Nonadiabatic coupling of the dynamical structure to the superconductivity in YSr2Cu2.75Mo0.25O7.54 and Sr2CuO3.3

Conradson, Steven D.; Geballe, Theodore H.; Jin, Chang-Qing; Cao, Li-Peng; Gauzzi, Andrea; Karppinen, Maarit; Baldinozzi, Gianguido; Li, Wen-Min; Gilioli, Edmondo; Jiang, Jack M.; Latimer, Matthew; Mueller, Oliver; Nasretdinova, Venera

doi:10.1073/pnas.2018336117

Title: Nonadiabatic coupling of the dynamical structure to the superconductivity in YSr₂Cu_2.75Mo_0.25O_7.54 and Sr₂CuO_3.3

Journal Article · Mon Dec 14 00:00:00 EST 2020 · Proceedings of the National Academy of Sciences of the United States of America

DOI:https://doi.org/10.1073/pnas.2018336117· OSTI ID:1755491

^[1]; Geballe, Theodore H. ^[2]; Jin, Chang-Qing ^[3]; Cao, Li-Peng ^[3];

^[4];

^[5];

^[6]; Li, Wen-Min ^[3];

^[7];

^[8]; Latimer, Matthew ^[9]; Mueller, Oliver ^[9];

^[10]

Jozef Stefan Inst. (IJS), Ljubljana (Slovenia); Washington State Univ., Pullman, WA (United States)
Stanford Univ., CA (United States)
Chinese Academy of Sciences (CAS), Beijing (China)
Sorbonne Univ., Paris (France); Centre National de la Recherche Scientifique (CNRS), Paris (France)
Aalto Univ., Otaniemi (Finland)
Univ. Paris-Saclay, Gif-sur-Yvette (France)
Consiglio Nazionale delle Ricerche (CNR), Parma (Italy)
Stanford Univ., CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES)
SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Synchrotron Radiation Lightsource (SSRL)
Jozef Stefan Inst. (IJS), Ljubljana (Slovenia)

A crucial issue in cuprates is the extent and mechanism of the coupling of the lattice to the electrons and the superconductivity. Here we report Cu K edge extended X-ray absorption fine structure measurements elucidating the internal quantum tunneling polaron (iqtp) component of the dynamical structure in two heavily overdoped superconducting cuprate compounds, tetragonal YSr₂Cu_2.75Mo_0.25O_7.54 with superconducting critical temperature, T_c = 84 K and hole density p = 0.3 to 0.5 per planar Cu, and the tetragonal phase of Sr₂CuO_3.3 with T_c = 95 K and p = 0.6. In YSr₂Cu_2.75Mo_0.25O_7.54 changes in the Cu-apical O two-site distribution reflect a sequential renormalization of the double-well potential of this site beginning at T_c, with the energy difference between the two minima increasing by ~6 meV between T_c and 52 K. Sr₂CuO_3.3 undergoes a radically larger transformation at T_c, >1-Å displacements of the apical O atoms. The principal feature of the dynamical structure underlying these transformations is the strongly anharmonic oscillation of the apical O atoms in a double-well potential that results in the observation of two distinct O sites whose Cu–O distances indicate different bonding modes and valence-charge distributions. The coupling of the superconductivity to the iqtp that originates in this nonadiabatic coupling between the electrons and lattice demonstrates an important role for the dynamical structure whereby pairing occurs even in a system where displacements of the atoms that are part of the transition are sufficiently large to alter the Fermi surface. The synchronization and dynamic coherence of the iqtps resulting from the strong interactions within a crystal would be expected to influence this process.

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Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States). Stanford Synchrotron Radiation Lightsource (SSRL); Stanford Univ., CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); Slovenian Research Agency (ARRS); National Science Foundation (NSF); Ministry of Science and Technology of the People’s Republic of China (MOST); National Natural Science Foundation of China (NSFC)

Grant/Contract Number:: AC02-76SF00515; 1928874

OSTI ID:: 1755491

Journal Information:: Proceedings of the National Academy of Sciences of the United States of America, Vol. 117, Issue 52; ISSN 0027-8424

Publisher:: National Academy of SciencesCopyright Statement

Country of Publication:: United States

Language:: English

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Title: Nonadiabatic coupling of the dynamical structure to the superconductivity in YSr2Cu2.75Mo0.25O7.54 and Sr2CuO3.3

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Title: Nonadiabatic coupling of the dynamical structure to the superconductivity in YSr₂Cu_2.75Mo_0.25O_7.54 and Sr₂CuO_3.3