Helicity-Selective Enhancement and Polarization Control of Attosecond High Harmonic Waveforms Driven by Bichromatic Circularly Polarized Laser Fields

Dorney, Kevin M.; Ellis, Jennifer L.; Hernández-García, Carlos; Hickstein, Daniel D.; Mancuso, Christopher A.; Brooks, Nathan; Fan, Tingting; Fan, Guangyu; Zusin, Dmitriy; Gentry, Christian; Grychtol, Patrik; Kapteyn, Henry C.; Murnane, Margaret M.

doi:10.1103/physrevlett.119.063201

Title: Helicity-Selective Enhancement and Polarization Control of Attosecond High Harmonic Waveforms Driven by Bichromatic Circularly Polarized Laser Fields

Journal Article · Tue Aug 08 00:00:00 EDT 2017 · Physical Review Letters

DOI:https://doi.org/10.1103/physrevlett.119.063201· OSTI ID:1686156

Dorney, Kevin M. ^[1]; Ellis, Jennifer L. ^[1]; Hernández-García, Carlos ^[2]; Hickstein, Daniel D. ^[1]; Mancuso, Christopher A. ^[1]; Brooks, Nathan ^[1]; Fan, Tingting ^[1]; Fan, Guangyu ^[3]; Zusin, Dmitriy ^[1]; Gentry, Christian ^[1]; Grychtol, Patrik ^[1]; Kapteyn, Henry C. ^[1]; Murnane, Margaret M. ^[1]

Univ. of Colorado, Boulder, CO (United States)
Univ. of Salamanca (Spain)
Vienna Univ. of Technology (Austria)

High harmonics driven by two-color counter-rotating circularly-polarized laser fields are a unique source of bright, circularly-polarized, extreme ultraviolet and soft x-ray beams, where the individual harmonics themselves are completely circularly polarized. Here, we demonstrate the ability to preferentially select either the right or left circularly polarized harmonics simply by adjusting the relative intensity ratio of the bichromatic circularly polarized driving laser field. In the frequency domain, this significantly enhances the harmonic orders that rotate in the same direction as the higher intensity driving laser. In the time domain, this helicity-dependent enhancement corresponds to control over the polarization of the resulting attosecond waveforms. Here, this helicity control enables the generation of circularly-polarized high harmonics with a user-defined polarization of the underlying attosecond bursts. In the future, this technique should allow for the production of bright highly elliptical harmonic supercontinua as well as the generation of isolated elliptically polarized attosecond pulses.

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Research Organization:: Univ. of Colorado, Boulder, CO (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: FG02-99ER14982

OSTI ID:: 1686156

Alternate ID(s):: OSTI ID: 1374457

Journal Information:: Physical Review Letters, Vol. 119, Issue 6; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 87 works

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High-order harmonic generation with twisted electrons Gemsheim, Sebastian; Rost, Jan-Michael Physical Review A, Vol. 100, Issue 4 https://doi.org/10.1103/physreva.100.043408	journal	October 2019
Modeling tomographic measurements of photoelectron vortices in counter-rotating circularly polarized laser pulses Armstrong, G. S. J.; Clarke, D. D. A.; Benda, J. Physical Review A, Vol. 100, Issue 6 https://doi.org/10.1103/physreva.100.063416	journal	December 2019
Two-color XUV plus near-IR multiphoton near-threshold ionization of the helium ion by circularly polarized light in the vicinity of the $3 p$ resonance Grum-Grzhimailo, A. N.; Douguet, N.; Meyer, M. Physical Review A, Vol. 100, Issue 3 https://doi.org/10.1103/physreva.100.033404	journal	September 2019
Probing atomic and molecular targets by intense bicircular counter-rotating laser fields Abu-samha, Mahmoud; Madsen, Lars Bojer Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 51, Issue 13 https://doi.org/10.1088/1361-6455/aac631	journal	June 2018
Perspective: Towards single shot time-resolved microscopy using short wavelength table-top light sources Helk, T.; Zürch, M.; Spielmann, C. Structural Dynamics, Vol. 6, Issue 1 https://doi.org/10.1063/1.5082686	journal	January 2019
Controlling the polarization and vortex charge of attosecond high-harmonic beams via simultaneous spin–orbit momentum conservation Dorney, Kevin M.; Rego, Laura; Brooks, Nathan J. Nature Photonics, Vol. 13, Issue 2 https://doi.org/10.1038/s41566-018-0304-3	journal	December 2018
Polarization control of isolated high-harmonic pulses Huang, Pei-Chi; Hernández-García, Carlos; Huang, Jen-Ting Nature Photonics, Vol. 12, Issue 6 https://doi.org/10.1038/s41566-018-0145-0	journal	April 2018
High Harmonic Generation with Twisted Electrons Gemsheim, Sebastian; Rost, Jan-Michael arXiv https://doi.org/10.48550/arxiv.1909.00728	text	January 2019

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