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Title: The Northern Marshall Islands radiological survey: A quality control program for radiochemical and gamma spectroscopy analysis

Technical Report ·
DOI:https://doi.org/10.2172/120871· OSTI ID:120871

From 1979 to 1989, approximately 25,000 Post Northern Marshall Islands Radiological Survey (PNMIRS) samples were collected, and over 71,400 radiochemical and gamma spectroscopy analyses were performed to establish the concentration of {sup 90}Sr, {sup 137}Cs, {sup 241}Am, and plutonium isotopes in soil, vegetation, fish, and animals in the Northern Marshall Islands. While the Low Level Gamma Counting Facility (B379) in the Health and Ecological Assessment (HEA) division accounted for over 80% of all gamma spectroscopy analyses, approximately 4889 radiochemical and 5437 gamma spectroscopy analyses were performed on 4784 samples of soil, vegetation, terrestrial animal, and marine organisms by outside laboratories. Four laboratories were used by Lawrence Livermore National Laboratory (LLNL) to perform the radiochemical analyses: Thermo Analytical Norcal, Richmond, California (TMA); Nuclear Energy Services, North Carolina State University (NCSU); Laboratory of Radiation Ecology, University of Washington (LRE); and Health and Ecological Assessment (HEA) division, LLNL, Livermore, California. Additionally, LRE and NCSU were used to perform gamma spectroscopy analyses. The analytical precision and accuracy were monitored by including blind duplicates and natural matrix standards in each group of samples analyzed. On the basis of reported analytical values for duplicates and standards, 88% of the gamma and 87% of the radiochemical analyses in this survey were accepted. By laboratory, 93% of the radiochemical analyses by TMA; 88% of the gamma-ray spectrometry and 100% of the radiochemistry analyses by NCSU; 89% of the gamma spectroscopy and 87% of the radiochemistry analyses by LRE; and 90% of the radiochemistry analyses performed by HEA`s radiochemistry department were accepted.

Research Organization:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Sponsoring Organization:
USDOE, Washington, DC (United States)
DOE Contract Number:
W-7405-ENG-48
OSTI ID:
120871
Report Number(s):
UCRL-ID-120429; ON: DE96001872; TRN: 95:024560
Resource Relation:
Other Information: PBD: Sep 1995
Country of Publication:
United States
Language:
English