cloud condensation nuclei (at 0.1% supersaturation) and cloud droplet number concentrations are also attributed to nitrate, causing an additional global average shortwave cooling of −0.8 W m ⁻² . Taking into consideration of changes in both longwave and shortwave radiation under all‐sky conditions, the net change in the top of the atmosphere radiative fluxes induced by including nitrate aerosol is −0.7 W m ⁻² .

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Research Organization:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Biological and Environmental Research (BER)

Grant/Contract Number:: AC05-76RL01830

OSTI ID:: 1780219

Alternate ID(s):: OSTI ID: 1782916; OSTI ID: 1815512

Journal Information:: Journal of Advances in Modeling Earth Systems, Journal Name: Journal of Advances in Modeling Earth Systems Vol. 13 Journal Issue: 4; ISSN 1942-2466

Publisher:: American Geophysical Union (AGU)Copyright Statement

Country of Publication:: United States

Language:: English

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