Three-Dimensional Microbatteries beyond Lithium Ion

Ni, Jiangfeng; Dai, Alvin; Yuan, Yifei; Li, Liang; Lu, Jun

doi:10.1016/j.matt.2020.04.020

Title: Three-Dimensional Microbatteries beyond Lithium Ion

Journal Article · Wed Jun 03 00:00:00 EDT 2020 · Matter (Online)

DOI:https://doi.org/10.1016/j.matt.2020.04.020· OSTI ID:1774514

Ni, Jiangfeng ^[1]; Dai, Alvin ^[2]; Yuan, Yifei ^[2]; Li, Liang ^[1]; Lu, Jun ^[2]

Soochow Univ., (China)
Argonne National Lab. (ANL), Argonne, IL (United States)

Ubiquitous implementation of microelectronics in microelectromechanical systems requires stable power supplies and necessitates development of on-chip miniature power sources, such as microbatteries. However, conventional thin-film batteries exhibit limited surface area and sluggish diffusion kinetics with insufficient energy and power density. In contrast, three-dimensional (3D) beyond-lithium (sodium, zinc, aluminum, etc.) battery architectures can significantly enhance the areal energy and power and meanwhile maintain the low-cost mass production. Despite this, the future of beyond-lithium systems is being questioned as they each present shortcomings. In this Comment, we discuss scientific advancements in reaction kinetics control, electrochemical stability improvements, and reaction mechanism understandings in 3D beyond-lithium battery systems, and finally, call for intensive research effort to address the challenges and develop strategies that can pave the way toward their commercialization.

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Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Transportation Office. Vehicle Technologies Office; National Natural Science Foundation of China (NSFC); Thousand Talents Plan (TTP) of China; Jiangsu Natural Science Foundation; USDOE Office of Energy Efficiency and Renewable Energy (EERE)

Grant/Contract Number:: AC02-06CH11357; 51872192; 51672182; 51772197; BK20180002; 19KJA170001; 17KJA430013

OSTI ID:: 1774514

Alternate ID(s):: OSTI ID: 1694358

Journal Information:: Matter (Online), Vol. 2, Issue 6; ISSN 2590-2385

Publisher:: Cell Press/ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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25 ENERGY STORAGE
beyond-lithium systems
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three-dimensional architecture
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Title: Three-Dimensional Microbatteries beyond Lithium Ion

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