Measurement of the optical dielectric function of monolayer transition-metal dichalcogenides: MoS2 , MoSe2 , WS2 , and WSe2

Li, Yilei; Chernikov, Alexey; Zhang, Xian; Rigosi, Albert; Hill, Heather M.; van der Zande, Arend M.; Chenet, Daniel A.; Shih, En-Min; Hone, James; Heinz, Tony F.

doi:10.1103/PhysRevB.90.205422

Title: Measurement of the optical dielectric function of monolayer transition-metal dichalcogenides: ${MoS}_{2}$ , $Mo S e_{2}$ , ${WS}_{2}$ , and $WS e_{2}$

Journal Article · Sat Nov 01 00:00:00 EDT 2014 · Physical Review. B, Condensed Matter and Materials Physics

DOI:https://doi.org/10.1103/PhysRevB.90.205422· OSTI ID:1370378

Li, Yilei; Chernikov, Alexey; Zhang, Xian; Rigosi, Albert; Hill, Heather M.; van der Zande, Arend M.; Chenet, Daniel A.; Shih, En-Min; Hone, James; Heinz, Tony F.

Cite

Export

Save

Research Organization:: Energy Frontier Research Centers (EFRC) (United States). Re-Defining Photovoltaic Efficiency Through Molecule Scale Control (RPEMSC)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

DOE Contract Number:: SC0001085

OSTI ID:: 1370378

Journal Information:: Physical Review. B, Condensed Matter and Materials Physics, Vol. 90, Issue 20; Related Information: RPEMSC partners with Columbia University (lead); Brookhaven National Laboratory; Purdue University; ISSN 1098-0121

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

References (50)

Coupled Spin and Valley Physics in Monolayers of ${MoS}_{2}$ and Other Group-VI Dichalcogenides Xiao, Di; Liu, Gui-Bin; Feng, Wanxiang Physical Review Letters, Vol. 108, Issue 19 https://doi.org/10.1103/PhysRevLett.108.196802	journal	May 2012
Photodetectors based on graphene, other two-dimensional materials and hybrid systems Koppens, F. H. L.; Mueller, T.; Avouris, Ph. Nature Nanotechnology, Vol. 9, Issue 10 https://doi.org/10.1038/nnano.2014.215	journal	October 2014
Tuning Many-Body Interactions in Graphene: The Effects of Doping on Excitons and Carrier Lifetimes Mak, Kin Fai; da Jornada, Felipe H.; He, Keliang Physical Review Letters, Vol. 112, Issue 20 https://doi.org/10.1103/PhysRevLett.112.207401	journal	May 2014
Mono- and Bilayer WS ₂ Light-Emitting Transistors Jo, Sanghyun; Ubrig, Nicolas; Berger, Helmuth Nano Letters, Vol. 14, Issue 4 https://doi.org/10.1021/nl500171v	journal	March 2014
Large-Area Vapor-Phase Growth and Characterization of MoS₂ Atomic Layers on a SiO₂ Substrate Zhan, Yongjie; Liu, Zheng; Najmaei, Sina Small, Vol. 8, Issue 7, p. 966-971 https://doi.org/10.1002/smll.201102654	journal	February 2012
Optical Properties and Band Gap of Single- and Few-Layer MoTe ₂ Crystals Ruppert, Claudia; Aslan, Ozgur Burak; Heinz, Tony F. Nano Letters, Vol. 14, Issue 11 https://doi.org/10.1021/nl502557g	journal	October 2014
Progress, Challenges, and Opportunities in Two-Dimensional Materials Beyond Graphene Butler, Sheneve Z.; Hollen, Shawna M.; Cao, Linyou ACS Nano, Vol. 7, Issue 4, p. 2898-2926 https://doi.org/10.1021/nn400280c	journal	March 2013
Emerging Photoluminescence in Monolayer MoS₂ Splendiani, Andrea; Sun, Liang; Zhang, Yuanbo Nano Letters, Vol. 10, Issue 4, p. 1271-1275 https://doi.org/10.1021/nl903868w	journal	April 2010
Spin and pseudospins in layered transition metal dichalcogenides Xu, Xiaodong; Yao, Wang; Xiao, Di Nature Physics, Vol. 10, Issue 5 https://doi.org/10.1038/nphys2942	journal	April 2014
Charge Dynamics and Electronic Structures of Monolayer MoS ₂ Films Grown by Chemical Vapor Deposition Shen, Chih-Chiang; Hsu, Yu-Te; Li, Lain-Jong Applied Physics Express, Vol. 6, Issue 12 https://doi.org/10.7567/APEX.6.125801	journal	December 2013
Growth of Large-Area and Highly Crystalline MoS₂ Thin Layers on Insulating Substrates Liu, Keng-Ku; Zhang, Wenjing; Lee, Yi-Hsien Nano Letters, Vol. 12, Issue 3, p. 1538-1544 https://doi.org/10.1021/nl2043612	journal	February 2012
Synthesis and Optical Properties of Large-Area Single-Crystalline 2D Semiconductor WS ₂ Monolayer from Chemical Vapor Deposition Cong, Chunxiao; Shang, Jingzhi; Wu, Xing Advanced Optical Materials, Vol. 2, Issue 2 https://doi.org/10.1002/adom.201300428	journal	December 2013
Three-band tight-binding model for monolayers of group-VIB transition metal dichalcogenides Liu, Gui-Bin; Shan, Wen-Yu; Yao, Yugui Physical Review B, Vol. 88, Issue 8 https://doi.org/10.1103/PhysRevB.88.085433	journal	August 2013
Giant spin-orbit-induced spin splitting in two-dimensional transition-metal dichalcogenide semiconductors Zhu, Z. Y.; Cheng, Y. C.; Schwingenschlögl, U. Physical Review B, Vol. 84, Issue 15 https://doi.org/10.1103/PhysRevB.84.153402	journal	October 2011
Investigation of the optical properties of MoS ₂ thin films using spectroscopic ellipsometry Yim, Chanyoung; O'Brien, Maria; McEvoy, Niall Applied Physics Letters, Vol. 104, Issue 10 https://doi.org/10.1063/1.4868108	journal	March 2014
Optical Spectrum of ${MoS}_{2}$ : Many-Body Effects and Diversity of Exciton States Qiu, Diana Y.; da Jornada, Felipe H.; Louie, Steven G. Physical Review Letters, Vol. 111, Issue 21 https://doi.org/10.1103/PhysRevLett.111.216805	journal	November 2013
Probing excitonic dark states in single-layer tungsten disulphide Ye, Ziliang; Cao, Ting; O’Brien, Kevin Nature, Vol. 513, Issue 7517 https://doi.org/10.1038/nature13734	journal	August 2014
Atomically Thin ${MoS}_{2}$ A New Direct-Gap Semiconductor Mak, Kin Fai; Lee, Changgu; Hone, James Physical Review Letters, Vol. 105, Issue 13, Article No.136805 https://doi.org/10.1103/PhysRevLett.105.136805	journal	September 2010
Synthesis of Large-Area MoS₂ Atomic Layers with Chemical Vapor Deposition Lee, Yi-Hsien; Zhang, Xin-Quan; Zhang, Wenjing Advanced Materials, Vol. 24, Issue 17, p. 2320-2325 https://doi.org/10.1002/adma.201104798	journal	March 2012
Valley-selective circular dichroism of monolayer molybdenum disulphide Cao, Ting; Wang, Gang; Han, Wenpeng Nature Communications, Vol. 3, Issue 1 https://doi.org/10.1038/ncomms1882	journal	January 2012
Electrical control of neutral and charged excitons in a monolayer semiconductor Ross, Jason S.; Wu, Sanfeng; Yu, Hongyi Nature Communications, Vol. 4, Issue 1 https://doi.org/10.1038/ncomms2498	journal	February 2013
Solar-energy conversion and light emission in an atomic monolayer p–n diode Pospischil, Andreas; Furchi, Marco M.; Mueller, Thomas Nature Nanotechnology, Vol. 9, Issue 4 https://doi.org/10.1038/nnano.2014.14	journal	March 2014
Band nesting and the optical response of two-dimensional semiconducting transition metal dichalcogenides Carvalho, A.; Ribeiro, R. M.; Castro Neto, A. H. Physical Review B, Vol. 88, Issue 11 https://doi.org/10.1103/PhysRevB.88.115205	journal	September 2013
Seeing Many-Body Effects in Single- and Few-Layer Graphene: Observation of Two-Dimensional Saddle-Point Excitons Mak, Kin Fai; Shan, Jie; Heinz, Tony F. Physical Review Letters, Vol. 106, Issue 4 https://doi.org/10.1103/PhysRevLett.106.046401	journal	January 2011
Atomically thin p–n junctions with van der Waals heterointerfaces Lee, Chul-Ho; Lee, Gwan-Hyoung; van der Zande, Arend M. Nature Nanotechnology, Vol. 9, Issue 9 https://doi.org/10.1038/nnano.2014.150	journal	August 2014
Giant bandgap renormalization and excitonic effects in a monolayer transition metal dichalcogenide semiconductor Ugeda, Miguel M.; Bradley, Aaron J.; Shi, Su-Fei Nature Materials, Vol. 13, Issue 12 https://doi.org/10.1038/nmat4061	journal	August 2014
Infrared-Reflectance Spectra of Layered Group-IV and Group-VI Transition-Metal Dichalcogenides Lucovsky, G.; White, R. M.; Benda, J. A. Physical Review B, Vol. 7, Issue 8 https://doi.org/10.1103/PhysRevB.7.3859	journal	April 1973
Electronic structure of ${MoSe}_{2}$ , ${MoS}_{2}$ , and ${WSe}_{2}$ . II. The nature of the optical band gaps Coehoorn, R.; Haas, C.; de Groot, R. A. Physical Review B, Vol. 35, Issue 12 https://doi.org/10.1103/PhysRevB.35.6203	journal	April 1987
Grains and grain boundaries in highly crystalline monolayer molybdenum disulphide van der Zande, Arend M.; Huang, Pinshane Y.; Chenet, Daniel A. Nature Materials, Vol. 12, Issue 6, p. 554-561 https://doi.org/10.1038/nmat3633	journal	May 2013
Large-Area Synthesis of Monolayer and Few-Layer MoSe ₂ Films on SiO ₂ Substrates Lu, Xin; Utama, M. Iqbal Bakti; Lin, Junhao Nano Letters, Vol. 14, Issue 5 https://doi.org/10.1021/nl5000906	journal	April 2014
Tightly Bound Excitons in Monolayer ${WSe}_{2}$ He, Keliang; Kumar, Nardeep; Zhao, Liang Physical Review Letters, Vol. 113, Issue 2 https://doi.org/10.1103/PhysRevLett.113.026803	journal	July 2014
Electrically tunable excitonic light-emitting diodes based on monolayer WSe2 p–n junctions Ross, Jason S.; Klement, Philip; Jones, Aaron M. Nature Nanotechnology, Vol. 9, Issue 4 https://doi.org/10.1038/nnano.2014.26	journal	March 2014
Strong Light-Matter Interactions in Heterostructures of Atomically Thin Films Britnell, L.; Ribeiro, R. M.; Eckmann, A. Science, Vol. 340, Issue 6138 https://doi.org/10.1126/science.1235547	journal	May 2013
Origin of Indirect Optical Transitions in Few-Layer MoS ₂ , WS ₂ , and WSe ₂ Zhao, Weijie; Ribeiro, R. M.; Toh, Minglin Nano Letters, Vol. 13, Issue 11 https://doi.org/10.1021/nl403270k	journal	October 2013
Infrared and Raman Studies of Long-Wavelength Optical Phonons in Hexagonal Mo $S_{2}$ Wieting, T. J.; Verble, J. L. Physical Review B, Vol. 3, Issue 12 https://doi.org/10.1103/PhysRevB.3.4286	journal	June 1971
Electronics and optoelectronics of two-dimensional transition metal dichalcogenides Wang, Qing Hua; Kalantar-Zadeh, Kourosh; Kis, Andras Nature Nanotechnology, Vol. 7, Issue 11, p. 699-712 https://doi.org/10.1038/nnano.2012.193	journal	November 2012
Light Generation and Harvesting in a van der Waals Heterostructure Lopez-Sanchez, Oriol; Alarcon Llado, Esther; Koman, Volodymyr ACS Nano, Vol. 8, Issue 3 https://doi.org/10.1021/nn500480u	journal	March 2014
The transition metal dichalcogenides discussion and interpretation of the observed optical, electrical and structural properties Wilson, J. A.; Yoffe, A. D. Advances in Physics, Vol. 18, Issue 73 https://doi.org/10.1080/00018736900101307	journal	May 1969
Band Structures of Transition-Metal-Dichalcogenide Layer Compounds Mattheiss, L. F. Physical Review B, Vol. 8, Issue 8 https://doi.org/10.1103/PhysRevB.8.3719	journal	October 1973
Optoelectronic devices based on electrically tunable p–n diodes in a monolayer dichalcogenide Baugher, Britton W. H.; Churchill, Hugh O. H.; Yang, Yafang Nature Nanotechnology, Vol. 9, Issue 4 https://doi.org/10.1038/nnano.2014.25	journal	March 2014
Kramers-Kronig analysis of the reflectivity spectra of 2H-MoS ₂ , 2H-MoSe ₂ and 2H-MoTe ₂ Beal, A. R.; Hughes, H. P. Journal of Physics C: Solid State Physics, Vol. 12, Issue 5 https://doi.org/10.1088/0022-3719/12/5/017	journal	March 1979
Two-dimensional atomic crystals Novoselov, K. S.; Jiang, D.; Schedin, F. Proceedings of the National Academy of Sciences, Vol. 102, Issue 30, p. 10451-10453 https://doi.org/10.1073/pnas.0502848102	journal	July 2005
Kramers–Kronig constrained variational analysis of optical spectra Kuzmenko, A. B. Review of Scientific Instruments, Vol. 76, Issue 8 https://doi.org/10.1063/1.1979470	journal	August 2005
Tightly bound trions in monolayer MoS2 Mak, Kin Fai; He, Keliang; Lee, Changgu Nature Materials, Vol. 12, Issue 3 https://doi.org/10.1038/nmat3505	journal	December 2012
Evolution of Electronic Structure in Atomically Thin Sheets of WS ₂ and WSe ₂ Zhao, Weijie; Ghorannevis, Zohreh; Chu, Leiqiang ACS Nano, Vol. 7, Issue 1 https://doi.org/10.1021/nn305275h	journal	December 2012
Exciton Binding Energy and Nonhydrogenic Rydberg Series in Monolayer ${WS}_{2}$ Chernikov, Alexey; Berkelbach, Timothy C.; Hill, Heather M. Physical Review Letters, Vol. 113, Issue 7 https://doi.org/10.1103/PhysRevLett.113.076802	journal	August 2014
Single-layer MoS₂ transistors Radisavljevic, B.; Radenovic, A.; Brivio, J. Nature Nanotechnology, Vol. 6, Issue 3, p. 147-150 https://doi.org/10.1038/nnano.2010.279	journal	January 2011
Kramers-Kronig analysis of the reflectivity spectra of 3R-WS ₂ and 2H-WSe ₂ Beal, A. R.; Liang, W. Y.; Hughes, H. P. Journal of Physics C: Solid State Physics, Vol. 9, Issue 12 https://doi.org/10.1088/0022-3719/9/12/027	journal	June 1976
Control of valley polarization in monolayer MoS2 by optical helicity Mak, Kin Fai; He, Keliang; Shan, Jie Nature Nanotechnology, Vol. 7, Issue 8 https://doi.org/10.1038/nnano.2012.96	journal	June 2012
Valley polarization in MoS2 monolayers by optical pumping Zeng, Hualing; Dai, Junfeng; Yao, Wang Nature Nanotechnology, Vol. 7, Issue 8 https://doi.org/10.1038/nnano.2012.95	journal	June 2012

Similar Records

Measurement of the optical dielectric function of monolayer transition-metal dichalcogenides:

{MoS}_{2}

Mo S e_{2}

{WS}_{2}

, and

WS e_{2}

Journal Article · Mon Nov 17 00:00:00 EST 2014 · Physical Review B · OSTI ID:1370378

Li, Yilei; Chernikov, Alexey; Zhang, Xian; +7 more

Time-dependent density-matrix functional theory for trion excitations: Application to monolayer

{MoS}_{2}

and other transition-metal dichalcogenides

Journal Article · Mon Aug 18 00:00:00 EDT 2014 · Physical Review B · OSTI ID:1370378

Ramirez-Torres, Alfredo; Turkowski, Volodymyr; Rahman, Talat S.

Lack of superconductivity in the phase diagram of single-crystalline

Eu {(F e_{1 - x} C o_{x})}_{2} A s_{2}

grown by transition metal arsenide flux

Journal Article · Tue Oct 02 00:00:00 EDT 2018 · Physical Review Materials · OSTI ID:1370378

Wang, Gang; Meier, William R.; Straszheim, Warren E.; +3 more

Title: Measurement of the optical dielectric function of monolayer transition-metal dichalcogenides: MoS 2 , Mo S e 2 , WS 2 , and WS e 2

Citation Formats

References (50)

Similar Records

Related Subjects

Title: Measurement of the optical dielectric function of monolayer transition-metal dichalcogenides: ${MoS}_{2}$ , $Mo S e_{2}$ , ${WS}_{2}$ , and $WS e_{2}$