A Highly Stretchable and Fatigue-Free Transparent Electrode Based on an In-Plane Buckled Au Nanotrough Network

Huang, Siya; Liu, Yuan; Guo, Chuan Fei; Ren, Zhifeng

doi:10.1002/aelm.201600534

Title: A Highly Stretchable and Fatigue-Free Transparent Electrode Based on an In-Plane Buckled Au Nanotrough Network

Journal Article · Mon Feb 20 00:00:00 EST 2017 · Advanced Electronic Materials

DOI:https://doi.org/10.1002/aelm.201600534· OSTI ID:1533057

Huang, Siya ^[1]; Liu, Yuan ^[1]; Guo, Chuan Fei ^[2]; Ren, Zhifeng ^[1]

Univ. of Houston, TX (United States)
Southern Univ. of Science & Technology (China)

Flexible transparent electrodes are an indispensable component of next-generation soft optoelectronics such as wearable electronics and electronic artificial skins (E-skins). Among the existing candidate materials, metal nanotrough networks exhibit optimal overall optoelectronic performance with impressive bendability. However, their further practical applications are hindered by their limited mechanical stretchability, which is highly desired in biointegrated systems. Here it is demonstrated that superior mechanical stretchability with tensile strains up to 300% can be achieved in Au nanotrough networks by introducing an in-plane sinusoidal wavy structure. For the first time it is shown that with a precisely tuned nanotrough geometry along with an optimized network configuration, the buckled Au nanotrough network can be repeatedly stretched to strains up to 120% for 100 000 cycles, exhibiting excellent fatigue performance. Such highly stretchable and fatigue-free (at a high tensile strain up to 100%) Au nanotrough networks present a competent sheet resistance (R_sh ≈ 10 Ω sq^-1) with high optical transparency (T = 91%), which are demonstrated to be highly compatible with human skins as conformal flexible transparent electrodes.

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Research Organization:: Univ. of Houston, TX (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: SC0010831; K16251101; Y01256120

OSTI ID:: 1533057

Alternate ID(s):: OSTI ID: 1401053

Journal Information:: Advanced Electronic Materials, Vol. 3, Issue 3; ISSN 2199-160X

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 33 works

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References (34)

Deformation-induced cold-welding for self-healing of super-durable flexible transparent electrodes Guo, Chuan Fei; Lan, Yucheng; Sun, Tianyi Nano Energy, Vol. 8 https://doi.org/10.1016/j.nanoen.2014.05.011	journal	September 2014
Highly Stretchable or Transparent Conductor Fabrication by a Hierarchical Multiscale Hybrid Nanocomposite Lee, Phillip; Ham, Jooyeun; Lee, Jinhwan Advanced Functional Materials, Vol. 24, Issue 36 https://doi.org/10.1002/adfm.201400972	journal	July 2014
Improvement of Transparent Metal Top Electrodes for Organic Solar Cells by Introducing a High Surface Energy Seed Layer Schubert, Sylvio; Meiss, Jan; Müller-Meskamp, Lars Advanced Energy Materials, Vol. 3, Issue 4 https://doi.org/10.1002/aenm.201200903	journal	January 2013
The Growth Mechanism of Copper Nanowires and Their Properties in Flexible, Transparent Conducting Films Rathmell, Aaron R.; Bergin, Stephen M.; Hua, Yi-Lei Advanced Materials, Vol. 22, Issue 32 https://doi.org/10.1002/adma.201000775	journal	June 2010
Dissolvable films of silk fibroin for ultrathin conformal bio-integrated electronics Kim, Dae-Hyeong; Viventi, Jonathan; Amsden, Jason J. Nature Materials, Vol. 9, Issue 6, p. 511-517 https://doi.org/10.1038/nmat2745	journal	April 2010
Fatigue-free, superstretchable, transparent, and biocompatible metal electrodes Guo, Chuan Fei; Liu, Qihan; Wang, Guohui Proceedings of the National Academy of Sciences, Vol. 112, Issue 40 https://doi.org/10.1073/pnas.1516873112	journal	September 2015
Spontaneous formation of ordered structures in thin films of metals supported on an elastomeric polymer Whitesides, George M.; Bowden, Ned; Brittain, Scott Nature, Vol. 393, Issue 6681, p. 146-149 https://doi.org/10.1038/30193	journal	May 1998
Skin-like pressure and strain sensors based on transparent elastic films of carbon nanotubes Lipomi, Darren J.; Vosgueritchian, Michael; Tee, Benjamin C-K. Nature Nanotechnology, Vol. 6, Issue 12, p. 788-792 https://doi.org/10.1038/nnano.2011.184	journal	October 2011
Transparent Ultrathin Oxygen-Doped Silver Electrodes for Flexible Organic Solar Cells Wang, Wei; Song, Myungkwan; Bae, Tae-Sung Advanced Functional Materials, Vol. 24, Issue 11 https://doi.org/10.1002/adfm.201301359	journal	November 2013
Epidermal Electronics Kim, D.-H.; Lu, N.; Ma, R. Science, Vol. 333, Issue 6044, p. 838-843 https://doi.org/10.1126/science.1206157	journal	August 2011
Room-Temperature Nanosoldering of a Very Long Metal Nanowire Network by Conducting-Polymer-Assisted Joining for a Flexible Touch-Panel Application Lee, Jinhwan; Lee, Phillip; Lee, Ha Beom Advanced Functional Materials, Vol. 23, Issue 34 https://doi.org/10.1002/adfm.201203802	journal	April 2013
Molecular Scale Buckling Mechanics in Individual Aligned Single-Wall Carbon Nanotubes on Elastomeric Substrates Khang, Dahl-Young; Xiao, Jianliang; Kocabas, Coskun Nano Letters, Vol. 8, Issue 1 https://doi.org/10.1021/nl072203s	journal	January 2008
Highly stretchable and transparent nanomesh electrodes made by grain boundary lithography Guo, Chuan Fei; Sun, Tianyi; Liu, Qihan Nature Communications, Vol. 5, Issue 1 https://doi.org/10.1038/ncomms4121	journal	January 2014
Emerging Transparent Electrodes Based on Thin Films of Carbon Nanotubes, Graphene, and Metallic Nanostructures Hecht, David S.; Hu, Liangbing; Irvin, Glen Advanced Materials, Vol. 23, Issue 13, p. 1482-1513 https://doi.org/10.1002/adma.201003188	journal	February 2011
Efficient and Flexible ITO-Free Organic Solar Cells Using Highly Conductive Polymer Anodes Na, Seok-In; Kim, Seok-Soon; Jo, Jang Advanced Materials, Vol. 20, Issue 21 https://doi.org/10.1002/adma.200800338	journal	November 2008
Buckled Au@PVP Nanofiber Networks for Highly Transparent and Stretchable Conductors Jin, Yusung; Hwang, Sunju; Ha, Hyunchul Advanced Electronic Materials, Vol. 2, Issue 2 https://doi.org/10.1002/aelm.201500302	journal	January 2016
Stretching our imagination LeMieux, Melburne C.; Bao, Zhenan Nature Nanotechnology, Vol. 3, Issue 10 https://doi.org/10.1038/nnano.2008.296	journal	October 2008
Silver Nanowire Networks as Flexible, Transparent, Conducting Films: Extremely High DC to Optical Conductivity Ratios De, Sukanta; Higgins, Thomas M.; Lyons, Philip E. ACS Nano, Vol. 3, Issue 7 https://doi.org/10.1021/nn900348c	journal	June 2009
Mechanical properties of ultrahigh-strength gold nanowires Wu, Bin; Heidelberg, Andreas; Boland, John J. Nature Materials, Vol. 4, Issue 7 https://doi.org/10.1038/nmat1403	journal	June 2005
Silver Nanowire Percolation Network Soldered with Graphene Oxide at Room Temperature and Its Application for Fully Stretchable Polymer Light-Emitting Diodes Liang, Jiajie; Li, Lu; Tong, Kwing ACS Nano, Vol. 8, Issue 2 https://doi.org/10.1021/nn405887k	journal	January 2014
Highly Conductive and Transparent PEDOT:PSS Films with a Fluorosurfactant for Stretchable and Flexible Transparent Electrodes Vosgueritchian, Michael; Lipomi, Darren J.; Bao, Zhenan Advanced Functional Materials, Vol. 22, Issue 2 https://doi.org/10.1002/adfm.201101775	journal	November 2011
Large-scale pattern growth of graphene films for stretchable transparent electrodes Kim, Keun Soo; Zhao, Yue; Jang, Houk Nature, Vol. 457, Issue 7230 https://doi.org/10.1038/nature07719	journal	January 2009
Highly Stretchable and Highly Conductive Metal Electrode by Very Long Metal Nanowire Percolation Network Lee, Phillip; Lee, Jinhwan; Lee, Hyungman Advanced Materials, Vol. 24, Issue 25, p. 3326-3332 https://doi.org/10.1002/adma.201200359	journal	May 2012
Avoiding indium Inganäs, Olle Nature Photonics, Vol. 5, Issue 4 https://doi.org/10.1038/nphoton.2011.46	journal	March 2011
Transparent, Conductive Carbon Nanotube Films Wu, Zhuangchun; Chen, Zhihong; Du, Xu Science, Vol. 305, Issue 5688, p. 1273-1276 https://doi.org/10.1126/science.1101243	journal	August 2004
Transparent, Conductive, and Flexible Carbon Nanotube Films and Their Application in Organic Light-Emitting Diodes Zhang, Daihua; Ryu, Koungmin; Liu, Xiaolei Nano Letters, Vol. 6, Issue 9, p. 1880-1886 https://doi.org/10.1021/nl0608543	journal	September 2006
Lateral Buckling Mechanics in Silicon Nanowires on Elastomeric Substrates Ryu, Seung Yoon; Xiao, Jianliang; Park, Won Il Nano Letters, Vol. 9, Issue 9 https://doi.org/10.1021/nl901450q	journal	September 2009
Highly Efficient and Bendable Organic Solar Cells with Solution-Processed Silver Nanowire Electrodes Song, Myungkwan; You, Dae Sung; Lim, Kyounga Advanced Functional Materials, Vol. 23, Issue 34 https://doi.org/10.1002/adfm.201202646	journal	April 2013
Stretchable and Transparent Electrodes using Hybrid Structures of Graphene–Metal Nanotrough Networks with High Performances and Ultimate Uniformity An, Byeong Wan; Hyun, Byung Gwan; Kim, So-Yun Nano Letters, Vol. 14, Issue 11 https://doi.org/10.1021/nl502755y	journal	October 2014
Flexible, Stretchable, Transparent Conducting Films Made from Superaligned Carbon Nanotubes Feng, Chen; Liu, Kai; Wu, Jeah-Sheng Advanced Functional Materials, Vol. 20, Issue 6 https://doi.org/10.1002/adfm.200901960	journal	February 2010
Roll-to-roll production of 30-inch graphene films for transparent electrodes Bae, Sukang; Kim, Hyeongkeun; Lee, Youngbin Nature Nanotechnology, Vol. 5, Issue 8, p. 574-578 https://doi.org/10.1038/nnano.2010.132	journal	June 2010
Transfer of Large-Area Graphene Films for High-Performance Transparent Conductive Electrodes Li, Xuesong; Zhu, Yanwu; Cai, Weiwei Nano Letters, Vol. 9, Issue 12 https://doi.org/10.1021/nl902623y	journal	December 2009
A transparent electrode based on a metal nanotrough network Wu, Hui; Kong, Desheng; Ruan, Zhichao Nature Nanotechnology, Vol. 8, Issue 6 https://doi.org/10.1038/nnano.2013.84	journal	May 2013
Synthesis of Ultralong Copper Nanowires for High-Performance Transparent Electrodes Zhang, Dieqing; Wang, Ranran; Wen, Meicheng Journal of the American Chemical Society, Vol. 134, Issue 35 https://doi.org/10.1021/ja3050184	journal	August 2012

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Deformable and Transparent Ionic and Electronic Conductors for Soft Energy Devices Park, Sangbaek; Parida, Kaushik; Lee, Pooi See Advanced Energy Materials, Vol. 7, Issue 22 https://doi.org/10.1002/aenm.201701369	journal	September 2017
Emerging Novel Metal Electrodes for Photovoltaic Applications Lu, Haifei; Ren, Xingang; Ouyang, Dan Small, Vol. 14, Issue 14 https://doi.org/10.1002/smll.201703140	journal	January 2018
Buckled Structures: Fabrication and Applications in Wearable Electronics Hu, Xiaoyu; Dou, Yuanyuan; Li, Jingjing Small, Vol. 15, Issue 32 https://doi.org/10.1002/smll.201804805	journal	February 2019
Deformable and Stretchable Electrodes for Soft Electronic Devices Kim, Yonghee; Kweon, O. Young; Won, Yousang Macromolecular Research, Vol. 27, Issue 7 https://doi.org/10.1007/s13233-019-7175-4	journal	July 2019
Digitally printed stretchable electronics: a review Fernandes, Daniel Félix; Majidi, Carmel; Tavakoli, Mahmoud Journal of Materials Chemistry C, Vol. 7, Issue 45 https://doi.org/10.1039/c9tc04246f	journal	January 2019

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Title: A Highly Stretchable and Fatigue-Free Transparent Electrode Based on an In-Plane Buckled Au Nanotrough Network

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