Highly Textured BaTiO 3 via Templated Grain Growth and Resulting Polarization Reversal Dynamics

Meier, William; Meyer, Kelsey Elizabeth; Sava Gallis, Dorina F.; Blea‐Kirby, Mia Angelica; Roth, Joshua; Felman, Daniel; Breuer, Tim; Dension, Gary J.; Zutavern, Fred J.; Huebner, Wayne; Brennecka, Geoff L.; Jones, ed., J.

doi:10.1111/jace.14048

Title: Highly Textured BaTiO ₃ via Templated Grain Growth and Resulting Polarization Reversal Dynamics

Journal Article · Sun Dec 13 00:00:00 EST 2015 · Journal of the American Ceramic Society

DOI:https://doi.org/10.1111/jace.14048· OSTI ID:1400530

Meier, William ^[1]; Meyer, Kelsey Elizabeth ^[2]; Sava Gallis, Dorina F. ^[3]; Blea‐Kirby, Mia Angelica ^[3]; Roth, Joshua ^[4]; Felman, Daniel ^[5]; Breuer, Tim ^[6]; Dension, Gary J. ^[3]; Zutavern, Fred J. ^[3]; Huebner, Wayne ^[7];

^[8]; Jones, ed., J.

Department of Physics &, Astronomy Iowa State University Ames Iowa 50011
Department of Mechanical and Aerospace Engineering University of Virginia Charlottesville Virginia 22904
Sandia National Laboratories Albuquerque New Mexico 87185
Department of Materials Science and Engineering Iowa State University Ames Iowa 50011
Department of Mechanical, Industrial, and Manufacturing Engineering Oregon State University Corvallis Oregon 97331
EaglePicher Technologies Joplin Missouri 64802
Department of Materials Science and Engineering Missouri S&,T Rolla Missouri 65409
Department of Metallurgical and Materials Engineering Colorado School of Mines Golden Colorado 80401

Samples of bulk textured polycrystalline BaTiO ₃ ceramics were fabricated using a templated grain growth ( TGG ) approach in order to investigate effects of polycrystallinity and texture related to ferroelectric domain reversal under high‐power drive conditions. Barium titanate platelets were formed via two‐step topochemical conversion of bismuth titanate platelets grown via molten salt synthesis, then aligned via tape casting within a matrix of fine BaTiO ₃ powder. The coarse‐grained parts showed a high degree of crystallographic texture after sintering. Combined with ceramics of similar density and polycrystallinity, but random orientation and commercial single‐crystal specimens, this sample set enabled direct isolation of crystallographic texture and polycrystallinity as the primary variables for high‐power polarization reversal studies. These studies have also demonstrated a link between grain size and polarization reversal time that strongly suggests that grain boundaries serve effectively as nucleation sites during the ferroelectric switching process.

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Sponsoring Organization:: USDOE

OSTI ID:: 1400530

Journal Information:: Journal of the American Ceramic Society, Journal Name: Journal of the American Ceramic Society Vol. 99 Journal Issue: 3; ISSN 0002-7820

Publisher:: Wiley-BlackwellCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 13 works

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References (41)

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