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Title: Scale-Up of Advanced Hot-Gas Desulfurization Sorbents

Technical Report ·
DOI:https://doi.org/10.2172/16008· OSTI ID:16008

The overall objective of this project is to develop regenerable sorbents for hot gas desulfurization in IGCC systems. The specific objective of the project is to develop durable advanced sorbents that demonstrate a strong resistance to attrition and chemical deactivation, and high activity at temperatures as low as 343 C (650 F). A number of formulations will be prepared and screened in a 1/2-inch fixed bed reactor at high pressure (1 to 20 atm) and high temperatures using simulated coal-derived fuel-gases. Screening criteria will include, chemical reactivity, stability, and regenerability over the temperature range of 343 C to 650 C. After initial screening, at least 3 promising formulations will be tested for 25-30 cycles of absorption and regeneration. One of the superior formulations with the best cyclic performance will be selected for investigating scale up parameters. The scaled-up formulation will be tested for long term durability and chemical reactivity.

Research Organization:
National Energy Technology Lab., Pittsburgh, PA, and Morgantown, WV (US)
Sponsoring Organization:
US Department of Energy (US)
DOE Contract Number:
FG22-95MT95011
OSTI ID:
16008
Report Number(s):
DOE/MT/95011-T; ON: DE97051097; TRN: US200511%%160
Resource Relation:
Other Information: Supercedes report DE00016008; Supercedes report DE97051097; PBD: 14 Oct 1996; PBD: 14 Oct 1996
Country of Publication:
United States
Language:
English