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Title: Near-infrared strong coupling between metamaterials and epsilon-near-zero modes in degenerately doped semiconductor nanolayers

Journal Article · · ACS Photonics

Epsilon-near-zero (ENZ) modes provide a new path for tailoring light–matter interactions at the nanoscale. In this paper, we analyze a strongly coupled system at near-infrared frequencies comprising plasmonic metamaterial resonators and ENZ modes supported by degenerately doped semiconductor nanolayers. In strongly coupled systems that combine optical cavities and intersubband transitions, the polariton splitting (i.e., the ratio of Rabi frequency to bare cavity frequency) scales with the square root of the wavelength, thus favoring the long-wavelength regime. In contrast, we observe that the polariton splitting in ENZ/metamaterial resonator systems increases linearly with the thickness of the nanolayer supporting the ENZ modes. In this work, we employ an indium-tin-oxide nanolayer and observe a large experimental polariton splitting of approximately 30% in the near-infrared. As a result, this approach opens up many promising applications, including nonlinear optical components and tunable optical filters based on controlling the polariton splitting by adjusting the frequency of the ENZ mode.

Research Organization:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
AC04-94AL85000
OSTI ID:
1240096
Report Number(s):
SAND-2016-0643J; 618937
Journal Information:
ACS Photonics, Vol. 3, Issue 2; ISSN 2330-4022
Publisher:
American Chemical SocietyCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 61 works
Citation information provided by
Web of Science

References (32)

Quantum vacuum properties of the intersubband cavity polariton field journal September 2005
Quantum Vacuum Radiation Spectra from a Semiconductor Microcavity with a Time-Modulated Vacuum Rabi Frequency journal March 2007
Strong coupling between surface plasmon-polaritons and organic molecules in subwavelength hole arrays journal January 2005
Ultrastrong Light-Matter Coupling Regime with Polariton Dots journal November 2010
Ultrastrong Coupling of the Cyclotron Transition of a 2D Electron Gas to a THz Metamaterial journal March 2012
Strong coupling in the sub-wavelength limit using metamaterial nanocavities journal November 2013
Terahertz meta-atoms coupled to a quantum well intersubband transition journal January 2011
Electrodynamic modeling of strong coupling between a metasurface and intersubband transitions in quantum wells journal April 2014
Optical Strong Coupling between near-Infrared Metamaterials and Intersubband Transitions in III-Nitride Heterostructures journal September 2014
Epsilon-Near-Zero Strong Coupling in Metamaterial-Semiconductor Hybrid Structures journal October 2013
Ultra-strong light–matter coupling for designer Reststrahlen band journal April 2014
Epsilon-Near-Zero Modes for Tailored Light-Matter Interaction journal October 2015
Pursuing Near-Zero Response journal April 2013
Circuits with Light at Nanoscales: Optical Nanocircuits Inspired by Metamaterials journal September 2007
Boosting optical nonlinearities in ε -near-zero plasmonic channels journal January 2012
Low-damping epsilon-near-zero slabs: Nonlinear and nonlocal optical properties journal April 2013
Possible implementation of epsilon-near-zero metamaterials working at optical frequencies journal July 2012
Narrow-beam antennas using an artificial dielectric medium with permittivity less than unity journal January 1971
A Metamaterial for Directive Emission journal November 2002
Analysis of Directive Radiation From a Line Source in a Metamaterial Slab With Low Permittivity journal March 2006
Epsilon-near-zero metamaterials and electromagnetic sources: Tailoring the radiation phase pattern journal April 2007
Berreman mode and epsilon near zero mode journal January 2012
Epsilon-Near-Zero Mode for Active Optoelectronic Devices journal December 2012
Theory of epsilon-near-zero modes in ultrathin films journal March 2015
Conductive oxide thin films: Model systems for understanding and controlling surface plasmon resonance journal July 2009
Enhanced third harmonic generation from the epsilon-near-zero modes of ultrathin films journal April 2015
Brewster phenomena in a lossy waveguide used just under the cut-off thickness journal May 1980
Principles of Optics book January 1999
Directional perfect absorption using deep subwavelength low-permittivity films journal August 2014
Optical Modes of Vibration in an Ionic Crystal Slab Including Retardation. II. Radiative Region journal October 1966
Broadband Epsilon-Near-Zero Perfect Absorption in the Near-Infrared journal August 2015
Dysprosium-doped cadmium oxide as a gateway material for mid-infrared plasmonics journal February 2015

Cited By (11)

Monochromatic Multimode Antennas on Epsilon‐Near‐Zero Materials journal March 2019
Launching of hyperbolic phonon-polaritons in h-BN slabs by resonant metal plasmonic antennas journal July 2019
Large optical nonlinearity of nanoantennas coupled to an epsilon-near-zero material journal January 2018
Near-zero-index materials for photonics journal September 2019
Epsilon-Near-Zero Photonics: A New Platform for Integrated Devices journal March 2018
Suppression of near-field coupling in plasmonic antennas on epsilon-near-zero substrates journal January 2018
Excitation of epsilon-near-zero resonance in ultra-thin indium tin oxide shell embedded nanostructured optical fiber journal February 2018
Accumulation and directionality of large spontaneous emission enabled by epsilon-near-zero film journal January 2019
Accumulation and directionality of large spontaneous emission enabled by epsilon-near-zero film conference January 2019
Launching of hyperbolic phonon-polaritons in h-BN slabs by resonant metal plasmonic antennas text January 2019
Excitation of epsilon-near-zero resonance in ultra-thin indium tin oxide shell embedded nanostructured optical fiber preprint January 2017