Origin and elimination of photocurrent hysteresis by fullerene passivation in CH3NH3PbI3 planar heterojunction solar cells

Shao, Yuchuan; Xiao, Zhengguo; Bi, Cheng; Yuan, Yongbo; Huang, Jinsong

doi:10.1038/ncomms6784

Title: Origin and elimination of photocurrent hysteresis by fullerene passivation in CH₃NH₃PbI₃ planar heterojunction solar cells

Journal Article · Mon Dec 15 00:00:00 EST 2014 · Nature Communications

DOI:https://doi.org/10.1038/ncomms6784· OSTI ID:1237996

Shao, Yuchuan ^[1]; Xiao, Zhengguo ^[1]; Bi, Cheng ^[1]; Yuan, Yongbo ^[1]; Huang, Jinsong ^[1]

Univ. of Nebraska, Lincoln, NE (United States)

The large photocurrent hysteresis observed in many organometal trihalide perovskite solar cells has become a major hindrance impairing the ultimate performance and stability of these devices, while its origin was unknown. Here we demonstrate the trap states on the surface and grain boundaries of the perovskite materials to be the origin of photocurrent hysteresis and that the fullerene layers deposited on perovskites can effectively passivate these charge trap states and eliminate the notorious photocurrent hysteresis. Fullerenes deposited on the top of the perovskites reduce the trap density by two orders of magnitude and double the power conversion efficiency of CH₃NH₃PbI₃ solar cells. As a result, the elucidation of the origin of photocurrent hysteresis and its elimination by trap passivation in perovskite solar cells provides important directions for future enhancements to device efficiency.

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Research Organization:: Univ. of Nebraska, Lincoln, NE (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: EE0006709

OSTI ID:: 1237996

Journal Information:: Nature Communications, Vol. 5, Issue 37; Conference: The Origin and Elimination of Photocurrent Hysteresis in Perovskite Planar Heterojunction Solar Cell, Program—Symposium W: Perovskite-Based and Related Novel Material Solar Cells, Boston, MA (United States), 2 Dec 2014; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 2407 works

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Employing Lead Thiocyanate Additive to Reduce the Hysteresis and Boost the Fill Factor of Planar Perovskite Solar Cells Ke, Weijun; Xiao, Chuanxiao; Wang, Changlei Advanced Materials, Vol. 28, Issue 26 https://doi.org/10.1002/adma.201600594	journal	May 2016
Lead-Free Inverted Planar Formamidinium Tin Triiodide Perovskite Solar Cells Achieving Power Conversion Efficiencies up to 6.22% Liao, Weiqiang; Zhao, Dewei; Yu, Yue Advanced Materials, Vol. 28, Issue 42 https://doi.org/10.1002/adma.201602992	journal	August 2016
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Planar‐Structure Perovskite Solar Cells with Efficiency beyond 21% Jiang, Qi; Chu, Zema; Wang, Pengyang Advanced Materials, Vol. 29, Issue 46 https://doi.org/10.1002/adma.201703852	journal	October 2017
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Grain-Boundary “Patches” by In Situ Conversion to Enhance Perovskite Solar Cells Stability Liu, Lang; Huang, Sheng; Lu, Yue Advanced Materials, Vol. 30, Issue 29 https://doi.org/10.1002/adma.201800544	journal	June 2018
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One‐Step Inkjet Printed Perovskite in Air for Efficient Light Harvesting Liang, Chao; Li, Pengwei; Gu, Hao Solar RRL, Vol. 2, Issue 2 https://doi.org/10.1002/solr.201700217	journal	January 2018
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Hydrothermally Treated SnO ₂ as the Electron Transport Layer in High‐Efficiency Flexible Perovskite Solar Cells with a Certificated Efficiency of 17.3% Liu, Chang; Zhang, Luozheng; Zhou, Xianyong Advanced Functional Materials, Vol. 29, Issue 47 https://doi.org/10.1002/adfm.201807604	journal	May 2019
NbF ₅ : A Novel α‐Phase Stabilizer for FA‐Based Perovskite Solar Cells with High Efficiency Yuan, Shihao; Qian, Fang; Yang, Shaomin Advanced Functional Materials, Vol. 29, Issue 47 https://doi.org/10.1002/adfm.201807850	journal	February 2019
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Polymer-Passivated Inorganic Cesium Lead Mixed-Halide Perovskites for Stable and Efficient Solar Cells with High Open-Circuit Voltage over 1.3 V Zeng, Qingsen; Zhang, Xiaoyu; Feng, Xiaolei Advanced Materials, Vol. 30, Issue 9 https://doi.org/10.1002/adma.201705393	journal	January 2018
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Title: Origin and elimination of photocurrent hysteresis by fullerene passivation in CH3NH3PbI3 planar heterojunction solar cells

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Title: Origin and elimination of photocurrent hysteresis by fullerene passivation in CH₃NH₃PbI₃ planar heterojunction solar cells