Localized Control of Curie Temperature in Perovskite Oxide Film by Capping-Layer-Induced Octahedral Distortion

Thomas, S.; Kuiper, B.; Hu, J.; Smit, J.; Liao, Z.; Zhong, Z.; Rijnders, G.; Vailionis, A.; Wu, R.; Koster, G.; Xia, J.

doi:10.1103/PhysRevLett.119.177203

Title: Localized Control of Curie Temperature in Perovskite Oxide Film by Capping-Layer-Induced Octahedral Distortion

Journal Article · Fri Oct 27 00:00:00 EDT 2017 · Physical Review Letters

DOI:https://doi.org/10.1103/PhysRevLett.119.177203· OSTI ID:1410802

Thomas, S. ^[1]; Kuiper, B. ^[2]; Hu, J. ^[3]; Smit, J. ^[4]; Liao, Z. ^[2]; Zhong, Z. ^[5]; Rijnders, G. ^[2]; Vailionis, A. ^[4]; Wu, R. ^[1]; Koster, G. ^[2]; Xia, J. ^[1]

Univ. of California, Irvine, CA (United States). Dept. of Physics and Astronomy
Univ. of Twente, Enschede (Netherlands). MESA+ Inst. for Nanotechnology
Univ. of California, Irvine, CA (United States). Dept. of Physics and Astronomy; Soochow Univ., Suzhou, Jiangsu (China). College of Physics, Optoelectronics and Energy
Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials
Chinese Academy of Sciences (CAS), Ningbo (China). Key Lab. of Magnetic Materials and Devices & Zhejiang Province Key Lab. of Magnetic Materials and Application Technology, Ningbo Inst. of Materials Technology and Engineering

With reduced dimensionality, it is often easier to modify the properties of ultrathin films than their bulk counterparts. Strain engineering, usually achieved by choosing appropriate substrates, has been proven effective in controlling the properties of perovskite oxide films. An emerging alternative route for developing new multifunctional perovskite is by modification of the oxygen octahedral structure. Here we report the control of structural oxygen octahedral rotation in ultrathin perovskite SrRuO₃ films by the deposition of a SrTiO₃ capping layer, which can be lithographically patterned to achieve local control. Here, using a scanning Sagnac magnetic microscope, we show an increase in the Curie temperature of SrRuO₃ due to the suppression octahedral rotations revealed by the synchrotron x-ray diffraction. Lastly, this capping-layer-based technique may open new possibilities for developing functional oxide materials.

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Research Organization:: SLAC National Accelerator Lab., Menlo Park, CA (United States)

Sponsoring Organization:: USDOE; National Science Foundation (NSF)

Grant/Contract Number:: DMR-1350122; ECCS-1542152; FG02-05ER46237; AC02-76SF00515

OSTI ID:: 1410802

Alternate ID(s):: OSTI ID: 1405207

Journal Information:: Physical Review Letters, Vol. 119, Issue 17; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 24 works

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Interface Engineered Room‐Temperature Ferromagnetic Insulating State in Ultrathin Manganite Films Li, Weiwei; Zhu, Bonan; He, Qian Advanced Science, Vol. 7, Issue 1 https://doi.org/10.1002/advs.201901606	journal	November 2019
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Interface Engineered Room-Temperature Ferromagnetic Insulating State in Ultrathin Manganite Films. Li, Weiwei; Zhu, Bonan; He, Qian Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.45761	text	January 2020
Interface Engineered Room-Temperature Ferromagnetic Insulating State in Ultrathin Manganite Films. Li, Weiwei; Zhu, Bonan; He, Qian Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.49048	text	January 2019

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