Search for multipolar instability in URu2Si2 studied by ultrasonic measurements under pulsed magnetic field

Yanagisawa, T.; Mombetsu, S.; Hidaka, H.; Amitsuka, H.; Cong, P. T.; Yasin, S; Zherlitsyn, S.; Wosnitza, J.; Huang, K.; Kanchanavatee, N.; Janoschek, Marc; Maple, M. B.; Aoki, D.

doi:10.1103/physrevb.97.155137

Title: Search for multipolar instability in URu₂Si₂ studied by ultrasonic measurements under pulsed magnetic field

Journal Article · Tue Apr 17 00:00:00 EDT 2018 · Physical Review B

DOI:https://doi.org/10.1103/physrevb.97.155137· OSTI ID:1766990

Yanagisawa, T. ^[1]; Mombetsu, S. ^[1]; Hidaka, H. ^[1]; Amitsuka, H. ^[1]; Cong, P. T. ^[2]; Yasin, S ^[2]; Zherlitsyn, S. ^[2]; Wosnitza, J. ^[3]; Huang, K. ^[4]; Kanchanavatee, N. ^[4];

^[5]; Maple, M. B. ^[4]; Aoki, D. ^[6]

Hokkaido Univ., Sapporo (Japan)
Helmholtz-Zentrum Dresden-Rossendorf, Dresden (Germany)
Helmholtz-Zentrum Dresden-Rossendorf, Dresden (Germany); Dresden Univ. of Technology (Germany)
Univ. of California, San Diego, CA (United States)
Univ. of California, San Diego, CA (United States); Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Tohoku Univ., Sendai (Japan); Alternative Energies and Atomic Energy Commission (CEA), Grenoble (France)

In this study, the elastic properties of URu₂Si₂ in the high magnetic field region above 40 T, over a wide temperature range from 1.5 to 120 K, were systematically investigated by means of high-frequency ultrasonic measurements. The investigation was performed at high magnetic fields to better investigate the innate bare 5f-electron properties, since the unidentified electronic thermodynamic phase of unknown origin, the so-called “hidden order” (HO), and associated hybridization of conduction and f-electrons (c-f hybridization) are suppressed at high magnetic fields. From the three different transverse modes we find contrasting results; both the Γ₄(B_2g) and Γ₅(E_g) symmetry modes C₆₆ and C₄₄ show elastic softening that is enhanced above 30 T, while the characteristic softening of the Γ₃(B_1g) symmetry mode (C₁₁ – C₁₂)/2 is suppressed in high magnetic fields. These results underscore the presence of a hybridization-driven Γ₃(B_1g) lattice instability in URu₂Si₂. However, the results from this work cannot be explained by using existing crystalline electric field schemes applied to the quadrupolar susceptibility in a local 5f² configuration. Instead, we present an analysis based on a band Jahn-Teller effect.

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE Office of Science (SC). Basic Energy Sciences (BES) (SC-22); USDOE National Nuclear Security Administration (NNSA); Japan Society for the Promotion of Science (JSPS)

Grant/Contract Number:: 89233218CNA000001; FG02-04-ER46105; JP17K05525(C); JP16H04006; JP15H05882; JP15H05884; JP15H05745; JP15KK0146; JP15K21732; JP23740250; JP23102701

OSTI ID:: 1766990

Alternate ID(s):: OSTI ID: 1433456

Report Number(s):: LA-UR-18-28593; TRN: US2206324

Journal Information:: Physical Review B, Vol. 97, Issue 15; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 9 works

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References (48)

High-Temperature Magnetic Investigations on Uranium Compounds Galatanu, Andrei; Haga, Yoshinori; D. Matsuda, Tatsuma Journal of the Physical Society of Japan, Vol. 74, Issue 5 https://doi.org/10.1143/JPSJ.74.1582	journal	May 2005
Partially gapped Fermi surface in the heavy-electron superconductor ${URu}_{2}$ ${Si}_{2}$ Maple, M. B.; Chen, J. W.; Dalichaouch, Y. Physical Review Letters, Vol. 56, Issue 2 https://doi.org/10.1103/PhysRevLett.56.185	journal	January 1986
Phase transition arising from the underscreened Anderson lattice model: A candidate concept for explaining hidden order in URu $_{2}$ Si $_{2}$ Riseborough, Peter S.; Coqblin, B.; Magalhães, S. G. Physical Review B, Vol. 85, Issue 16 https://doi.org/10.1103/PhysRevB.85.165116	journal	April 2012
A Study of Elastic Properties of URu ₂ Si ₂ in Comparison with the Non-5 f Contribution of ThRu ₂ Si ₂ Yanagisawa, T.; Saito, H.; Watanabe, Y. Journal of Physics: Conference Series, Vol. 391 https://doi.org/10.1088/1742-6596/391/1/012079	journal	December 2012
Hidden and antiferromagnetic order as a rank-5 superspin in URu $_{2}$ Si $_{2}$ Rau, Jeffrey G.; Kee, Hae-Young Physical Review B, Vol. 85, Issue 24 https://doi.org/10.1103/PhysRevB.85.245112	journal	June 2012
On the Hidden Order in URu$_{2}$Si$_{2}$ --- Antiferro Hexadecapole Order and its Consequences Kusunose, Hiroaki; Harima, Hisatomo arXiv https://doi.org/10.48550/arxiv.1104.2374	text	January 2011
Magnetoelastic interaction in rare earth systems Dohm, Volker; Fulde, Peter Zeitschrift f�r Physik B Condensed Matter and Quanta, Vol. 21, Issue 4 https://doi.org/10.1007/BF01325397	journal	December 1975
Rare Earth systems in a magnetic field: Coupling of elastic and magnetic properties Thalmeier, Peter; Fulde, Peter Zeitschrift f�r Physik B Condensed Matter and Quanta, Vol. 22, Issue 4 https://doi.org/10.1007/BF01312806	journal	December 1975
Elastic constants of antiferro-quadrupole ordering system DyB2C2 Nemoto, Y. Physica B: Condensed Matter, Vol. 329-333 https://doi.org/10.1016/S0921-4526(02)02552-8	journal	May 2003
High-Magnetic-Field Lattice Length Changes in ${URu}_{2} {Si}_{2}$ Correa, V. F.; Francoual, S.; Jaime, M. Physical Review Letters, Vol. 109, Issue 24 https://doi.org/10.1103/PhysRevLett.109.246405	journal	December 2012
Field-induced spin-density wave beyond hidden order in URu2Si2 Knafo, W.; Duc, F.; Bourdarot, F. Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms13075	journal	October 2016
Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of ${URu}_{2} {Si}_{2}$ Mydosh, J. A.; Oppeneer, P. M. Reviews of Modern Physics, Vol. 83, Issue 4 https://doi.org/10.1103/RevModPhys.83.1301	journal	November 2011
Magnetic-Field-Induced Quantum Critical Point and Competing Order Parameters in ${U R u}_{2} {S i}_{2}$ Kim, K. H.; Harrison, N.; Jaime, M. Physical Review Letters, Vol. 91, Issue 25 https://doi.org/10.1103/PhysRevLett.91.256401	journal	December 2003
Importance of In-Plane Anisotropy in the Quasi-Two-Dimensional Antiferromagnet ${BaNi}_{2} V_{2} O_{8}$ Knafo, W.; Meingast, C.; Grube, K. Physical Review Letters, Vol. 99, Issue 13 https://doi.org/10.1103/PhysRevLett.99.137206	journal	September 2007
Evidence for a nematic component to the hidden-order parameter in URu2Si2 from differential elastoresistance measurements Riggs, Scott C.; Shapiro, M. C.; Maharaj, Akash V. Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms7425	journal	March 2015
Emergent rank-5 nematic order in URu2Si2 Ikeda, Hiroaki; Suzuki, Michi-To; Arita, Ryotaro Nature Physics, Vol. 8, Issue 7 https://doi.org/10.1038/nphys2330	journal	June 2012
Hidden orbital order in the heavy fermion metal URu2Si2 Chandra, P.; Coleman, P.; Mydosh, J. A. Nature, Vol. 417, Issue 6891 https://doi.org/10.1038/nature00795	journal	June 2002
Interplay of magnetism, Fermi surface reconstructions, and hidden order in the heavy-fermion material URu $_{2}$ Si $_{2}$ Scheerer, G. W.; Knafo, W.; Aoki, D. Physical Review B, Vol. 85, Issue 9 https://doi.org/10.1103/PhysRevB.85.094402	journal	March 2012
Group theory and octupolar order in $U {Ru}_{2} {Si}_{2}$ Kiss, Annamária; Fazekas, Patrik Physical Review B, Vol. 71, Issue 5 https://doi.org/10.1103/PhysRevB.71.054415	journal	February 2005
Structural Quantum Criticality and Superconductivity in Iron-Based Superconductor Ba(Fe _{1- x} Co _x ) ₂ As ₂ Yoshizawa, Masahito; Kimura, Daichi; Chiba, Taiji Journal of the Physical Society of Japan, Vol. 81, Issue 2 https://doi.org/10.1143/JPSJ.81.024604	journal	February 2012
Possible Phase Transition Deep Inside the Hidden Order Phase of Ultraclean ${URu}_{2} {Si}_{2}$ Shishido, H.; Hashimoto, K.; Shibauchi, T. Physical Review Letters, Vol. 102, Issue 15 https://doi.org/10.1103/PhysRevLett.102.156403	journal	April 2009
Possible Phase Transition Deep Inside the Hidden Order Phase of Ultraclean URu2Si2 Shishido, H.; Hashimoto, K.; Shibauchi, T. arXiv https://doi.org/10.48550/arxiv.0903.3821	text	January 2009
Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2 Tonegawa, S.; Kasahara, S.; Fukuda, T. arXiv https://doi.org/10.48550/arxiv.1406.5040	text	January 2014
Structural quantum criticality and superconductivity in iron-based superconductor Ba(Fe1-xCox)2As2 Yoshizawa, Masahito; Kimura, Daichi; Chiba, Taiji arXiv https://doi.org/10.48550/arxiv.1111.0366	text	January 2011
Hybridization-driven orthorhombic lattice instability in URu $_{2}$ Si $_{2}$ Yanagisawa, T.; Mombetsu, S.; Hidaka, H. Physical Review B, Vol. 88, Issue 19 https://doi.org/10.1103/PhysRevB.88.195150	journal	November 2013
LaAg x In1?x: II. Phonon dispersion, elastic constants and structural instability Knorr, K.; Renker, B.; Assmus, W. Zeitschrift f�r Physik B Condensed Matter, Vol. 39, Issue 2 https://doi.org/10.1007/BF01301521	journal	June 1980
Resonant X-ray scattering study of hidden order in URu ₂ Si ₂ using a low-stress single crystal Amitsuka, H.; Inami, T.; Yokoyama, M. Journal of Physics: Conference Series, Vol. 200, Issue 1 https://doi.org/10.1088/1742-6596/200/1/012007	journal	January 2010
Arrested Kondo effect and hidden order in URu_2Si_2 Haule, Kristjan; Kotliar, Gabriel arXiv https://doi.org/10.48550/arxiv.0907.3889	text	January 2009
Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2 Okazaki, R.; Shibauchi, T.; Shi, H. J. arXiv https://doi.org/10.48550/arxiv.1107.5480	text	January 2011
On the Hidden Order in URu ₂ Si ₂ – Antiferro Hexadecapole Order and Its Consequences Kusunose, Hiroaki; Harima, Hisatomo Journal of the Physical Society of Japan, Vol. 80, Issue 8 https://doi.org/10.1143/JPSJ.80.084702	journal	August 2011
Crystalline electric field effects in ${UPt}_{2}$ ${Si}_{2}$ and ${URu}_{2}$ ${Si}_{2}$ Nieuwenhuys, G. J. Physical Review B, Vol. 35, Issue 10 https://doi.org/10.1103/PhysRevB.35.5260	journal	April 1987
Hidden order in URu2Si2 originates from Fermi surface gapping induced by dynamic symmetry breaking Elgazzar, S.; Rusz, J.; Amft, M. Nature Materials, Vol. 8, Issue 4 https://doi.org/10.1038/nmat2395	journal	February 2009
Arrested Kondo effect and hidden order in URu2Si2 Haule, Kristjan; Kotliar, Gabriel Nature Physics, Vol. 5, Issue 11 https://doi.org/10.1038/nphys1392	journal	September 2009
Direct bulk-sensitive probe of 5 f symmetry in URu ₂ Si ₂ Sundermann, Martin; Haverkort, Maurits W.; Agrestini, Stefano Proceedings of the National Academy of Sciences, Vol. 113, Issue 49 https://doi.org/10.1073/pnas.1612791113	journal	November 2016
Chirality density wave of the 'hidden order' phase in URu$_2$Si$_2$ Kung, H. -H.; Baumbach, R. E.; Bauer, E. D. arXiv https://doi.org/10.48550/arxiv.1410.6398	text	January 2014
Superconductivity and magnetic order in a strongly interacting fermi-system: URu2Si2 Schlabitz, W.; Baumann, J.; Pollit, B. Zeitschrift f�r Physik B Condensed Matter, Vol. 62, Issue 2 https://doi.org/10.1007/BF01323427	journal	June 1986
Heavy-fermion behaviours in URu ₂ Si ₂ Hanzawa, Katsurou; Watanabe, Naoto Journal of Physics: Condensed Matter, Vol. 17, Issue 41 https://doi.org/10.1088/0953-8984/17/41/L04	journal	September 2005
Superconducting and Magnetic Transitions in the Heavy-Fermion System U ${Ru}_{2}$ ${Si}_{2}$ Palstra, T. T. M.; Menovsky, A. A.; Berg, J. van den Physical Review Letters, Vol. 55, Issue 24 https://doi.org/10.1103/PhysRevLett.55.2727	journal	December 1985
Symmetry of the Excitations in the Hidden Order State of ${URu}_{2} {Si}_{2}$ Buhot, J.; Méasson, M. -A.; Gallais, Y. Physical Review Letters, Vol. 113, Issue 26 https://doi.org/10.1103/PhysRevLett.113.266405	journal	December 2014
Critical Slowing Down of Quadrupole and Hexadecapole Orderings in Iron Pnictide Superconductor Kurihara, Ryosuke; Mitsumoto, Keisuke; Akatsu, Mitsuhiro Journal of the Physical Society of Japan, Vol. 86, Issue 6 https://doi.org/10.7566/JPSJ.86.064706	journal	June 2017
High-magnetic field lattice length changes in URu2Si2 Correa, V. F.; Francoual, S.; Jaime, M. arXiv https://doi.org/10.48550/arxiv.1211.3051	text	January 2012
Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2 Okazaki, R.; Shibauchi, T.; Shi, H. J. Science, Vol. 331, Issue 6016 https://doi.org/10.1126/science.1197358	journal	January 2011
Chirality density wave of the "hidden order" phase in URu2Si2 Kung, H. - H.; Baumbach, R. E.; Bauer, E. D. Science, Vol. 347, Issue 6228 https://doi.org/10.1126/science.1259729	journal	February 2015
Crystal Field Model of the Magnetic Properties of U ${Ru}_{2}$ ${Si}_{2}$ Santini, P.; Amoretti, G. Physical Review Letters, Vol. 73, Issue 7 https://doi.org/10.1103/PhysRevLett.73.1027	journal	August 1994
Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2 Tonegawa, S.; Kasahara, S.; Fukuda, T. Nature Communications, Vol. 5, Issue 1 https://doi.org/10.1038/ncomms5188	journal	June 2014
Hidden Order in ${URu}_{2} {Si}_{2}$ Unveiled Ressouche, E.; Ballou, R.; Bourdarot, F. Physical Review Letters, Vol. 109, Issue 6 https://doi.org/10.1103/PhysRevLett.109.067202	journal	August 2012
Γ ₃ -Type Lattice Instability and the Hidden Order of URu ₂ Si ₂ Yanagisawa, Tatsuya; Mombetsu, Shota; Hidaka, Hiroyuki Journal of the Physical Society of Japan, Vol. 82, Issue 1 https://doi.org/10.7566/JPSJ.82.013601	journal	January 2013
Evidence for a nematic component to the Hidden Order parameter in URu2Si2 from differential elastoresistance measurements Riggs, Scott C.; Shapiro, M. C.; Maharaj, Akash V. arXiv https://doi.org/10.48550/arxiv.1405.7403	text	January 2014

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Evidence for the Single-Site Quadrupolar Kondo Effect in the Dilute Non-Kramers System $Y_{1 - x} \Pr_{x} {Ir}_{2} {Zn}_{20}$ Yanagisawa, T.; Hidaka, H.; Amitsuka, H. Physical Review Letters, Vol. 123, Issue 6 https://doi.org/10.1103/physrevlett.123.067201	journal	August 2019
Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu ₂ Si ₂ Mydosh, J. A.; Oppeneer, P. M.; Riseborough, P. S. Journal of Physics: Condensed Matter, Vol. 32, Issue 14 https://doi.org/10.1088/1361-648x/ab5eba	journal	January 2020
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Title: Search for multipolar instability in URu2Si2 studied by ultrasonic measurements under pulsed magnetic field

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Title: Search for multipolar instability in URu₂Si₂ studied by ultrasonic measurements under pulsed magnetic field