Effects of strain relaxation in Pr0.67Sr0.33MnO3 films probed by polarization dependent X-ray absorption near edge structure

zhang, Bangmin; Chen, Jingsheng; Venkatesan, T.; Sun, Cheng -Jun; Heald, Steve M.; Chow, Gan Moog; Yang, Ping; Chi, Xiao; Lin, Weinan

doi:10.1038/srep19886

Title: Effects of strain relaxation in Pr_0.67Sr_0.33MnO₃ films probed by polarization dependent X-ray absorption near edge structure

Journal Article · Thu Jan 28 00:00:00 EST 2016 · Scientific Reports

DOI:https://doi.org/10.1038/srep19886· OSTI ID:1248885

zhang, Bangmin ^[1]; Chen, Jingsheng ^[1]; Venkatesan, T. ^[1]; Sun, Cheng -Jun ^[2]; Heald, Steve M. ^[2]; Chow, Gan Moog ^[1]; Yang, Ping ^[1]; Chi, Xiao ^[1]; Lin, Weinan ^[1]

National Univ. of Singapore (Singapore)
Argonne National Lab. (ANL), Argonne, IL (United States)

In this study, the Mn K edge X-ray absorption near edge structure (XANES) of Pr_0.67Sr_0.33MnO₃ films with different thicknesses on (001) LaAlO₃ substrate were measured, and the effects of strain relaxation on film properties were investigated. The films experienced in-plane compressive strain and out-of-plane tensile strain. Strain relaxation evolved with the film thickness. In the polarization dependent XANES measurements, the in-plane (parallel) and out-of-plane (perpendicular) XANES spectrocopies were anisotropic with different absorption energy E_r. The resonance energy Er along two directions shifted towards each other with increasing film thickness. Based on the X-ray diffraction results, it was suggested that the strain relaxation weakened the difference of the local environment and probability of electronic charge transfer (between Mn 3d and O 2p orbitals) along the in-plane and out-of-plane directions, which was responsible for the change of E_r. XANES is a useful tool to probe the electronic structures, of which the effects on magnetic properties with the strain relaxation was also been studied.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1248885

Journal Information:: Scientific Reports, Vol. 6, Issue 2; ISSN 2045-2322

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 12 works

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