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Title: Study of Quasielastic Barrier Distributions as a Step towards the Synthesis of Superheavy Elements with Hot Fusion Reactions

Journal Article · · Physical Review Letters
ORCiD logo [1];  [2];  [3];  [3];  [3]; ORCiD logo [4]; ORCiD logo [4]; ORCiD logo [4]; ORCiD logo [4];  [5];  [6];  [3];  [7];  [2]; ORCiD logo [4]; ORCiD logo [4]; ORCiD logo [4]; ORCiD logo [3]; ORCiD logo [4];  [8]
  1. RIKEN Nishina Center for Accelerator-Based Science, Saitama (Japan); Kyushu Univ., Fukuoka (Japan); Australian National Univ., Canberra, ACT (Australia)
  2. RIKEN Nishina Center for Accelerator-Based Science, Saitama (Japan); Kyushu Univ., Fukuoka (Japan)
  3. RIKEN Nishina Center for Accelerator-Based Science, Saitama (Japan)
  4. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  5. RIKEN Nishina Center for Accelerator-Based Science, Saitama (Japan); Yamagata Univ. (Japan)
  6. RIKEN Nishina Center for Accelerator-Based Science, Saitama (Japan); Japan Atomic Energy Agency (JAEA), Tokai (Japan). Advanced Science Research Center
  7. Japan Atomic Energy Agency (JAEA), Tokai (Japan). Advanced Science Research Center
  8. Tohoku Univ., Sendai (Japan); Tohoku Univ., Sendai (Japan). Research Center for Electron Photon Science; Kyoto Univ. (Japan)

The excitation functions for quasielastic scattering of Ne 22 + Cm 248 , Mg 26 + Cm 248 , and Ca 48 + U 238 are measured using a gas-filled recoil ion separator. The quasielastic barrier distributions are extracted for these systems and are compared with coupled-channel calculations. The results indicate that the barrier distribution is affected dominantly by deformation of the actinide target nuclei, but also by vibrational or rotational excitations of the projectile nuclei, as well as neutron transfer processes before capture. From a comparison between the experimental barrier distributions and the evaporation residue cross sections for Sg ( Z = 106 ), Hs (108), Cn (112), and Lv (116), it is suggested that the hot fusion reactions take advantage of a compact collision, where the projectile approaches along the short axis of a prolately deformed nucleus. Overall, a new method is proposed to estimate the optimum incident energy to synthesize unknown superheavy nuclei using the barrier distribution.

Research Organization:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Nuclear Physics (NP); Ministry of Education, Culture, Sports, Science and Technology of Japan
Grant/Contract Number:
AC05-00OR22725; 19002005
OSTI ID:
1669769
Journal Information:
Physical Review Letters, Vol. 124, Issue 5; ISSN 0031-9007
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (61)

Production of multi-charged ions in the RIKEN 18 GHz ECRIS journal November 2004
Discovery of Enhanced Nuclear Stability near the Deformed Shells N = 162 and Z = 108 journal August 1994
Synthesis of the isotopes of elements 118 and 116 in the Cf 249 and Cm 245 + Ca 48 fusion reactions journal October 2006
A program for coupled-channel calculations with all order couplings for heavy-ion fusion reactions journal December 1999
Shell structure of superheavy nuclei in self-consistent mean-field models text January 1999
Production cross sections of superheavy elements Z = 119 and 120 in hot fusion reactions journal February 2014
Decay properties of 265 Sg ( Z = 106 ) and 266 Sg ( Z = 106 ) journal April 1998
A program for coupled-channels calculations with all order couplings for heavy-ion fusion reactions text January 1999
Barrier distribution for a ‘superheavy’ nucleus–nucleus collision journal July 2007
Fusion of deformed nuclei in the reactions of 76 Ge + 150 Nd and 28 Si + 198 Pt at the Coulomb barrier region journal May 2000
Synthesis of a New Element with Atomic Number Z = 117 journal April 2010
Synthesis and decay process of superheavy nuclei with Z=119-122 via hot-fusion reactions journal September 2016
Recent developments in heavy-ion fusion reactions journal March 2014
Strength of deep-inelastic scattering for 58Ni+124Sn at sub-barrier energies journal October 1987
Closed shells for Z > 82 and N > 126 in a diffuse potential well journal September 1966
Determination of Fusion Barrier Distributions from Quasielastic Scattering Cross Sections towards Superheavy Nuclei Synthesis journal January 2018
Production of 265 Sg in the 248 Cm( 22 Ne,5 n ) 265 Sg reaction and decay properties of two isomeric states in 265 Sg journal February 2012
The reaction 48Ca + 248Cm → 296116* studied at the GSI-SHIP journal May 2012
How elements up to 118 were reached and how to go beyond journal January 2017
Nuclear ground-state masses and deformations: FRDM(2012) journal May 2016
On the stability of superheavy nuclei against fission journal June 1969
Physico-chemical characterization of seaborgium as oxide hydroxide journal January 2001
Fusion-Fission versus Quasifission: Effect of Nuclear Orientation journal February 1995
Synthesis of superheavy nuclei: A search for new production reactions journal September 2008
Estimating fission-barrier height by the spherical-basis method journal November 2014
Quantum Tunneling in Nuclear Fusion text January 1997
Observation of the 3 n Evaporation Channel in the Complete Hot-Fusion Reaction Mg 26 + Cm 248 Leading to the New Superheavy Nuclide Hs 271 journal April 2008
Status and perspectives of the Dubna superheavy element factory journal January 2016
Reduced electric-octupole transition probabilities, B(E3;01+ → 31−), for even-even nuclides throughout the periodic table journal May 1989
On the search for elements beyond Z =118. An outlook based on lessons from the heaviest known elements journal January 2016
Production and decay of the isotope 271 Ds (Z = 110) journal August 2004
Measurements of cross sections and decay properties of the isotopes of elements 112, 114, and 116 produced in the fusion reactions U 233 , 238 , Pu 242 , and Cm 248 + Ca 48 journal December 2004
Quantum tunneling in nuclear fusion journal January 1998
Large-angle scattering and quasielastic barrier distributions journal May 2004
The reaction 48Ca + 238U → 286112* studied at the GSI-SHIP journal June 2007
Experiments on the synthesis of element 115 in the reaction Am 243 ( Ca 48 , x n ) 115 291 x journal February 2004
Subbarrier fusion reactions and many-particle quantum tunneling text January 2012
Time-dependent Hartree-Fock plus Langevin approach for hot fusion reactions to synthesize the Z = 120 superheavy element journal May 2019
Estimation for Synthesis of Superheavy Elements
  • Aritomo, Yoshihiro; Liyana, Nur; Tanaka, Shoya
  • Proceedings of the Ito International Research Center Symposium "Perspectives of the Physics of Nuclear Structure" https://doi.org/10.7566/JPSCP.23.013001
conference December 2018
Variable frequency heavy-ion linac, RILAC
  • Odera, Masatoshi; Chiba, Yoshiaki; Tonuma, Tadao
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 227, Issue 2 https://doi.org/10.1016/0168-9002(84)90121-9
journal November 1984
Isotopic dependence of fusion cross sections in reactions with heavy nuclei text January 1999
Subbarrier Fusion Reactions and Many-Particle Quantum Tunneling journal December 2012
Probing fusion barrier distributions with quasi-elastic scattering journal February 1995
Measurements of cross sections for the fusion-evaporation reactions Pu 244 ( Ca 48 , x n ) 292 x 114 and Cm 245 ( Ca 48 , x n ) 293 x 116 journal May 2004
Estimates of production and structure of nuclei with Z= 119 journal February 2018
Barrier Distributions Derived from Quasielastic Backscattering of Ti 48 , Cr 54 , Fe 56 , Ni 64 , and Zn 70 Projectiles on a Pb 208 Target journal November 2007
Measuring Barriers to Fusion journal December 1998
Hot fusion reactions with deformed nuclei for synthesis of superheavy nuclei: An extension of the fusion-by-diffusion model journal July 2018
On the “distribution of barriers” interpretation of heavy-ion fusion journal January 1991
Review of even element super-heavy nuclei and search for element 120 journal June 2016
Nuclear masses and deformations journal June 1966
Barrier distributions from the fusion of oxygen ions with Sm 1 4 4 , 1 4 8 , 1 5 4 and W 186 journal December 1995
Severe Inhibition of Fusion by Quasifission in Reactions Forming T 220 h journal December 2002
Isotopic dependence of fusion cross sections in reactions with heavy nuclei journal September 2000
Fission and quasifission toward the superheavy mass region journal August 2019
Fission and Quasifission Toward the Superheavy Mass Region conference December 2019
Shell structure of superheavy nuclei in self-consistent mean-field models journal August 1999
Transition Probability from the Ground to the First-Excited 2+ State of Even–Even Nuclides journal May 2001
RIKEN isotope separator on-line GARIS/IGISOL journal August 1992
Note: Effect of hot liner in producing 40,48 Ca beam from RIKEN 18-GHz electron cyclotron resonance ion source journal January 2015
Inverse quasifission in the reactions Gd 156 , 160 + W 186 journal December 2017