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Title: Increasing the detection sensitivity of the Radionuclide Aerosol Sampler/Analyzer using a cosmic veto system

Journal Article · · Nuclear Instruments and Methods in Physics Research. Section A, Accelerators, Spectrometers, Detectors and Associated Equipment

Different configurations of a cosmic veto system have been evaluated for the Radionuclide Aerosol Sampler/Analyzer (RASA). The upgrade has the potential to resolve the issue that U.S. IMS radionuclide stations have difficulty meeting the 140Ba Minimum Detectable Concentration (MDC) certification requirement when the natural background radioactivity is high. It also aims to improve the detection sensitivity of the RASA system for other fission and activation products indicative of a nuclear explosion. This proof of principal utilizes a prototype RASA system located at Pacific Northwest National Laboratory (PNNL), and has demonstrated background reductions by up to 11.3% and improvements in the average MDC by up to 7.7%. Recommendations are made for either a 1 or 3 plate configuration, which improves the 140Ba MDC by 5.6% and 7.2% for a blank filter. Whilst elevated 212Pb activity remains problematic, the cosmic veto system provides a practical solution for sensitivity improvement with little design modification of the RASA. It also has value in improving sensitivity and preventing false-positives at remote U.S. IMS station locations where sample transfer for laboratory analysis is logistically difficult.

Research Organization:
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
AC05-76RL01830
OSTI ID:
1559279
Report Number(s):
PNNL-SA-140402
Journal Information:
Nuclear Instruments and Methods in Physics Research. Section A, Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 944
Country of Publication:
United States
Language:
English

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